ACS Nano, volume 6, issue 9, pages 8448-8455

A charge-orbital balance picture of doping in colloidal quantum dot solids.

Oleksandr Voznyy ¹

David Zhitomirsky ¹

Philipp Stadler ¹

Zhijun Ning ¹

Sjoerd Hoogland ¹

Edward H Sargent ¹

Hide authors affiliations Show authors affiliations: 1 affiliation

Department of Electrical and Computer Engineering, University of Toronto, 10 King’s College Road, Toronto, Ontario, M5S 3G4, Canada |

Publication type: Journal Article

Publication date: 2012-09-07

American Chemical Society (ACS)

Journal: ACS Nano

Quartile SCImago

Quartile WOS

Impact factor: 17.1

ISSN: 19360851, 1936086X

DOI: 10.1021/nn303364d

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General Physics and Astronomy

General Materials Science

General Engineering

Abstract

We present a framework--validated using both modeling and experiment--to predict doping in CQD films. In the ionic semiconductors widely deployed in CQD films, the framework reduces to a simple accounting of the contributions of the oxidation state of each constituent, including both inorganic species and organic ligands. We use density functional theory simulations to confirm that the type of doping can be reliably predicted based on the overall stoichiometry of the CQDs, largely independent of microscopic geometrical bonding configurations. Studies employing field-effect transistors constructed from CQDs that have undergone various chemical treatments, coupled with Rutherford backscattering and X-ray photoelectron spectroscopy to provide compositional analysis, allow us to test and confirm the proposed model in an experimental framework. We investigate both p- and n-type electronic doping spanning a wide range of carrier concentrations from 10(16) cm(-3) to over 10(18) cm(-3), and demonstrate reversible switching between p- and n-type doping by changing the CQD stoichiometry. We show that the summation of the contributions from all cations and anions within the film can be used to predict accurately the majority carrier type. The findings enable predictable control over majority carrier concentration via tuning of the overall stoichiometry.

By date By citations

Top-30

Citations by journals

	2 4 6 8 10 12 14 16 18
ACS Nano	ACS Nano, 18, 8.57% ACS Nano 18 publications, 8.57%
Chemistry of Materials	Chemistry of Materials, 15, 7.14% Chemistry of Materials 15 publications, 7.14%
Advanced Materials	Advanced Materials, 11, 5.24% Advanced Materials 11 publications, 5.24%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 9, 4.29% Journal of Physical Chemistry Letters 9 publications, 4.29%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 8, 3.81% Journal of Physical Chemistry C 8 publications, 3.81%
Nano Letters	Nano Letters, 7, 3.33% Nano Letters 7 publications, 3.33%
ACS applied materials & interfaces	ACS applied materials & interfaces, 7, 3.33% ACS applied materials & interfaces 7 publications, 3.33%
Chemical Reviews	Chemical Reviews, 6, 2.86% Chemical Reviews 6 publications, 2.86%
Nature Communications	Nature Communications, 5, 2.38% Nature Communications 5 publications, 2.38%
Scientific Reports	Scientific Reports, 5, 2.38% Scientific Reports 5 publications, 2.38%
Advanced Functional Materials	Advanced Functional Materials, 5, 2.38% Advanced Functional Materials 5 publications, 2.38%
ACS Energy Letters	ACS Energy Letters, 5, 2.38% ACS Energy Letters 5 publications, 2.38%
Applied Physics Letters	Applied Physics Letters, 4, 1.9% Applied Physics Letters 4 publications, 1.9%
Energy and Environmental Science	Energy and Environmental Science, 4, 1.9% Energy and Environmental Science 4 publications, 1.9%
Nanoscale	Nanoscale, 4, 1.9% Nanoscale 4 publications, 1.9%
Nature Materials	Nature Materials, 3, 1.43% Nature Materials 3 publications, 1.43%
Applied Surface Science	Applied Surface Science, 3, 1.43% Applied Surface Science 3 publications, 1.43%
Advanced Energy Materials	Advanced Energy Materials, 3, 1.43% Advanced Energy Materials 3 publications, 1.43%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 3, 1.43% Journal of Materials Chemistry C 3 publications, 1.43%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 3, 1.43% Physical Chemistry Chemical Physics 3 publications, 1.43%
Chemical Society Reviews	Chemical Society Reviews, 3, 1.43% Chemical Society Reviews 3 publications, 1.43%
Communications Materials	Communications Materials, 2, 0.95% Communications Materials 2 publications, 0.95%
Nanotechnology	Nanotechnology, 2, 0.95% Nanotechnology 2 publications, 0.95%
Procedia Engineering	Procedia Engineering, 2, 0.95% Procedia Engineering 2 publications, 0.95%
Organic Electronics	Organic Electronics, 2, 0.95% Organic Electronics 2 publications, 0.95%
Journal of the American Chemical Society	Journal of the American Chemical Society, 2, 0.95% Journal of the American Chemical Society 2 publications, 0.95%
ACS Applied Energy Materials	ACS Applied Energy Materials, 2, 0.95% ACS Applied Energy Materials 2 publications, 0.95%
Accounts of Chemical Research	Accounts of Chemical Research, 2, 0.95% Accounts of Chemical Research 2 publications, 0.95%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 2, 0.95% Journal of Materials Chemistry A 2 publications, 0.95%
	2 4 6 8 10 12 14 16 18

