ACS Nano, volume 5, issue 1, pages 183-190

Tuning the Synthesis of Ternary Lead Chalcogenide Quantum Dots by Balancing Precursor Reactivity

Danielle K. Smith ¹

Joseph M. Luther ¹

Octavi E Semonin ^{1, 2}

Arthur J. Nozik ^{1, 3}

Matthew C Beard ¹

Hide authors affiliations Show authors affiliations: 3 affiliations

Center for Advanced Solar Photophysics, Chemical and Materials Sciences, National Renewable Energy Laboratory, Golden, Colorado 80401, United States |

Department of Physics

Department of Chemistry and Biochemistry

Publication type: Journal Article

Publication date: 2010-12-08

American Chemical Society (ACS)

Journal: ACS Nano

Quartile SCImago

Quartile WOS

Impact factor: 17.1

ISSN: 19360851, 1936086X

DOI: 10.1021/nn102878u

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General Physics and Astronomy

General Materials Science

General Engineering

Abstract

We report the synthesis and characterization of composition-tunable ternary lead chalcogenide alloys PbSe(x)Te(1-x), PbS(x)Te(1-x), and PbS(x)Se(1-x). This work explores the relative reaction rates of chalcogenide precursors to produce alloyed quantum dots (QDs), and we find the highly reactive bis(trimethylsilyl) (TMS(2))-based precursors allow for the homogeneous incorporation of anions. By varying the Pb to oleic acid ratio, we demonstrate size control of similar composition alloys. We find the resulting QDs are Pb-rich but the Pb/anion ratio is size- and composition-dependent in all alloyed QD as well as in PbSe, PbTe, and PbS QDs and is consistent with the reaction rates of the anion precursors. A more reactive anion precursor results in a lower Pb/anion ratio.

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Citations by journals

	2 4 6 8 10 12 14 16 18
Chemistry of Materials	Chemistry of Materials, 17, 13.49% Chemistry of Materials 17 publications, 13.49%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 8, 6.35% Journal of Physical Chemistry C 8 publications, 6.35%
ACS Nano	ACS Nano, 8, 6.35% ACS Nano 8 publications, 6.35%
Journal of the American Chemical Society	Journal of the American Chemical Society, 5, 3.97% Journal of the American Chemical Society 5 publications, 3.97%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 5, 3.97% Journal of Materials Chemistry A 5 publications, 3.97%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 4, 3.17% Journal of Physical Chemistry Letters 4 publications, 3.17%
CrystEngComm	CrystEngComm, 4, 3.17% CrystEngComm 4 publications, 3.17%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 4, 3.17% Physical Chemistry Chemical Physics 4 publications, 3.17%
Nano Letters	Nano Letters, 3, 2.38% Nano Letters 3 publications, 2.38%
Chemical Reviews	Chemical Reviews, 3, 2.38% Chemical Reviews 3 publications, 2.38%
Nanoscale	Nanoscale, 3, 2.38% Nanoscale 3 publications, 2.38%
RSC Advances	RSC Advances, 3, 2.38% RSC Advances 3 publications, 2.38%
Inorganics	Inorganics, 2, 1.59% Inorganics 2 publications, 1.59%
Nanotechnology	Nanotechnology, 2, 1.59% Nanotechnology 2 publications, 1.59%
Russian Chemical Reviews	Russian Chemical Reviews, 2, 1.59% Russian Chemical Reviews 2 publications, 1.59%
Solar Energy	Solar Energy, 2, 1.59% Solar Energy 2 publications, 1.59%
Advanced Energy Materials	Advanced Energy Materials, 2, 1.59% Advanced Energy Materials 2 publications, 1.59%
Angewandte Chemie	Angewandte Chemie, 2, 1.59% Angewandte Chemie 2 publications, 1.59%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 2, 1.59% Angewandte Chemie - International Edition 2 publications, 1.59%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 2, 1.59% Journal of Materials Chemistry C 2 publications, 1.59%
Journal of Materials Science: Materials in Electronics	Journal of Materials Science: Materials in Electronics, 1, 0.79% Journal of Materials Science: Materials in Electronics 1 publication, 0.79%
Physical Review B	Physical Review B, 1, 0.79% Physical Review B 1 publication, 0.79%
Recent Innovations in Chemical Engineering	Recent Innovations in Chemical Engineering, 1, 0.79% Recent Innovations in Chemical Engineering 1 publication, 0.79%
Chemistry Letters	Chemistry Letters, 1, 0.79% Chemistry Letters 1 publication, 0.79%
EPJ Applied Physics	EPJ Applied Physics, 1, 0.79% EPJ Applied Physics 1 publication, 0.79%
Materials	Materials, 1, 0.79% Materials 1 publication, 0.79%
Science China Technological Sciences	Science China Technological Sciences, 1, 0.79% Science China Technological Sciences 1 publication, 0.79%
Silicon	Silicon, 1, 0.79% Silicon 1 publication, 0.79%
Journal of Inorganic and Organometallic Polymers and Materials	Journal of Inorganic and Organometallic Polymers and Materials, 1, 0.79% Journal of Inorganic and Organometallic Polymers and Materials 1 publication, 0.79%
	2 4 6 8 10 12 14 16 18

