Iron-Catalyzed Highly Enantioselective Hydrosilylation of Unactivated Terminal Alkenes
Тип публикации: Journal Article
Дата публикации: 2018-03-28
SCImago Q1
Tоп 10% SCImago
WOS Q1
БС1
SJR: 5.491
CiteScore: 22
Impact factor: 16.6
ISSN: 00027863, 15205126
PubMed ID:
29589919
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Краткое описание
The iron-catalyzed highly Markovnikov-type selective and enantioselective hydrosilylation of terminal aliphatic alkenes with good functional group tolerance is developed. This operationally simple protocol uses earth-abundant transition metal catalyst, readily available aliphatic alkenes and hydrosilanes to construct valuable chiral organosilanes with better than 99% ee in most cases. The chiral aliphatic alkan-2-ol and chiral dihydroxysilane as an analogue of ketone could be efficiently synthesized via further derivatization of chiral organosilanes without any racemization.
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ГОСТ
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Cheng B., Liu W., Lu Z. Iron-Catalyzed Highly Enantioselective Hydrosilylation of Unactivated Terminal Alkenes // Journal of the American Chemical Society. 2018. Vol. 140. No. 15. pp. 5014-5017.
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Cheng B., Liu W., Lu Z. Iron-Catalyzed Highly Enantioselective Hydrosilylation of Unactivated Terminal Alkenes // Journal of the American Chemical Society. 2018. Vol. 140. No. 15. pp. 5014-5017.
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RIS
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TY - JOUR
DO - 10.1021/jacs.8b01638
UR - https://doi.org/10.1021/jacs.8b01638
TI - Iron-Catalyzed Highly Enantioselective Hydrosilylation of Unactivated Terminal Alkenes
T2 - Journal of the American Chemical Society
AU - Cheng, Biao
AU - Liu, Wenbo
AU - Lu, Zhan
PY - 2018
DA - 2018/03/28
PB - American Chemical Society (ACS)
SP - 5014-5017
IS - 15
VL - 140
PMID - 29589919
SN - 0002-7863
SN - 1520-5126
ER -
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BibTex (до 50 авторов)
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@article{2018_Cheng,
author = {Biao Cheng and Wenbo Liu and Zhan Lu},
title = {Iron-Catalyzed Highly Enantioselective Hydrosilylation of Unactivated Terminal Alkenes},
journal = {Journal of the American Chemical Society},
year = {2018},
volume = {140},
publisher = {American Chemical Society (ACS)},
month = {mar},
url = {https://doi.org/10.1021/jacs.8b01638},
number = {15},
pages = {5014--5017},
doi = {10.1021/jacs.8b01638}
}
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MLA
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Cheng, Biao, et al. “Iron-Catalyzed Highly Enantioselective Hydrosilylation of Unactivated Terminal Alkenes.” Journal of the American Chemical Society, vol. 140, no. 15, Mar. 2018, pp. 5014-5017. https://doi.org/10.1021/jacs.8b01638.
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