A Carbon Nitride/Fe Quaterpyridine Catalytic System for Photostimulated CO2-to-CO Conversion with Visible Light
Claudio Cometto
1
,
Ryo Kuriki
2, 3
,
Lingjing Chen
4
,
Kazuhiko Maeda
2
,
Tai Tap Lau
5
,
Osamu Ishitani
2
,
Publication type: Journal Article
Publication date: 2018-06-11
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
29888920
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
Efficient and selective photostimulated CO2-to-CO reduction by a photocatalytic system consisting of an iron-complex catalyst and a mesoporous graphitic carbon nitride (mpg-C3N4) redox photosensitizer is reported for the first time. Irradiation in the visible region (λ ≥ 400 nm) of an CH3CN/triethanolamine (4:1, v/v) solution containing [Fe(qpy)(H2O)2]2+ (qpy = 2,2':6',2'':6'',2''-quaterpyridine) and mpg-C3N4 resulted in CO evolution with 97% selectivity, a turnover number of 155, and an apparent quantum yield of ca. 4.2%. This hybrid catalytic system, comprising only earth abundant elements, opens new perspectives for solar fuels production using CO2 as a renewable feedstock.
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Total citations:
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Citations from 2024:
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GOST
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Cometto C. et al. A Carbon Nitride/Fe Quaterpyridine Catalytic System for Photostimulated CO2-to-CO Conversion with Visible Light // Journal of the American Chemical Society. 2018. Vol. 140. No. 24. pp. 7437-7440.
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Cometto C., Kuriki R., Chen L., Maeda K., Lau T. T., Ishitani O., Robert M. A Carbon Nitride/Fe Quaterpyridine Catalytic System for Photostimulated CO2-to-CO Conversion with Visible Light // Journal of the American Chemical Society. 2018. Vol. 140. No. 24. pp. 7437-7440.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/jacs.8b04007
UR - https://doi.org/10.1021/jacs.8b04007
TI - A Carbon Nitride/Fe Quaterpyridine Catalytic System for Photostimulated CO2-to-CO Conversion with Visible Light
T2 - Journal of the American Chemical Society
AU - Cometto, Claudio
AU - Kuriki, Ryo
AU - Chen, Lingjing
AU - Maeda, Kazuhiko
AU - Lau, Tai Tap
AU - Ishitani, Osamu
AU - Robert, Marc
PY - 2018
DA - 2018/06/11
PB - American Chemical Society (ACS)
SP - 7437-7440
IS - 24
VL - 140
PMID - 29888920
SN - 0002-7863
SN - 1520-5126
ER -
Cite this
BibTex (up to 50 authors)
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@article{2018_Cometto,
author = {Claudio Cometto and Ryo Kuriki and Lingjing Chen and Kazuhiko Maeda and Tai Tap Lau and Osamu Ishitani and Marc Robert},
title = {A Carbon Nitride/Fe Quaterpyridine Catalytic System for Photostimulated CO2-to-CO Conversion with Visible Light},
journal = {Journal of the American Chemical Society},
year = {2018},
volume = {140},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/jacs.8b04007},
number = {24},
pages = {7437--7440},
doi = {10.1021/jacs.8b04007}
}
Cite this
MLA
Copy
Cometto, Claudio, et al. “A Carbon Nitride/Fe Quaterpyridine Catalytic System for Photostimulated CO2-to-CO Conversion with Visible Light.” Journal of the American Chemical Society, vol. 140, no. 24, Jun. 2018, pp. 7437-7440. https://doi.org/10.1021/jacs.8b04007.