Nano Letters, volume 11, issue 3, pages 1136-1140

Biexciton quantum yield of single semiconductor nanocrystals from photon statistics.

Gautham Nair ¹

Jiyong Zhao ¹

Moungi G. Bawendi ¹

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Department of Chemistry, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge, Massachusetts 02139, United States |

Publication type: Journal Article

Publication date: 2011-02-02

American Chemical Society (ACS)

Journal: Nano Letters

Quartile SCImago

Quartile WOS

Impact factor: 10.8

ISSN: 15306984, 15306992

DOI: 10.1021/nl104054t

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PubMed ID: 21288042

General Chemistry

Condensed Matter Physics

General Materials Science

Mechanical Engineering

Bioengineering

Abstract

Biexciton properties strongly affect the usability of a light emitter in quantum photon sources and lasers but are difficult to measure for single fluorophores at room temperature due to luminescence intermittency and bleaching at the high excitation fluences usually required. Here, we observe the biexciton (BX) to exciton (X) to ground photoluminescence cascade of single colloidal semiconductor nanocrystals (NCs) under weak excitation in a g((2)) photon correlation measurement and show that the normalized amplitude of the cascade feature is equal to the ratio of the BX to X fluorescence quantum yields. This imposes a limit on the attainable depth of photon antibunching and provides a robust means to study single emitter biexciton physics. In NC samples, we show that the BX quantum yield is considerably inhomogeneous, consistent with the defect sensitivity expected of the Auger nonradiative recombination mechanism. The method can be extended to study X,BX spectral and polarization correlations.

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ACS Nano	ACS Nano, 12, 5.36% ACS Nano 12 publications, 5.36%
Physical Review B	Physical Review B, 10, 4.46% Physical Review B 10 publications, 4.46%
ACS Photonics	ACS Photonics, 9, 4.02% ACS Photonics 9 publications, 4.02%
Nature Communications	Nature Communications, 8, 3.57% Nature Communications 8 publications, 3.57%
Journal of Chemical Physics	Journal of Chemical Physics, 7, 3.13% Journal of Chemical Physics 7 publications, 3.13%
Chemical Reviews	Chemical Reviews, 5, 2.23% Chemical Reviews 5 publications, 2.23%
Journal of the American Chemical Society	Journal of the American Chemical Society, 5, 2.23% Journal of the American Chemical Society 5 publications, 2.23%
Nature Materials	Nature Materials, 4, 1.79% Nature Materials 4 publications, 1.79%
Small	Small, 4, 1.79% Small 4 publications, 1.79%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 4, 1.79% Physical Chemistry Chemical Physics 4 publications, 1.79%
Physical Review Letters	Physical Review Letters, 3, 1.34% Physical Review Letters 3 publications, 1.34%
Nature Nanotechnology	Nature Nanotechnology, 3, 1.34% Nature Nanotechnology 3 publications, 1.34%
Scientific Reports	Scientific Reports, 3, 1.34% Scientific Reports 3 publications, 1.34%
Advanced Optical Materials	Advanced Optical Materials, 3, 1.34% Advanced Optical Materials 3 publications, 1.34%
Applied Physics Letters	Applied Physics Letters, 2, 0.89% Applied Physics Letters 2 publications, 0.89%
Light: Science and Applications	Light: Science and Applications, 2, 0.89% Light: Science and Applications 2 publications, 0.89%
Advanced Materials	Advanced Materials, 2, 0.89% Advanced Materials 2 publications, 0.89%
ACS Applied Nano Materials	ACS Applied Nano Materials, 2, 0.89% ACS Applied Nano Materials 2 publications, 0.89%
Chemical Society Reviews	Chemical Society Reviews, 2, 0.89% Chemical Society Reviews 2 publications, 0.89%
Proceedings of SPIE - The International Society for Optical Engineering	Proceedings of SPIE - The International Society for Optical Engineering, 2, 0.89% Proceedings of SPIE - The International Society for Optical Engineering 2 publications, 0.89%
Optics Express	Optics Express, 2, 0.89% Optics Express 2 publications, 0.89%
Photonics Research	Photonics Research, 2, 0.89% Photonics Research 2 publications, 0.89%
Optics Letters	Optics Letters, 2, 0.89% Optics Letters 2 publications, 0.89%
APL Materials	APL Materials, 1, 0.45% APL Materials 1 publication, 0.45%
Review of Scientific Instruments	Review of Scientific Instruments, 1, 0.45% Review of Scientific Instruments 1 publication, 0.45%
	5 10 15 20 25 30 35

