Journal of Physical Chemistry C, volume 111, issue 37, pages 13777-13785

Energetics of Photoinduced Electron-Transfer Reactions Decided by Quantum Confinement

Gregory D. Scholes ¹

Marcus Jones ¹

Sandeep Kumar ¹

Hide authors affiliations Show authors affiliations: 1 affiliation

Department of Chemistry, 80 Saint George Street, Institute for Optical Sciences, and Centre for Quantum Information and Quantum Control, University of Toronto, Toronto, Ontario M5S 3H6 Canada |

Publication type: Journal Article

Publication date: 2007-08-24

American Chemical Society (ACS)

Journal: Journal of Physical Chemistry C

Quartile SCImago

Quartile WOS

Impact factor: 3.7

ISSN: 19327447, 19327455

DOI: 10.1021/jp0754583

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Surfaces, Coatings and Films

Electronic, Optical and Magnetic Materials

Physical and Theoretical Chemistry

General Energy

Abstract

The photophysics of linear CdSe−CdTe nanorod heterostructures are reported. Charge-transfer emission and absorption bands are identified. Analysis of these bands reveals the factors governing photoinduced electron transfer from CdTe to CdSe, and it is thereby shown how quantum confinement effects decide the thermodynamic parameters of the Marcus−Hush theory. An important finding is the very small reorganization energy associated with the nuclear degrees of freedom (∼20 meV in toluene), which seems to be a characteristic of these nanoscale donor−acceptor systems and differentiates them from most analogous molecular systems. Therefore Marcus “inverted region” behavior is found to be typical for these systems. By analyzing the mixing between the CdTe exciton and the charge-transfer states for one sample, we find the electronic coupling matrix element that promotes the charge separation to be ∼50 meV.

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Journal of Physical Chemistry C	Journal of Physical Chemistry C, 12, 18.75% Journal of Physical Chemistry C 12 publications, 18.75%
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Nano Letters	Nano Letters, 5, 7.81% Nano Letters 5 publications, 7.81%
Journal of the American Chemical Society	Journal of the American Chemical Society, 4, 6.25% Journal of the American Chemical Society 4 publications, 6.25%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 4, 6.25% Journal of Physical Chemistry Letters 4 publications, 6.25%
Chemistry of Materials	Chemistry of Materials, 3, 4.69% Chemistry of Materials 3 publications, 4.69%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 2, 3.13% Journal of Materials Chemistry A 2 publications, 3.13%
Nature Communications	Nature Communications, 2, 3.13% Nature Communications 2 publications, 3.13%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 2, 3.13% Journal of Alloys and Compounds 2 publications, 3.13%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 2, 3.13% Physical Chemistry Chemical Physics 2 publications, 3.13%
Results in Physics	Results in Physics, 1, 1.56% Results in Physics 1 publication, 1.56%
Journal of Materials Research	Journal of Materials Research, 1, 1.56% Journal of Materials Research 1 publication, 1.56%
Inorganic Materials	Inorganic Materials, 1, 1.56% Inorganic Materials 1 publication, 1.56%
Journal of Chemical Physics	Journal of Chemical Physics, 1, 1.56% Journal of Chemical Physics 1 publication, 1.56%
Physical Review Letters	Physical Review Letters, 1, 1.56% Physical Review Letters 1 publication, 1.56%
Modern Physics Letters B	Modern Physics Letters B, 1, 1.56% Modern Physics Letters B 1 publication, 1.56%
Science China Information Sciences	Science China Information Sciences, 1, 1.56% Science China Information Sciences 1 publication, 1.56%
Physica E: Low-Dimensional Systems and Nanostructures	Physica E: Low-Dimensional Systems and Nanostructures, 1, 1.56% Physica E: Low-Dimensional Systems and Nanostructures 1 publication, 1.56%
Journal of Luminescence	Journal of Luminescence, 1, 1.56% Journal of Luminescence 1 publication, 1.56%
Solar Energy Materials and Solar Cells	Solar Energy Materials and Solar Cells, 1, 1.56% Solar Energy Materials and Solar Cells 1 publication, 1.56%
Biochimica et Biophysica Acta - Bioenergetics	Biochimica et Biophysica Acta - Bioenergetics, 1, 1.56% Biochimica et Biophysica Acta - Bioenergetics 1 publication, 1.56%
Coordination Chemistry Reviews	Coordination Chemistry Reviews, 1, 1.56% Coordination Chemistry Reviews 1 publication, 1.56%
ChemSusChem	ChemSusChem, 1, 1.56% ChemSusChem 1 publication, 1.56%
Advanced Functional Materials	Advanced Functional Materials, 1, 1.56% Advanced Functional Materials 1 publication, 1.56%
Small	Small, 1, 1.56% Small 1 publication, 1.56%
ACS Omega	ACS Omega, 1, 1.56% ACS Omega 1 publication, 1.56%
Advanced Materials	Advanced Materials, 1, 1.56% Advanced Materials 1 publication, 1.56%
Science advances	Science advances, 1, 1.56% Science advances 1 publication, 1.56%
Proceedings of the National Academy of Sciences of the United States of America	Proceedings of the National Academy of Sciences of the United States of America, 1, 1.56% Proceedings of the National Academy of Sciences of the United States of America 1 publication, 1.56%
	2 4 6 8 10 12

