Preparation, Properties, and Structures of the Radical Anions and Dianions of Azapentacenes
Тип публикации: Journal Article
Дата публикации: 2017-10-26
scimago Q1
wos Q1
БС1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
28988473
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Краткое описание
A series of diazapentacenes (5,14-diethynyldibenzo[b,i]phenazine, 6,13-diethynylnaphtho[2,3-b]phenazine) and tetraazapentacenes (7,12-diethynylbenzo[g]quinoxalino[2,3-b]quinoxaline, 6,13-diethynylquinoxalino[2,3-b]phenazine) were reduced to their radical anions and dianions, employing either potassium anthracenide or lithium naphthalenide in THF. The anionic species formed were investigated by UV-vis-NIR, fluorescence and EPR spectroscopy, spectroelectrochemistry, and quantum chemical calculations. Single crystal X-ray structures of three of their radical anions and of three of their dianions were obtained. In contrast to the acenes, the anions of the azapentacenes are persistent and, in some cases, even moderately stable toward air, and were characterized.
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Ji L. et al. Preparation, Properties, and Structures of the Radical Anions and Dianions of Azapentacenes // Journal of the American Chemical Society. 2017. Vol. 139. No. 44. pp. 15968-15976.
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Ji L., Friedrich A., Krummenacher I., Eichhorn A., Braunschweig H., Moos M., Hahn S., Geyer F. L., Tverskoy O., Han J., Lambert C., Dreuw A., Marder T. B., Bunz U. H. F. Preparation, Properties, and Structures of the Radical Anions and Dianions of Azapentacenes // Journal of the American Chemical Society. 2017. Vol. 139. No. 44. pp. 15968-15976.
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TY - JOUR
DO - 10.1021/jacs.7b09460
UR - https://doi.org/10.1021/jacs.7b09460
TI - Preparation, Properties, and Structures of the Radical Anions and Dianions of Azapentacenes
T2 - Journal of the American Chemical Society
AU - Ji, Lei
AU - Friedrich, Alexandra
AU - Krummenacher, Ivo
AU - Eichhorn, Antonius
AU - Braunschweig, Holger
AU - Moos, Michael
AU - Hahn, Sebastian
AU - Geyer, Florian L.
AU - Tverskoy, Olena
AU - Han, Jie
AU - Lambert, Christoph
AU - Dreuw, Andreas
AU - Marder, Todd B.
AU - Bunz, Uwe H. F.
PY - 2017
DA - 2017/10/26
PB - American Chemical Society (ACS)
SP - 15968-15976
IS - 44
VL - 139
PMID - 28988473
SN - 0002-7863
SN - 1520-5126
ER -
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@article{2017_Ji,
author = {Lei Ji and Alexandra Friedrich and Ivo Krummenacher and Antonius Eichhorn and Holger Braunschweig and Michael Moos and Sebastian Hahn and Florian L. Geyer and Olena Tverskoy and Jie Han and Christoph Lambert and Andreas Dreuw and Todd B. Marder and Uwe H. F. Bunz},
title = {Preparation, Properties, and Structures of the Radical Anions and Dianions of Azapentacenes},
journal = {Journal of the American Chemical Society},
year = {2017},
volume = {139},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/jacs.7b09460},
number = {44},
pages = {15968--15976},
doi = {10.1021/jacs.7b09460}
}
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MLA
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Ji, Lei, et al. “Preparation, Properties, and Structures of the Radical Anions and Dianions of Azapentacenes.” Journal of the American Chemical Society, vol. 139, no. 44, Oct. 2017, pp. 15968-15976. https://doi.org/10.1021/jacs.7b09460.