C60-Adsorbed Single-Walled Carbon Nanotubes as Metal-Free, pH-Universal, and Multifunctional Catalysts for Oxygen Reduction, Oxygen Evolution, and Hydrogen Evolution
Тип публикации: Journal Article
Дата публикации: 2019-06-26
SCImago Q1
Tоп 10% SCImago
WOS Q1
БС1
SJR: 5.491
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
31241328
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Краткое описание
Buckminsterfullerene (C60) was adsorbed onto single-walled carbon nanotubes (SWCNTs) as an electron-acceptor to induce intermolecular charge-transfer with the SWCNTs, leading to a class of new metal-free C60-SWCNT electrocatalysts. For the first time, these newly developed C60-SWCNTs were demonstrated to act as trifunctional metal-free catalysts for oxygen reduction reaction (ORR), oxygen evolution reaction (OER), and hydrogen evolution reaction (HER) over a wide range of pH values, from acid to alkaline, with even higher electrocatalytic activities and better long-term stabilities than those of commercial Pt and RuO2 counterparts. Thus, the adsorption-induced intermolecular charge-transfer with the C60 electron-acceptor can provide a general approach to high-performance, metal-free, pH-universal carbon-based trifunctional metal-free electrocatalysts for water-splitting and beyond.
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Gao R. et al. C60-Adsorbed Single-Walled Carbon Nanotubes as Metal-Free, pH-Universal, and Multifunctional Catalysts for Oxygen Reduction, Oxygen Evolution, and Hydrogen Evolution // Journal of the American Chemical Society. 2019. Vol. 141. No. 29. pp. 11658-11666.
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Gao R., Dai Q., Du F., Yan D., Dai L. C60-Adsorbed Single-Walled Carbon Nanotubes as Metal-Free, pH-Universal, and Multifunctional Catalysts for Oxygen Reduction, Oxygen Evolution, and Hydrogen Evolution // Journal of the American Chemical Society. 2019. Vol. 141. No. 29. pp. 11658-11666.
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TY - JOUR
DO - 10.1021/jacs.9b05006
UR - https://doi.org/10.1021/jacs.9b05006
TI - C60-Adsorbed Single-Walled Carbon Nanotubes as Metal-Free, pH-Universal, and Multifunctional Catalysts for Oxygen Reduction, Oxygen Evolution, and Hydrogen Evolution
T2 - Journal of the American Chemical Society
AU - Gao, Rui
AU - Dai, Quanbin
AU - Du, Feng
AU - Yan, Dongpeng
AU - Dai, Liming
PY - 2019
DA - 2019/06/26
PB - American Chemical Society (ACS)
SP - 11658-11666
IS - 29
VL - 141
PMID - 31241328
SN - 0002-7863
SN - 1520-5126
ER -
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@article{2019_Gao,
author = {Rui Gao and Quanbin Dai and Feng Du and Dongpeng Yan and Liming Dai},
title = {C60-Adsorbed Single-Walled Carbon Nanotubes as Metal-Free, pH-Universal, and Multifunctional Catalysts for Oxygen Reduction, Oxygen Evolution, and Hydrogen Evolution},
journal = {Journal of the American Chemical Society},
year = {2019},
volume = {141},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/jacs.9b05006},
number = {29},
pages = {11658--11666},
doi = {10.1021/jacs.9b05006}
}
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Gao, Rui, et al. “C60-Adsorbed Single-Walled Carbon Nanotubes as Metal-Free, pH-Universal, and Multifunctional Catalysts for Oxygen Reduction, Oxygen Evolution, and Hydrogen Evolution.” Journal of the American Chemical Society, vol. 141, no. 29, Jun. 2019, pp. 11658-11666. https://doi.org/10.1021/jacs.9b05006.
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