Solution Synthesis of Semiconducting Two-Dimensional Polymer via Trimerization of Carbonitrile
Publication type: Journal Article
Publication date: 2017-07-24
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
28685573
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
The synthesis of crystalline two-dimensional polymers (2DPs) with proper bandgaps and well-defined repeating units presents a great challenge to synthetic chemists. Here we report the first solution synthesis of a single-layer/few-layer triazine-based 2DP via trimerization of carbonitrile at the interface of dichloromethane and trifluoromethanesulfonic acid. The processable triazine-based 2DP can be assembled into mechanically strong layered free-standing films with a high specific surface area via filtration. Moreover, the highly crystalline triazine-based 2DP can function as the active semiconducting layer in a field-effect transistor via drop coating and exhibits slightly bipolar behavior with a high on/off ratio of 103 and a remarkable mobility of 0.15 cm2 V-1 s-1.
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Total citations:
200
Citations from 2024:
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(14%)
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GOST
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Liu J. et al. Solution Synthesis of Semiconducting Two-Dimensional Polymer via Trimerization of Carbonitrile // Journal of the American Chemical Society. 2017. Vol. 139. No. 34. pp. 11666-11669.
GOST all authors (up to 50)
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Liu J., Wu Z., Li K., Yang Y., Bu F., Xu Y. Solution Synthesis of Semiconducting Two-Dimensional Polymer via Trimerization of Carbonitrile // Journal of the American Chemical Society. 2017. Vol. 139. No. 34. pp. 11666-11669.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/jacs.7b05025
UR - https://doi.org/10.1021/jacs.7b05025
TI - Solution Synthesis of Semiconducting Two-Dimensional Polymer via Trimerization of Carbonitrile
T2 - Journal of the American Chemical Society
AU - Liu, Jingjing
AU - Wu, Zan
AU - Li, Ke
AU - Yang, Yang
AU - Bu, Fan-Xing
AU - Xu, Yuxi
PY - 2017
DA - 2017/07/24
PB - American Chemical Society (ACS)
SP - 11666-11669
IS - 34
VL - 139
PMID - 28685573
SN - 0002-7863
SN - 1520-5126
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2017_Liu,
author = {Jingjing Liu and Zan Wu and Ke Li and Yang Yang and Fan-Xing Bu and Yuxi Xu},
title = {Solution Synthesis of Semiconducting Two-Dimensional Polymer via Trimerization of Carbonitrile},
journal = {Journal of the American Chemical Society},
year = {2017},
volume = {139},
publisher = {American Chemical Society (ACS)},
month = {jul},
url = {https://doi.org/10.1021/jacs.7b05025},
number = {34},
pages = {11666--11669},
doi = {10.1021/jacs.7b05025}
}
Cite this
MLA
Copy
Liu, Jingjing, et al. “Solution Synthesis of Semiconducting Two-Dimensional Polymer via Trimerization of Carbonitrile.” Journal of the American Chemical Society, vol. 139, no. 34, Jul. 2017, pp. 11666-11669. https://doi.org/10.1021/jacs.7b05025.