Photoreforming of Lignocellulose into H2 Using Nanoengineered Carbon Nitride under Benign Conditions
Тип публикации: Journal Article
Дата публикации: 2018-08-28
SCImago Q1
Tоп 10% SCImago
WOS Q1
БС1
SJR: 5.491
CiteScore: 22
Impact factor: 16.6
ISSN: 00027863, 15205126
PubMed ID:
30153420
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Краткое описание
Photoreforming of lignocellulose is a promising approach toward sustainable H2 generation, but this kinetically challenging reaction currently requires UV-absorbing or toxic light absorbers under harsh conditions. Here, we report a cyanamide-functionalized carbon nitride, NCNCNx, which shows enhanced performance upon ultrasonication. This activated NCNCNx allows for the visible-light driven conversion of purified and raw lignocellulose samples into H2 in the presence of various proton reduction cocatalysts. The reported room-temperature photoreforming process operates under benign aqueous conditions (pH ≈ 2-15) without the need for toxic components.
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MLA
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ГОСТ
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Kasap H. et al. Photoreforming of Lignocellulose into H2 Using Nanoengineered Carbon Nitride under Benign Conditions // Journal of the American Chemical Society. 2018. Vol. 140. No. 37. pp. 11604-11607.
ГОСТ со всеми авторами (до 50)
Скопировать
Kasap H., Achilleos D. S., Huang A., Reisner E. Photoreforming of Lignocellulose into H2 Using Nanoengineered Carbon Nitride under Benign Conditions // Journal of the American Chemical Society. 2018. Vol. 140. No. 37. pp. 11604-11607.
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RIS
Скопировать
TY - JOUR
DO - 10.1021/jacs.8b07853
UR - https://pubs.acs.org/doi/10.1021/jacs.8b07853
TI - Photoreforming of Lignocellulose into H2 Using Nanoengineered Carbon Nitride under Benign Conditions
T2 - Journal of the American Chemical Society
AU - Kasap, Hatice
AU - Achilleos, Demetra S
AU - Huang, Ailun
AU - Reisner, Erwin
PY - 2018
DA - 2018/08/28
PB - American Chemical Society (ACS)
SP - 11604-11607
IS - 37
VL - 140
PMID - 30153420
SN - 0002-7863
SN - 1520-5126
ER -
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BibTex (до 50 авторов)
Скопировать
@article{2018_Kasap,
author = {Hatice Kasap and Demetra S Achilleos and Ailun Huang and Erwin Reisner},
title = {Photoreforming of Lignocellulose into H2 Using Nanoengineered Carbon Nitride under Benign Conditions},
journal = {Journal of the American Chemical Society},
year = {2018},
volume = {140},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://pubs.acs.org/doi/10.1021/jacs.8b07853},
number = {37},
pages = {11604--11607},
doi = {10.1021/jacs.8b07853}
}
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MLA
Скопировать
Kasap, Hatice, et al. “Photoreforming of Lignocellulose into H2 Using Nanoengineered Carbon Nitride under Benign Conditions.” Journal of the American Chemical Society, vol. 140, no. 37, Aug. 2018, pp. 11604-11607. https://pubs.acs.org/doi/10.1021/jacs.8b07853.
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