Citations by publishers

	10 20 30 40 50 60
American Chemical Society (ACS)	American Chemical Society (ACS), 51, 40.48% American Chemical Society (ACS) 51 publications, 40.48%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 28, 22.22% Royal Society of Chemistry (RSC) 28 publications, 22.22%
Wiley	Wiley, 13, 10.32% Wiley 13 publications, 10.32%
Elsevier	Elsevier, 10, 7.94% Elsevier 10 publications, 7.94%
Springer Nature	Springer Nature, 5, 3.97% Springer Nature 5 publications, 3.97%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 3, 2.38% Multidisciplinary Digital Publishing Institute (MDPI) 3 publications, 2.38%
IOP Publishing	IOP Publishing, 3, 2.38% IOP Publishing 3 publications, 2.38%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 2, 1.59% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 2 publications, 1.59%
American Physical Society (APS)	American Physical Society (APS), 1, 0.79% American Physical Society (APS) 1 publication, 0.79%
Bentham Science	Bentham Science, 1, 0.79% Bentham Science 1 publication, 0.79%
The Chemical Society of Japan	The Chemical Society of Japan, 1, 0.79% The Chemical Society of Japan 1 publication, 0.79%
EDP Sciences	EDP Sciences, 1, 0.79% EDP Sciences 1 publication, 0.79%
Taylor & Francis	Taylor & Francis, 1, 0.79% Taylor & Francis 1 publication, 0.79%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 1, 0.79% Korean Society of Industrial Engineering Chemistry 1 publication, 0.79%
Pleiades Publishing	Pleiades Publishing, 1, 0.79% Pleiades Publishing 1 publication, 0.79%
Walter de Gruyter	Walter de Gruyter, 1, 0.79% Walter de Gruyter 1 publication, 0.79%
Optical Society of America	Optical Society of America, 1, 0.79% Optical Society of America 1 publication, 0.79%
	10 20 30 40 50 60

We do not take into account publications without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

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Smith D. K. et al. Tuning the Synthesis of Ternary Lead Chalcogenide Quantum Dots by Balancing Precursor Reactivity // ACS Nano. 2010. Vol. 5. No. 1. pp. 183-190.

GOST all authors (up to 50) Copy

Smith D. K., Luther J. M., Semonin O. E., Nozik A. J., Beard M. C. Tuning the Synthesis of Ternary Lead Chalcogenide Quantum Dots by Balancing Precursor Reactivity // ACS Nano. 2010. Vol. 5. No. 1. pp. 183-190.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/nn102878u

UR - https://doi.org/10.1021/nn102878u

TI - Tuning the Synthesis of Ternary Lead Chalcogenide Quantum Dots by Balancing Precursor Reactivity

T2 - ACS Nano

AU - Smith, Danielle K.

AU - Semonin, Octavi E

AU - Luther, Joseph M.

AU - Nozik, Arthur J.

AU - Beard, Matthew C

PY - 2010

DA - 2010/12/08 00:00:00

PB - American Chemical Society (ACS)

SP - 183-190

IS - 1

VL - 5

SN - 1936-0851

SN - 1936-086X

ER -

BibTex |

Cite this

BibTex Copy

@article{2010_Smith,

author = {Danielle K. Smith and Octavi E Semonin and Joseph M. Luther and Arthur J. Nozik and Matthew C Beard},

title = {Tuning the Synthesis of Ternary Lead Chalcogenide Quantum Dots by Balancing Precursor Reactivity},

journal = {ACS Nano},

year = {2010},

volume = {5},

publisher = {American Chemical Society (ACS)},

month = {dec},

url = {https://doi.org/10.1021/nn102878u},

number = {1},

pages = {183--190},

doi = {10.1021/nn102878u}

}

MLA

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MLA Copy

Smith, Danielle K., et al. “Tuning the Synthesis of Ternary Lead Chalcogenide Quantum Dots by Balancing Precursor Reactivity.” ACS Nano, vol. 5, no. 1, Dec. 2010, pp. 183-190. https://doi.org/10.1021/nn102878u.

Found error?

Publisher

American Chemical Society (ACS)

Journal

ACS Nano

Quartile SCImago

Quartile WOS

Impact factor

17.1

ISSN

19360851 (Print)
1936086X (Electronic)