Citations by publishers

	5 10 15 20 25 30 35
American Chemical Society (ACS)	American Chemical Society (ACS), 35, 54.69% American Chemical Society (ACS) 35 publications, 54.69%
Elsevier	Elsevier, 8, 12.5% Elsevier 8 publications, 12.5%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 4, 6.25% Royal Society of Chemistry (RSC) 4 publications, 6.25%
Wiley	Wiley, 4, 6.25% Wiley 4 publications, 6.25%
Springer Nature	Springer Nature, 2, 3.13% Springer Nature 2 publications, 3.13%
Cambridge University Press	Cambridge University Press, 1, 1.56% Cambridge University Press 1 publication, 1.56%
Pleiades Publishing	Pleiades Publishing, 1, 1.56% Pleiades Publishing 1 publication, 1.56%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 1, 1.56% American Institute of Physics (AIP) 1 publication, 1.56%
American Physical Society (APS)	American Physical Society (APS), 1, 1.56% American Physical Society (APS) 1 publication, 1.56%
World Scientific	World Scientific, 1, 1.56% World Scientific 1 publication, 1.56%
Science in China Press	Science in China Press, 1, 1.56% Science in China Press 1 publication, 1.56%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 1.56% American Association for the Advancement of Science (AAAS) 1 publication, 1.56%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 1, 1.56% Proceedings of the National Academy of Sciences (PNAS) 1 publication, 1.56%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.56% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.56%
	5 10 15 20 25 30 35

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Scholes G. D., Jones M., Kumar S. Energetics of Photoinduced Electron-Transfer Reactions Decided by Quantum Confinement // Journal of Physical Chemistry C. 2007. Vol. 111. No. 37. pp. 13777-13785.

GOST all authors (up to 50) Copy

Scholes G. D., Jones M., Kumar S. Energetics of Photoinduced Electron-Transfer Reactions Decided by Quantum Confinement // Journal of Physical Chemistry C. 2007. Vol. 111. No. 37. pp. 13777-13785.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1021/jp0754583

UR - https://doi.org/10.1021/jp0754583

TI - Energetics of Photoinduced Electron-Transfer Reactions Decided by Quantum Confinement

T2 - Journal of Physical Chemistry C

AU - Kumar, Sandeep

AU - Scholes, Gregory D.

AU - Jones, Marcus

PY - 2007

DA - 2007/08/24 00:00:00

PB - American Chemical Society (ACS)

SP - 13777-13785

IS - 37

VL - 111

SN - 1932-7447

SN - 1932-7455

ER -

BibTex |

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BibTex Copy

@article{2007_Scholes,

author = {Sandeep Kumar and Gregory D. Scholes and Marcus Jones},

title = {Energetics of Photoinduced Electron-Transfer Reactions Decided by Quantum Confinement},

journal = {Journal of Physical Chemistry C},

year = {2007},

volume = {111},

publisher = {American Chemical Society (ACS)},

month = {aug},

url = {https://doi.org/10.1021/jp0754583},

number = {37},

pages = {13777--13785},

doi = {10.1021/jp0754583}

}

MLA

Cite this

MLA Copy

Scholes, Gregory D., et al. “Energetics of Photoinduced Electron-Transfer Reactions Decided by Quantum Confinement.” Journal of Physical Chemistry C, vol. 111, no. 37, Aug. 2007, pp. 13777-13785. https://doi.org/10.1021/jp0754583.

Found error?

Publisher

American Chemical Society (ACS)

Journal

Journal of Physical Chemistry C

Quartile SCImago

Quartile WOS

Impact factor

3.7

ISSN

19327447 (Print)
19327455 (Electronic)