The Regioselective Switch for Amino-NHC Mediated C–H Activation of Benzimidazole via Ni–Al Synergistic Catalysis
Wei Chun Shih
1
,
Wen-Ching CHEN
1
,
Ying Chieh Lai
1
,
Ming Shiuan Yu
1
,
Jhao Jhe Ho
1
,
Glenn P. A. Yap
1
,
T. Tzen Ong
1
Publication type: Journal Article
Publication date: 2012-04-05
scimago Q1
wos Q1
SJR: 1.235
CiteScore: 8.7
Impact factor: 5.0
ISSN: 15237060, 15237052
PubMed ID:
22480155
Organic Chemistry
Biochemistry
Physical and Theoretical Chemistry
Abstract
We have disclosed a new mode of a chemically regioselective switch for C-H bond functionalization of benzimidazole derivatives via a cooperative effect invoked by Ni-Al bimetallic catalysis to create a steric requirement for obtaining the linear product of styrene insertion. Yet, excluding the AlMe(3) cocatalyst switches the reaction toward branch selectivity.
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Metrics
93
Total citations:
93
Citations from 2025:
4
(4.3%)
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MLA
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GOST
Copy
Shih W. C. et al. The Regioselective Switch for Amino-NHC Mediated C–H Activation of Benzimidazole via Ni–Al Synergistic Catalysis // Organic Letters. 2012. Vol. 14. No. 8. pp. 2046-2049.
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Shih W. C., CHEN W., Lai Y. C., Yu M. S., Ho J. J., Yap G. P. A., Ong T. T. The Regioselective Switch for Amino-NHC Mediated C–H Activation of Benzimidazole via Ni–Al Synergistic Catalysis // Organic Letters. 2012. Vol. 14. No. 8. pp. 2046-2049.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/ol300570f
UR - https://doi.org/10.1021/ol300570f
TI - The Regioselective Switch for Amino-NHC Mediated C–H Activation of Benzimidazole via Ni–Al Synergistic Catalysis
T2 - Organic Letters
AU - Shih, Wei Chun
AU - CHEN, Wen-Ching
AU - Lai, Ying Chieh
AU - Yu, Ming Shiuan
AU - Ho, Jhao Jhe
AU - Yap, Glenn P. A.
AU - Ong, T. Tzen
PY - 2012
DA - 2012/04/05
PB - American Chemical Society (ACS)
SP - 2046-2049
IS - 8
VL - 14
PMID - 22480155
SN - 1523-7060
SN - 1523-7052
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2012_Shih,
author = {Wei Chun Shih and Wen-Ching CHEN and Ying Chieh Lai and Ming Shiuan Yu and Jhao Jhe Ho and Glenn P. A. Yap and T. Tzen Ong},
title = {The Regioselective Switch for Amino-NHC Mediated C–H Activation of Benzimidazole via Ni–Al Synergistic Catalysis},
journal = {Organic Letters},
year = {2012},
volume = {14},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/ol300570f},
number = {8},
pages = {2046--2049},
doi = {10.1021/ol300570f}
}
Cite this
MLA
Copy
Shih, Wei Chun, et al. “The Regioselective Switch for Amino-NHC Mediated C–H Activation of Benzimidazole via Ni–Al Synergistic Catalysis.” Organic Letters, vol. 14, no. 8, Apr. 2012, pp. 2046-2049. https://doi.org/10.1021/ol300570f.