Photoelectrochemical Properties of J Aggregates of Benzothiazole Merocyanine Dyes on a Nanostructured TiO2 Film
Тип публикации: Journal Article
Дата публикации: 2002-01-19
scimago Q1
wos Q3
БС2
SJR: 0.742
CiteScore: 5.3
Impact factor: 2.9
ISSN: 15206106, 15205207, 10895647
Materials Chemistry
Surfaces, Coatings and Films
Physical and Theoretical Chemistry
Краткое описание
We studied the photoelectrochemical properties of nanoporous TiO2 electrodes sensitized by a series of benzothiazole merocyanine dyes, 3-carboxyalkyl-5-[2-(3-alkyl-2-benzothiazolinyldene) ethylidene]-2-thioxo-4-thiazolidinone, having a different alkyl chain length. Broadening of absorption spectra and a large red shift of the absorption threshold up to 680 nm were observed by adsorbing dyes on a porous TiO2 electrode, suggesting the formation of various kinds of J aggregates of the dye on the TiO2 surface. The dye was fixed by a chelate-like linkage of the carboxylate anchoring group on the TiO2 surface, rather than by an ester linkage. The solar light-to-power conversion efficiency (ηsun) and the incident photon-to-current conversion efficiency (IPCE) increased with increasing the length of alkyl chain attached to the benzothiazole ring. The maximum ηsun value was 4.5%, which is the second highest value among organic dye systems reported so far (AM-1.5, 100 mW/cm2). The J aggregates of the dyes having lo...
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Sayama K. et al. Photoelectrochemical Properties of J Aggregates of Benzothiazole Merocyanine Dyes on a Nanostructured TiO2 Film // Journal of Physical Chemistry B. 2002. Vol. 106. No. 6. pp. 1363-1371.
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Sayama K., Tsukagoshi S., Hara K., Ohga Y., Shinpou A., Abe Y., SUGA S., Arakawa H. Photoelectrochemical Properties of J Aggregates of Benzothiazole Merocyanine Dyes on a Nanostructured TiO2 Film // Journal of Physical Chemistry B. 2002. Vol. 106. No. 6. pp. 1363-1371.
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TY - JOUR
DO - 10.1021/jp0129380
UR - https://doi.org/10.1021/jp0129380
TI - Photoelectrochemical Properties of J Aggregates of Benzothiazole Merocyanine Dyes on a Nanostructured TiO2 Film
T2 - Journal of Physical Chemistry B
AU - Sayama, Kazuhiro
AU - Tsukagoshi, Shingo
AU - Hara, Kohjiro
AU - Ohga, Yasuyo
AU - Shinpou, Akira
AU - Abe, Yoshimoto
AU - SUGA, Sadaharu
AU - Arakawa, Hironori
PY - 2002
DA - 2002/01/19
PB - American Chemical Society (ACS)
SP - 1363-1371
IS - 6
VL - 106
SN - 1520-6106
SN - 1520-5207
SN - 1089-5647
ER -
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@article{2002_Sayama,
author = {Kazuhiro Sayama and Shingo Tsukagoshi and Kohjiro Hara and Yasuyo Ohga and Akira Shinpou and Yoshimoto Abe and Sadaharu SUGA and Hironori Arakawa},
title = {Photoelectrochemical Properties of J Aggregates of Benzothiazole Merocyanine Dyes on a Nanostructured TiO2 Film},
journal = {Journal of Physical Chemistry B},
year = {2002},
volume = {106},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/jp0129380},
number = {6},
pages = {1363--1371},
doi = {10.1021/jp0129380}
}
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MLA
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Sayama, Kazuhiro, et al. “Photoelectrochemical Properties of J Aggregates of Benzothiazole Merocyanine Dyes on a Nanostructured TiO2 Film.” Journal of Physical Chemistry B, vol. 106, no. 6, Jan. 2002, pp. 1363-1371. https://doi.org/10.1021/jp0129380.