Citations by publishers

	10 20 30 40 50 60 70 80 90
American Chemical Society (ACS)	American Chemical Society (ACS), 88, 41.9% American Chemical Society (ACS) 88 publications, 41.9%
Wiley	Wiley, 30, 14.29% Wiley 30 publications, 14.29%
Springer Nature	Springer Nature, 24, 11.43% Springer Nature 24 publications, 11.43%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 22, 10.48% Royal Society of Chemistry (RSC) 22 publications, 10.48%
Elsevier	Elsevier, 20, 9.52% Elsevier 20 publications, 9.52%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 5, 2.38% American Institute of Physics (AIP) 5 publications, 2.38%
IEEE	IEEE, 3, 1.43% IEEE 3 publications, 1.43%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 0.95% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 0.95%
Cambridge University Press	Cambridge University Press, 2, 0.95% Cambridge University Press 2 publications, 0.95%
IOP Publishing	IOP Publishing, 2, 0.95% IOP Publishing 2 publications, 0.95%
Walter de Gruyter	Walter de Gruyter, 2, 0.95% Walter de Gruyter 2 publications, 0.95%
American Physical Society (APS)	American Physical Society (APS), 1, 0.48% American Physical Society (APS) 1 publication, 0.48%
Pleiades Publishing	Pleiades Publishing, 1, 0.48% Pleiades Publishing 1 publication, 0.48%
Taylor & Francis	Taylor & Francis, 1, 0.48% Taylor & Francis 1 publication, 0.48%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.48% American Association for the Advancement of Science (AAAS) 1 publication, 0.48%
Trans Tech Publications	Trans Tech Publications, 1, 0.48% Trans Tech Publications 1 publication, 0.48%
SPIE	SPIE, 1, 0.48% SPIE 1 publication, 0.48%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.48% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.48%
	10 20 30 40 50 60 70 80 90

We do not take into account publications without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

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GOST Copy

Voznyy O. et al. A charge-orbital balance picture of doping in colloidal quantum dot solids. // ACS Nano. 2012. Vol. 6. No. 9. pp. 8448-8455.

GOST all authors (up to 50) Copy

Voznyy O., Zhitomirsky D., Stadler P., Ning Z., Hoogland S., Sargent E. H. A charge-orbital balance picture of doping in colloidal quantum dot solids. // ACS Nano. 2012. Vol. 6. No. 9. pp. 8448-8455.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1021/nn303364d

UR - https://doi.org/10.1021/nn303364d

TI - A charge-orbital balance picture of doping in colloidal quantum dot solids.

T2 - ACS Nano

AU - Zhitomirsky, David

AU - Voznyy, Oleksandr

AU - Stadler, Philipp

AU - Ning, Zhijun

AU - Hoogland, Sjoerd

AU - Sargent, Edward H

PY - 2012

DA - 2012/09/07 00:00:00

PB - American Chemical Society (ACS)

SP - 8448-8455

IS - 9

VL - 6

SN - 1936-0851

SN - 1936-086X

ER -

BibTex |

Cite this

BibTex Copy

@article{2012_Voznyy,

author = {David Zhitomirsky and Oleksandr Voznyy and Philipp Stadler and Zhijun Ning and Sjoerd Hoogland and Edward H Sargent},

title = {A charge-orbital balance picture of doping in colloidal quantum dot solids.},

journal = {ACS Nano},

year = {2012},

volume = {6},

publisher = {American Chemical Society (ACS)},

month = {sep},

url = {https://doi.org/10.1021/nn303364d},

number = {9},

pages = {8448--8455},

doi = {10.1021/nn303364d}

}

MLA

Cite this

MLA Copy

Voznyy, Oleksandr, et al. “A charge-orbital balance picture of doping in colloidal quantum dot solids..” ACS Nano, vol. 6, no. 9, Sep. 2012, pp. 8448-8455. https://doi.org/10.1021/nn303364d.

Found error?

Publisher

American Chemical Society (ACS)

Journal

ACS Nano

Quartile SCImago

Quartile WOS

Impact factor

17.1

ISSN

19360851 (Print)
1936086X (Electronic)