Metal-Free Photocatalyst for H2 Evolution in Visible to Near-Infrared Region: Black Phosphorus/Graphitic Carbon Nitride
Ming-Shan Zhu
1
,
Sooyeon Kim
1
,
Liang Mao
2
,
Mamoru Fujitsuka
1
,
Junying Zhang
2
,
Xinchen Wang
3
,
Tetsuro Majima
1
Publication type: Journal Article
Publication date: 2017-09-08
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
28856885
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
In the drive toward green and sustainable chemistry, exploring efficient and stable metal-free photocatalysts with broadband solar absorption from the UV to near-infrared region for the photoreduction of water to H2 remains a big challenge. To this end, a binary nanohybrid (BP/CN) of two-dimensional (2D) black phosphorus (BP) and graphitic carbon nitride (CN) was designed and used as a metal-free photocatalyst for the first time. During irradiation of BP/CN in water with >420 and >780 nm light, solid H2 gas was generated, respectively. Owing to the interfacial interaction between BP and CN, efficient charge transfer occurred, thereby enhancing the photocatalytic performance. The efficient charge-trapping and transfer processes were thoroughly investigated with time-resolved diffuse reflectance spectroscopic measurement. The present results show that BP/CN is a metal-free photocatalyst for artificial photosynthesis and renewable energy conversion.
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Total citations:
990
Citations from 2025:
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Zhu M. et al. Metal-Free Photocatalyst for H2 Evolution in Visible to Near-Infrared Region: Black Phosphorus/Graphitic Carbon Nitride // Journal of the American Chemical Society. 2017. Vol. 139. No. 37. pp. 13234-13242.
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Zhu M., Kim S., Mao L., Fujitsuka M., Zhang J., Wang X., Majima T. Metal-Free Photocatalyst for H2 Evolution in Visible to Near-Infrared Region: Black Phosphorus/Graphitic Carbon Nitride // Journal of the American Chemical Society. 2017. Vol. 139. No. 37. pp. 13234-13242.
Cite this
RIS
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TY - JOUR
DO - 10.1021/jacs.7b08416
UR - https://doi.org/10.1021/jacs.7b08416
TI - Metal-Free Photocatalyst for H2 Evolution in Visible to Near-Infrared Region: Black Phosphorus/Graphitic Carbon Nitride
T2 - Journal of the American Chemical Society
AU - Zhu, Ming-Shan
AU - Kim, Sooyeon
AU - Mao, Liang
AU - Fujitsuka, Mamoru
AU - Zhang, Junying
AU - Wang, Xinchen
AU - Majima, Tetsuro
PY - 2017
DA - 2017/09/08
PB - American Chemical Society (ACS)
SP - 13234-13242
IS - 37
VL - 139
PMID - 28856885
SN - 0002-7863
SN - 1520-5126
ER -
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BibTex (up to 50 authors)
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@article{2017_Zhu,
author = {Ming-Shan Zhu and Sooyeon Kim and Liang Mao and Mamoru Fujitsuka and Junying Zhang and Xinchen Wang and Tetsuro Majima},
title = {Metal-Free Photocatalyst for H2 Evolution in Visible to Near-Infrared Region: Black Phosphorus/Graphitic Carbon Nitride},
journal = {Journal of the American Chemical Society},
year = {2017},
volume = {139},
publisher = {American Chemical Society (ACS)},
month = {sep},
url = {https://doi.org/10.1021/jacs.7b08416},
number = {37},
pages = {13234--13242},
doi = {10.1021/jacs.7b08416}
}
Cite this
MLA
Copy
Zhu, Ming-Shan, et al. “Metal-Free Photocatalyst for H2 Evolution in Visible to Near-Infrared Region: Black Phosphorus/Graphitic Carbon Nitride.” Journal of the American Chemical Society, vol. 139, no. 37, Sep. 2017, pp. 13234-13242. https://doi.org/10.1021/jacs.7b08416.