Direct Synthesis of Well-Defined Alcohol-Functionalized Polymers via Acyclic Diene Metathesis (ADMET) Polymerization
Publication type: Journal Article
Publication date: 1998-04-17
scimago Q1
wos Q1
SJR: 1.352
CiteScore: 9.0
Impact factor: 5.2
ISSN: 00249297, 15205835
Materials Chemistry
Organic Chemistry
Inorganic Chemistry
Polymers and Plastics
Abstract
Because of its robust nature, Grubbs' ruthenium benzylidene catalyst RuCl2(CHPh)(PCy3)2 promotes the successful acyclic diene metathesis (ADMET) bulk polymerization of alcohol-functionalized dienes, thus providing a method for the direct synthesis of linear polymers containing hydroxy groups. Primary, secondary, and tertiary alcohol functional groups can be placed at precise intervals along an unsaturated hydrocarbon backbone. Exhaustive hydrogenation of the secondary alcohol homologue produces a well-defined ethylenevinyl alcohol copolymer. Only the unsaturated and saturated secondary alcohol polymers crystallize, a phenomenon likely attributed to the enhanced packing propensity of these macromolecules in comparison with those of their primary and tertiary analogues.
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Total citations:
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Citations from 2024:
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GOST
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Valenti D. J., Wagener K. B. Direct Synthesis of Well-Defined Alcohol-Functionalized Polymers via Acyclic Diene Metathesis (ADMET) Polymerization // Macromolecules. 1998. Vol. 31. No. 9. pp. 2764-2773.
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Valenti D. J., Wagener K. B. Direct Synthesis of Well-Defined Alcohol-Functionalized Polymers via Acyclic Diene Metathesis (ADMET) Polymerization // Macromolecules. 1998. Vol. 31. No. 9. pp. 2764-2773.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/ma9714833
UR - https://doi.org/10.1021/ma9714833
TI - Direct Synthesis of Well-Defined Alcohol-Functionalized Polymers via Acyclic Diene Metathesis (ADMET) Polymerization
T2 - Macromolecules
AU - Valenti, Dominick J
AU - Wagener, Kenneth B.
PY - 1998
DA - 1998/04/17
PB - American Chemical Society (ACS)
SP - 2764-2773
IS - 9
VL - 31
SN - 0024-9297
SN - 1520-5835
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{1998_Valenti,
author = {Dominick J Valenti and Kenneth B. Wagener},
title = {Direct Synthesis of Well-Defined Alcohol-Functionalized Polymers via Acyclic Diene Metathesis (ADMET) Polymerization},
journal = {Macromolecules},
year = {1998},
volume = {31},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/ma9714833},
number = {9},
pages = {2764--2773},
doi = {10.1021/ma9714833}
}
Cite this
MLA
Copy
Valenti, Dominick J., and Kenneth B. Wagener. “Direct Synthesis of Well-Defined Alcohol-Functionalized Polymers via Acyclic Diene Metathesis (ADMET) Polymerization.” Macromolecules, vol. 31, no. 9, Apr. 1998, pp. 2764-2773. https://doi.org/10.1021/ma9714833.