High-Temperature Ferroelectricity and Photoluminescence in a Hybrid Organic–Inorganic Compound: (3-Pyrrolinium)MnCl3
Heng-Yun Ye
1
,
Zhou Qionghua
2
,
Xianghong Niu
2
,
Wei-Qiang Liao
1
,
Da-Wei Fu
1
,
Yi Zhang
1
,
Yu-Meng You
1
,
Jinlan Wang
2
,
Zhong-Ning Chen
3
,
Ren-Gen Xiong
1
Publication type: Journal Article
Publication date: 2015-09-29
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
26383504
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
Coupling of ferroelectricity and optical properties has become an interesting aspect of material research. The switchable spontaneous polarization in ferroelectrics provides an alternative way to manipulate the light-matter interaction. The recent observation of strong photoluminescence emission in ferroelectric hybrid organic-inorganic compounds, (pyrrolidinium)MnX3 (X = Cl or Br), is an attractive approach to high efficiency luminescence with the advantages of ferroelectricity. However, (pyrrolidinium)MnX3 only displays ferroelectricity near or below room temperature, which limits its future applications in optoelectronics and multifunctional devices. Here, we rationally designed and synthesized high-temperature luminescent ferroelectric materials. The new hybrid compound (3-pyrrolinium)MnCl3 has a very high Curie temperature, Tc = 376 K, large spontaneous electronic polarization of 6.2 μC/cm(2), and high fatigue resistance, as well as high emission efficiency of 28%. This finding is a further step to the practical use of ferroelectric luminescence based on organic-inorganic compounds.
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Ye H. et al. High-Temperature Ferroelectricity and Photoluminescence in a Hybrid Organic–Inorganic Compound: (3-Pyrrolinium)MnCl3 // Journal of the American Chemical Society. 2015. Vol. 137. No. 40. pp. 13148-13154.
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Ye H., Qionghua Z., Niu X., Liao W., Fu D., Zhang Y., You Y., Wang J., Chen Z., Xiong R. High-Temperature Ferroelectricity and Photoluminescence in a Hybrid Organic–Inorganic Compound: (3-Pyrrolinium)MnCl3 // Journal of the American Chemical Society. 2015. Vol. 137. No. 40. pp. 13148-13154.
Cite this
RIS
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TY - JOUR
DO - 10.1021/jacs.5b08290
UR - https://doi.org/10.1021/jacs.5b08290
TI - High-Temperature Ferroelectricity and Photoluminescence in a Hybrid Organic–Inorganic Compound: (3-Pyrrolinium)MnCl3
T2 - Journal of the American Chemical Society
AU - Ye, Heng-Yun
AU - Qionghua, Zhou
AU - Niu, Xianghong
AU - Liao, Wei-Qiang
AU - Fu, Da-Wei
AU - Zhang, Yi
AU - You, Yu-Meng
AU - Wang, Jinlan
AU - Chen, Zhong-Ning
AU - Xiong, Ren-Gen
PY - 2015
DA - 2015/09/29
PB - American Chemical Society (ACS)
SP - 13148-13154
IS - 40
VL - 137
PMID - 26383504
SN - 0002-7863
SN - 1520-5126
ER -
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@article{2015_Ye,
author = {Heng-Yun Ye and Zhou Qionghua and Xianghong Niu and Wei-Qiang Liao and Da-Wei Fu and Yi Zhang and Yu-Meng You and Jinlan Wang and Zhong-Ning Chen and Ren-Gen Xiong},
title = {High-Temperature Ferroelectricity and Photoluminescence in a Hybrid Organic–Inorganic Compound: (3-Pyrrolinium)MnCl3},
journal = {Journal of the American Chemical Society},
year = {2015},
volume = {137},
publisher = {American Chemical Society (ACS)},
month = {sep},
url = {https://doi.org/10.1021/jacs.5b08290},
number = {40},
pages = {13148--13154},
doi = {10.1021/jacs.5b08290}
}
Cite this
MLA
Copy
Ye, Heng-Yun, et al. “High-Temperature Ferroelectricity and Photoluminescence in a Hybrid Organic–Inorganic Compound: (3-Pyrrolinium)MnCl3.” Journal of the American Chemical Society, vol. 137, no. 40, Sep. 2015, pp. 13148-13154. https://doi.org/10.1021/jacs.5b08290.