Ligand-Directed Reticular Synthesis of Catalytically Active Missing Zirconium-Based Metal–Organic Frameworks
Zhijie Chen
1
,
Penghao Li
1
,
Xingjie Wang
1
,
Ken-ichi Otake
1
,
Xuan Zhang
1
,
Lee Robison
1
,
Ahmet Atilgan
1
,
Timur Islamoglu
1
,
Morgan G Hall
2
,
J Fraser Stoddart
1, 3, 4
,
Publication type: Journal Article
Publication date: 2019-07-25
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
31343872
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
Zirconium-based metal-organic frameworks (Zr-MOFs) based on edge-transitive nets such as fcu, spn, she, csq, and ftw with diverse potential applications have been widely reported. Zr-MOFs based on the highly connected 6,12-connected alb net, however, remain absent on account of synthetic challenges. Herein we report the ligand-directed reticular syntheses and isoreticular expansion of a series of Zr-MOFs with the edge-transitive alb net from 12-connected hexagonal-prismatic Zr6 nodes and 6-connected trigonal-prismatic linkers, i.e., microporous NU-1600, mesoporous NU-1601, and mesoporous NU-1602. These Zr-MOFs exhibit remarkable activities toward the destruction of a nerve agent (soman) and a nerve agent simulant (DMNP).
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Total citations:
82
Citations from 2024:
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(35%)
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GOST
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Chen Z. et al. Ligand-Directed Reticular Synthesis of Catalytically Active Missing Zirconium-Based Metal–Organic Frameworks // Journal of the American Chemical Society. 2019. Vol. 141. No. 31. pp. 12229-12235.
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Chen Z., Li P., Wang X., Otake K., Zhang X., Robison L., Atilgan A., Islamoglu T., Hall M. G., Peterson G. W., Stoddart J. F., Farha O. K. Ligand-Directed Reticular Synthesis of Catalytically Active Missing Zirconium-Based Metal–Organic Frameworks // Journal of the American Chemical Society. 2019. Vol. 141. No. 31. pp. 12229-12235.
Cite this
RIS
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TY - JOUR
DO - 10.1021/jacs.9b06179
UR - https://doi.org/10.1021/jacs.9b06179
TI - Ligand-Directed Reticular Synthesis of Catalytically Active Missing Zirconium-Based Metal–Organic Frameworks
T2 - Journal of the American Chemical Society
AU - Chen, Zhijie
AU - Li, Penghao
AU - Wang, Xingjie
AU - Otake, Ken-ichi
AU - Zhang, Xuan
AU - Robison, Lee
AU - Atilgan, Ahmet
AU - Islamoglu, Timur
AU - Hall, Morgan G
AU - Peterson, Gregory W
AU - Stoddart, J Fraser
AU - Farha, Omar K.
PY - 2019
DA - 2019/07/25
PB - American Chemical Society (ACS)
SP - 12229-12235
IS - 31
VL - 141
PMID - 31343872
SN - 0002-7863
SN - 1520-5126
ER -
Cite this
BibTex (up to 50 authors)
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@article{2019_Chen,
author = {Zhijie Chen and Penghao Li and Xingjie Wang and Ken-ichi Otake and Xuan Zhang and Lee Robison and Ahmet Atilgan and Timur Islamoglu and Morgan G Hall and Gregory W Peterson and J Fraser Stoddart and Omar K. Farha},
title = {Ligand-Directed Reticular Synthesis of Catalytically Active Missing Zirconium-Based Metal–Organic Frameworks},
journal = {Journal of the American Chemical Society},
year = {2019},
volume = {141},
publisher = {American Chemical Society (ACS)},
month = {jul},
url = {https://doi.org/10.1021/jacs.9b06179},
number = {31},
pages = {12229--12235},
doi = {10.1021/jacs.9b06179}
}
Cite this
MLA
Copy
Chen, Zhijie, et al. “Ligand-Directed Reticular Synthesis of Catalytically Active Missing Zirconium-Based Metal–Organic Frameworks.” Journal of the American Chemical Society, vol. 141, no. 31, Jul. 2019, pp. 12229-12235. https://doi.org/10.1021/jacs.9b06179.