Terahertz HgTe Nanocrystals: Beyond Confinement
Nicolas Goubet
1, 2, 3
,
Amardeep Jagtap
1
,
Clément Livache
1, 2, 3
,
Bertille Martinez
1, 2, 3
,
Hervé Portalès
4
,
Xiang-Zhen Xu
2, 3
,
R.P.S.M. Lobo
2, 3
,
Benoît Dubertret
2, 3
,
1
2
Publication type: Journal Article
Publication date: 2018-04-04
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
29617124
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
We report the synthesis of nanocrystals with an optical feature in the THz range. To do so, we develop a new synthetic procedure for the growth of HgTe, HgSe, and HgS nanocrystals, with strong size tunability from 5 to 200 nm. This is used to tune the absorption of the nanocrystals all over the infrared range up to terahertz (from 2 to 65 μm for absorption peak and even 200 μm for cutoff wavelength). The interest for this procedure is not limited to large sizes since for small objects we demonstrate low aggregation and good shape control (i.e., spherical object) while using nonexpansive and simple mercury halogenide precursors. By integrating these nanocrystals into an electrolyte-gated transistor, we evidence a change of carrier density from p-doped to n-doped as the confinement is vanishing.
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Metrics
131
Total citations:
131
Citations from 2024:
29
(22.14%)
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GOST
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Goubet N. et al. Terahertz HgTe Nanocrystals: Beyond Confinement // Journal of the American Chemical Society. 2018. Vol. 140. No. 15. pp. 5033-5036.
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Goubet N., Jagtap A., Livache C., Martinez B., Portalès H., Xu X., Lobo R., Dubertret B., Lhuillier E. Terahertz HgTe Nanocrystals: Beyond Confinement // Journal of the American Chemical Society. 2018. Vol. 140. No. 15. pp. 5033-5036.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/jacs.8b02039
UR - https://doi.org/10.1021/jacs.8b02039
TI - Terahertz HgTe Nanocrystals: Beyond Confinement
T2 - Journal of the American Chemical Society
AU - Goubet, Nicolas
AU - Jagtap, Amardeep
AU - Livache, Clément
AU - Martinez, Bertille
AU - Portalès, Hervé
AU - Xu, Xiang-Zhen
AU - Lobo, R.P.S.M.
AU - Dubertret, Benoît
AU - Lhuillier, Emmanuel
PY - 2018
DA - 2018/04/04
PB - American Chemical Society (ACS)
SP - 5033-5036
IS - 15
VL - 140
PMID - 29617124
SN - 0002-7863
SN - 1520-5126
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2018_Goubet,
author = {Nicolas Goubet and Amardeep Jagtap and Clément Livache and Bertille Martinez and Hervé Portalès and Xiang-Zhen Xu and R.P.S.M. Lobo and Benoît Dubertret and Emmanuel Lhuillier},
title = {Terahertz HgTe Nanocrystals: Beyond Confinement},
journal = {Journal of the American Chemical Society},
year = {2018},
volume = {140},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/jacs.8b02039},
number = {15},
pages = {5033--5036},
doi = {10.1021/jacs.8b02039}
}
Cite this
MLA
Copy
Goubet, Nicolas, et al. “Terahertz HgTe Nanocrystals: Beyond Confinement.” Journal of the American Chemical Society, vol. 140, no. 15, Apr. 2018, pp. 5033-5036. https://doi.org/10.1021/jacs.8b02039.