Citations by publishers

	20 40 60 80 100 120
American Chemical Society (ACS)	American Chemical Society (ACS), 107, 47.77% American Chemical Society (ACS) 107 publications, 47.77%
Springer Nature	Springer Nature, 26, 11.61% Springer Nature 26 publications, 11.61%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 20, 8.93% Royal Society of Chemistry (RSC) 20 publications, 8.93%
American Physical Society (APS)	American Physical Society (APS), 17, 7.59% American Physical Society (APS) 17 publications, 7.59%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 12, 5.36% American Institute of Physics (AIP) 12 publications, 5.36%
Wiley	Wiley, 11, 4.91% Wiley 11 publications, 4.91%
IOP Publishing	IOP Publishing, 6, 2.68% IOP Publishing 6 publications, 2.68%
Optical Society of America	Optical Society of America, 6, 2.68% Optical Society of America 6 publications, 2.68%
Elsevier	Elsevier, 5, 2.23% Elsevier 5 publications, 2.23%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 3, 1.34% Multidisciplinary Digital Publishing Institute (MDPI) 3 publications, 1.34%
SPIE	SPIE, 2, 0.89% SPIE 2 publications, 0.89%
Materials Research Society	Materials Research Society, 1, 0.45% Materials Research Society 1 publication, 0.45%
Cambridge University Press	Cambridge University Press, 1, 0.45% Cambridge University Press 1 publication, 0.45%
Pleiades Publishing	Pleiades Publishing, 1, 0.45% Pleiades Publishing 1 publication, 0.45%
Walter de Gruyter	Walter de Gruyter, 1, 0.45% Walter de Gruyter 1 publication, 0.45%
Chinese Physical Society	Chinese Physical Society, 1, 0.45% Chinese Physical Society 1 publication, 0.45%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 1, 0.45% Proceedings of the National Academy of Sciences (PNAS) 1 publication, 0.45%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.45% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.45%
Research Square Platform LLC	Research Square Platform LLC, 1, 0.45% Research Square Platform LLC 1 publication, 0.45%
	20 40 60 80 100 120

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Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

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Nair G., Zhao J., Bawendi M. G. Biexciton quantum yield of single semiconductor nanocrystals from photon statistics. // Nano Letters. 2011. Vol. 11. No. 3. pp. 1136-1140.

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Nair G., Zhao J., Bawendi M. G. Biexciton quantum yield of single semiconductor nanocrystals from photon statistics. // Nano Letters. 2011. Vol. 11. No. 3. pp. 1136-1140.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/nl104054t

UR - https://doi.org/10.1021/nl104054t

TI - Biexciton quantum yield of single semiconductor nanocrystals from photon statistics.

T2 - Nano Letters

AU - Nair, Gautham

AU - Zhao, Jiyong

AU - Bawendi, Moungi G.

PY - 2011

DA - 2011/02/02 00:00:00

PB - American Chemical Society (ACS)

SP - 1136-1140

IS - 3

VL - 11

PMID - 21288042

SN - 1530-6984

SN - 1530-6992

ER -

BibTex |

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BibTex Copy

@article{2011_Nair,

author = {Gautham Nair and Jiyong Zhao and Moungi G. Bawendi},

title = {Biexciton quantum yield of single semiconductor nanocrystals from photon statistics.},

journal = {Nano Letters},

year = {2011},

volume = {11},

publisher = {American Chemical Society (ACS)},

month = {feb},

url = {https://doi.org/10.1021/nl104054t},

number = {3},

pages = {1136--1140},

doi = {10.1021/nl104054t}

}

MLA

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MLA Copy

Nair, Gautham, et al. “Biexciton quantum yield of single semiconductor nanocrystals from photon statistics..” Nano Letters, vol. 11, no. 3, Feb. 2011, pp. 1136-1140. https://doi.org/10.1021/nl104054t.

Found error?

Publisher

American Chemical Society (ACS)

Journal

Nano Letters

Quartile SCImago

Quartile WOS

Impact factor

10.8

ISSN

15306984 (Print)
15306992 (Electronic)