Spin Frustration in an Organic Radical Ion Salt Based on a Kagome-Coupled Chain Structure
Lars Postulka
1
,
Stephen M Winter
1
,
Adam G Mihailov
2
,
Aaron Mailman
2
,
Abdeljalil Assoud
2
,
Craig A. Robertson
3
,
Bernd Wolf
1
,
Michael Lang
1
,
Richard Oakley
2
Publication type: Journal Article
Publication date: 2016-08-18
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
27537064
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
Electro-oxidation of the quinoidal bisdithiazole BT in dichloroethane in the presence of [Bu4N][GaBr4] affords the 1:1 radical ion salt [BT][GaBr4], crystals of which belong to the trigonal space group P3. The packing pattern of the radical cations provides a rare example of an organic kagome basket structure, with S = 1/2 radical ion chains located at the triangular corners of a trihexagonal lattice. Magnetic measurements over a wide temperature range from 30 mK to 300 K suggest strongly frustrated AFM interactions on the scale of J/kb ∼ 30 K, but reveal no anomalies that would be associated with magnetic order. These observations are discussed in terms of the symmetry allowed magnetic interactions within and between the frustrated layers.
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Total citations:
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Citations from 2024:
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Postulka L. et al. Spin Frustration in an Organic Radical Ion Salt Based on a Kagome-Coupled Chain Structure // Journal of the American Chemical Society. 2016. Vol. 138. No. 34. pp. 10738-10741.
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Postulka L., Winter S. M., Mihailov A. G., Mailman A., Assoud A., Robertson C. A., Wolf B., Lang M., Oakley R. Spin Frustration in an Organic Radical Ion Salt Based on a Kagome-Coupled Chain Structure // Journal of the American Chemical Society. 2016. Vol. 138. No. 34. pp. 10738-10741.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/jacs.6b05079
UR - https://doi.org/10.1021/jacs.6b05079
TI - Spin Frustration in an Organic Radical Ion Salt Based on a Kagome-Coupled Chain Structure
T2 - Journal of the American Chemical Society
AU - Postulka, Lars
AU - Winter, Stephen M
AU - Mihailov, Adam G
AU - Mailman, Aaron
AU - Assoud, Abdeljalil
AU - Robertson, Craig A.
AU - Wolf, Bernd
AU - Lang, Michael
AU - Oakley, Richard
PY - 2016
DA - 2016/08/18
PB - American Chemical Society (ACS)
SP - 10738-10741
IS - 34
VL - 138
PMID - 27537064
SN - 0002-7863
SN - 1520-5126
ER -
Cite this
BibTex (up to 50 authors)
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@article{2016_Postulka,
author = {Lars Postulka and Stephen M Winter and Adam G Mihailov and Aaron Mailman and Abdeljalil Assoud and Craig A. Robertson and Bernd Wolf and Michael Lang and Richard Oakley},
title = {Spin Frustration in an Organic Radical Ion Salt Based on a Kagome-Coupled Chain Structure},
journal = {Journal of the American Chemical Society},
year = {2016},
volume = {138},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/jacs.6b05079},
number = {34},
pages = {10738--10741},
doi = {10.1021/jacs.6b05079}
}
Cite this
MLA
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Postulka, Lars, et al. “Spin Frustration in an Organic Radical Ion Salt Based on a Kagome-Coupled Chain Structure.” Journal of the American Chemical Society, vol. 138, no. 34, Aug. 2016, pp. 10738-10741. https://doi.org/10.1021/jacs.6b05079.