A General Strategy for Fabricating Isolated Single Metal Atomic Site Catalysts in Y Zeolite
Yi Wei Liu
1
,
Zhi Li
1
,
Qiuying Yu
2
,
Yanfei Chen
3
,
Ziwei Chai
4
,
Guofeng Zhao
5
,
Shoujie Liu
6
,
Weng Chon Cheong
1
,
Yuan Pan
1
,
Qinghua Zhang
7
,
Lin Gu
7
,
Li-Rong Zheng
8
,
Yu Wang
9
,
Yong Lu
5
,
Dingsheng Wang
1
,
C. Chen
1
,
Qing Peng
1
,
Yunqi Liu
3
,
Li-Min Liu
4
,
Jie Sheng Chen
2
,
Yadong Li
1
2
5
Publication type: Journal Article
Publication date: 2019-05-22
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
31117651
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
Exploring high-performance zeolite-supported metal catalysts is of great significance. Herein, we develop a strategy for fabricating isolated single metal atomic site catalysts in Y zeolite (M-ISAS@Y, M = Pt, Pd, Ru, Rh, Co, Ni, Cu) by in situ separating and confining a metal-ethanediamine complex into β-cages during the crystallization process followed by thermal treatment. The M-ISAS are stabilized by skeletal oxygens of Y zeolite, and the crystallinity, porosity, and large surface area are well inherited in M-ISAS@Y. As a demonstration, acidic Pt-ISAS@Y is used for n-hexane isomerization involving consecutive catalytic dehydrogenation/hydrogenation on Pt-ISAS and isomerization on Brønsted acid sites. The turnover frequency value of Pt-ISAS reaches 727 h-1, 5 times more than Pt nanoparticles (∼3.5 nm), with a total isomer selectivity of more than 98%. This strategy provides a convenient route to fabricate promising zeolite-based M-ISAS catalysts for industrial applications.
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254
Total citations:
254
Citations from 2024:
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(31.89%)
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Liu Y. W. et al. A General Strategy for Fabricating Isolated Single Metal Atomic Site Catalysts in Y Zeolite // Journal of the American Chemical Society. 2019. Vol. 141. No. 23. pp. 9305-9311.
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Liu Y. W., Li Z., Yu Q., Chen Y., Chai Z., Zhao G., Liu S., Cheong W. C., Pan Y., Zhang Q., Gu L., Zheng L., Wang Yu., Lu Y., Wang D., Chen C., Peng Q., Liu Y., Liu L., Chen J. S., Li Y. A General Strategy for Fabricating Isolated Single Metal Atomic Site Catalysts in Y Zeolite // Journal of the American Chemical Society. 2019. Vol. 141. No. 23. pp. 9305-9311.
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TY - JOUR
DO - 10.1021/jacs.9b02936
UR - https://doi.org/10.1021/jacs.9b02936
TI - A General Strategy for Fabricating Isolated Single Metal Atomic Site Catalysts in Y Zeolite
T2 - Journal of the American Chemical Society
AU - Liu, Yi Wei
AU - Li, Zhi
AU - Yu, Qiuying
AU - Chen, Yanfei
AU - Chai, Ziwei
AU - Zhao, Guofeng
AU - Liu, Shoujie
AU - Cheong, Weng Chon
AU - Pan, Yuan
AU - Zhang, Qinghua
AU - Gu, Lin
AU - Zheng, Li-Rong
AU - Wang, Yu
AU - Lu, Yong
AU - Wang, Dingsheng
AU - Chen, C.
AU - Peng, Qing
AU - Liu, Yunqi
AU - Liu, Li-Min
AU - Chen, Jie Sheng
AU - Li, Yadong
PY - 2019
DA - 2019/05/22
PB - American Chemical Society (ACS)
SP - 9305-9311
IS - 23
VL - 141
PMID - 31117651
SN - 0002-7863
SN - 1520-5126
ER -
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BibTex (up to 50 authors)
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@article{2019_Liu,
author = {Yi Wei Liu and Zhi Li and Qiuying Yu and Yanfei Chen and Ziwei Chai and Guofeng Zhao and Shoujie Liu and Weng Chon Cheong and Yuan Pan and Qinghua Zhang and Lin Gu and Li-Rong Zheng and Yu Wang and Yong Lu and Dingsheng Wang and C. Chen and Qing Peng and Yunqi Liu and Li-Min Liu and Jie Sheng Chen and Yadong Li},
title = {A General Strategy for Fabricating Isolated Single Metal Atomic Site Catalysts in Y Zeolite},
journal = {Journal of the American Chemical Society},
year = {2019},
volume = {141},
publisher = {American Chemical Society (ACS)},
month = {may},
url = {https://doi.org/10.1021/jacs.9b02936},
number = {23},
pages = {9305--9311},
doi = {10.1021/jacs.9b02936}
}
Cite this
MLA
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Liu, Yi Wei, et al. “A General Strategy for Fabricating Isolated Single Metal Atomic Site Catalysts in Y Zeolite.” Journal of the American Chemical Society, vol. 141, no. 23, May. 2019, pp. 9305-9311. https://doi.org/10.1021/jacs.9b02936.