Chemoselective (Hetero)Arene Electroreduction Enabled by Rapid Alternating Polarity
2
Abbvie Process Research and Development, 1401 North Sheridan Road, North Chicago, Illinois 60064, United States
|
Publication type: Journal Article
Publication date: 2022-03-29
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
35347984
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
Conventional chemical and even electrochemical Birch-type reductions suffer from a lack of chemoselectivity due to a reliance on alkali metals or harshly reducing conditions. This study reveals that a simpler avenue is available for such reductions by simply altering the waveform of current delivery, namely rapid alternating polarity (rAP). The developed method solves these issues, proceeding in a protic solvent, and can be easily scaled up without any metal additives or stringently anhydrous conditions.
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Metrics
108
Total citations:
108
Citations from 2024:
66
(61.11%)
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MLA
Cite this
GOST
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Hayashi K. et al. Chemoselective (Hetero)Arene Electroreduction Enabled by Rapid Alternating Polarity // Journal of the American Chemical Society. 2022. Vol. 144. No. 13. pp. 5762-5768.
GOST all authors (up to 50)
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Hayashi K., Griffin J., Harper K. C., Kawamata Yu., Baran P. S. Chemoselective (Hetero)Arene Electroreduction Enabled by Rapid Alternating Polarity // Journal of the American Chemical Society. 2022. Vol. 144. No. 13. pp. 5762-5768.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/jacs.2c02102
UR - https://doi.org/10.1021/jacs.2c02102
TI - Chemoselective (Hetero)Arene Electroreduction Enabled by Rapid Alternating Polarity
T2 - Journal of the American Chemical Society
AU - Hayashi, Kyohei
AU - Griffin, Jeremy
AU - Harper, Kaid C
AU - Kawamata, Yu
AU - Baran, Phil S
PY - 2022
DA - 2022/03/29
PB - American Chemical Society (ACS)
SP - 5762-5768
IS - 13
VL - 144
PMID - 35347984
SN - 0002-7863
SN - 1520-5126
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2022_Hayashi,
author = {Kyohei Hayashi and Jeremy Griffin and Kaid C Harper and Yu Kawamata and Phil S Baran},
title = {Chemoselective (Hetero)Arene Electroreduction Enabled by Rapid Alternating Polarity},
journal = {Journal of the American Chemical Society},
year = {2022},
volume = {144},
publisher = {American Chemical Society (ACS)},
month = {mar},
url = {https://doi.org/10.1021/jacs.2c02102},
number = {13},
pages = {5762--5768},
doi = {10.1021/jacs.2c02102}
}
Cite this
MLA
Copy
Hayashi, Kyohei, et al. “Chemoselective (Hetero)Arene Electroreduction Enabled by Rapid Alternating Polarity.” Journal of the American Chemical Society, vol. 144, no. 13, Mar. 2022, pp. 5762-5768. https://doi.org/10.1021/jacs.2c02102.