Methane Activation on In-Modified ZSM-5: The State of Indium in the Zeolite and Pathways of Methane Transformation to Surface Species
Тип публикации: Journal Article
Дата публикации: 2014-04-04
SCImago Q1
WOS Q3
БС1
SJR: 0.82
CiteScore: 6.2
Impact factor: 3.2
ISSN: 19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Краткое описание
Methane activation pathways as well as methane involvement in the reaction of ethylene aromatization on In-modified H-ZSM-5 zeolite (In/H-ZSM-5) have been studied with solid-state NMR spectroscopy. The state of indium in In/H-ZSM-5 in dependence of the zeolite activation procedure, reductive or oxidative, has been analyzed with X-ray photoelectron spectroscopy (XPS). On the basis of 1H MAS NMR analysis of the evolution of the quantity of Bronsted acid sites (BAS) and XPS analysis of the state of indium in dependence of zeolite activation procedure, it has been inferred that indium exists in the form of either In+ or InO+ isolated cationic species in the zeolite. Methane interaction with different indium cationic species has been analyzed with 13C MAS NMR spectroscopy. In+ species has been concluded to be inactive, whereas InO+ species provides dissociative adsorption of methane to afford primarily the oxyindium–methyl species. The secondary products of oxyindium–methyl species transformation are oxyindium...
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Gabrienko A. A. et al. Methane Activation on In-Modified ZSM-5: The State of Indium in the Zeolite and Pathways of Methane Transformation to Surface Species // Journal of Physical Chemistry C. 2014. Vol. 118. No. 15. pp. 8034-8043.
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Gabrienko A. A., ARZUMANOV S., Moroz I. B., Prosvirin I. P., Toktarev A., Wang W., Stepanov A. Methane Activation on In-Modified ZSM-5: The State of Indium in the Zeolite and Pathways of Methane Transformation to Surface Species // Journal of Physical Chemistry C. 2014. Vol. 118. No. 15. pp. 8034-8043.
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TY - JOUR
DO - 10.1021/jp501314j
UR - https://doi.org/10.1021/jp501314j
TI - Methane Activation on In-Modified ZSM-5: The State of Indium in the Zeolite and Pathways of Methane Transformation to Surface Species
T2 - Journal of Physical Chemistry C
AU - Gabrienko, A A
AU - ARZUMANOV, S
AU - Moroz, Ilya B
AU - Prosvirin, Igor P.
AU - Toktarev, A.
AU - Wang, Wei
AU - Stepanov, Alexander
PY - 2014
DA - 2014/04/04
PB - American Chemical Society (ACS)
SP - 8034-8043
IS - 15
VL - 118
SN - 1932-7447
SN - 1932-7455
ER -
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@article{2014_Gabrienko,
author = {A A Gabrienko and S ARZUMANOV and Ilya B Moroz and Igor P. Prosvirin and A. Toktarev and Wei Wang and Alexander Stepanov},
title = {Methane Activation on In-Modified ZSM-5: The State of Indium in the Zeolite and Pathways of Methane Transformation to Surface Species},
journal = {Journal of Physical Chemistry C},
year = {2014},
volume = {118},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/jp501314j},
number = {15},
pages = {8034--8043},
doi = {10.1021/jp501314j}
}
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Gabrienko, A. A., et al. “Methane Activation on In-Modified ZSM-5: The State of Indium in the Zeolite and Pathways of Methane Transformation to Surface Species.” Journal of Physical Chemistry C, vol. 118, no. 15, Apr. 2014, pp. 8034-8043. https://doi.org/10.1021/jp501314j.
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