Synthesis and Electron-Donor Ability of the First Conjugated π-Extended Tetrathiafulvalene Dimers
Тип публикации: Journal Article
Дата публикации: 2004-06-01
scimago Q2
wos Q1
БС1
SJR: 0.737
CiteScore: 6.1
Impact factor: 3.6
ISSN: 00223263, 15206904
PubMed ID:
15202907
Organic Chemistry
Краткое описание
A series of novel conjugated homo (16a,b) and heterodimers (20) of pi-extended tetrathiafulvalenes with p-quinodimethane structures (exTTFs) linked by a conjugative vinyl spacer have been prepared by olefination Wittig-Horner reaction from the corresponding quinones (14, 19) and phosphonates (15a,b). The redox properties, determined by cyclic voltammetry, reveal a strong donor character and the presence of only one four-electron oxidation wave to form the tetracation species at oxidation potential values quite similar to those found for the related monomers. Theoretical calculations (PM3) show a planar central stilbene moiety and highly distorted exTTF units. The electronic spectra support as well as the electrochemical data and theoretical calculation the lack of significant communication between the exTTF units.
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Díaz M. C. et al. Synthesis and Electron-Donor Ability of the First Conjugated π-Extended Tetrathiafulvalene Dimers // Journal of Organic Chemistry. 2004. Vol. 69. No. 13. pp. 4492-4499.
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Díaz M. C., Illescas B. M., Seoane C., Martin N. Synthesis and Electron-Donor Ability of the First Conjugated π-Extended Tetrathiafulvalene Dimers // Journal of Organic Chemistry. 2004. Vol. 69. No. 13. pp. 4492-4499.
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TY - JOUR
DO - 10.1021/jo049741z
UR - https://doi.org/10.1021/jo049741z
TI - Synthesis and Electron-Donor Ability of the First Conjugated π-Extended Tetrathiafulvalene Dimers
T2 - Journal of Organic Chemistry
AU - Díaz, Marta C
AU - Illescas, Beatriz M.
AU - Seoane, Carlos
AU - Martin, Nazario
PY - 2004
DA - 2004/06/01
PB - American Chemical Society (ACS)
SP - 4492-4499
IS - 13
VL - 69
PMID - 15202907
SN - 0022-3263
SN - 1520-6904
ER -
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@article{2004_Díaz,
author = {Marta C Díaz and Beatriz M. Illescas and Carlos Seoane and Nazario Martin},
title = {Synthesis and Electron-Donor Ability of the First Conjugated π-Extended Tetrathiafulvalene Dimers},
journal = {Journal of Organic Chemistry},
year = {2004},
volume = {69},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/jo049741z},
number = {13},
pages = {4492--4499},
doi = {10.1021/jo049741z}
}
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MLA
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Díaz, Marta C., et al. “Synthesis and Electron-Donor Ability of the First Conjugated π-Extended Tetrathiafulvalene Dimers.” Journal of Organic Chemistry, vol. 69, no. 13, Jun. 2004, pp. 4492-4499. https://doi.org/10.1021/jo049741z.