Influence of intermolecular hydrogen bonding on magnetic properties of mononuclear cobalt and nickel pivalates with amidine ligands
I.G. Fomina
1
,
A. A. Sidorov
1
,
G.G. Aleksandrov
1
,
T B Mikhailova
1
,
E V Pakhmutova
1
,
V. M. Novotortsev
1
,
V. N. Ikorskii
2
,
Publication type: Journal Article
Publication date: 2004-07-01
scimago Q3
SJR: 0.305
CiteScore: 2.8
Impact factor: —
ISSN: 10665285, 15739171
General Chemistry
Abstract
The magnetic properties of the mononuclear cobalt(ii) amidine complex Co(Me3CCOO)2{H2N(C5H3N)NH(MeC=NH} (1) having a tetrahedral structure and its solvate 1·HOOCCMe3·0.5C6H6 (1a) are substantially different. Complex 1 possesses ferromagnetic properties and exhibits residual magnetization at liquid-helium temperatures, whereas solvate 1a and the octahedral amidine complex Ni(Me3CCOO)2{H2N(C5H3N)NH(MeC=NH}·MeCN (3·MeCN) show antiferromagnetic properties. Apparently, this is associated with the difference in the type of intermolecular nonbonded interactions in the crystals of 1, 1a, and 3·MeCN, which form channels for spin-spin exchange. The tetrahedral isostructural mononuclear complexes ML2 (M = Co (5), Ni (6), L is N-tosyl-2,5-dimethyl-8-aminoquinoline) were synthesized. These complexes exhibit antiferromagnetic properties.
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Fomina I. et al. Influence of intermolecular hydrogen bonding on magnetic properties of mononuclear cobalt and nickel pivalates with amidine ligands // Russian Chemical Bulletin. 2004. Vol. 53. No. 7. pp. 1477-1487.
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Fomina I., Sidorov A. A., Aleksandrov G., Mikhailova T. B., Pakhmutova E. V., Novotortsev V. M., Ikorskii V. N., Eremenko I. L. Influence of intermolecular hydrogen bonding on magnetic properties of mononuclear cobalt and nickel pivalates with amidine ligands // Russian Chemical Bulletin. 2004. Vol. 53. No. 7. pp. 1477-1487.
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TY - JOUR
DO - 10.1023/B:RUCB.0000046244.43123.98
UR - https://doi.org/10.1023/B:RUCB.0000046244.43123.98
TI - Influence of intermolecular hydrogen bonding on magnetic properties of mononuclear cobalt and nickel pivalates with amidine ligands
T2 - Russian Chemical Bulletin
AU - Fomina, I.G.
AU - Sidorov, A. A.
AU - Aleksandrov, G.G.
AU - Mikhailova, T B
AU - Pakhmutova, E V
AU - Novotortsev, V. M.
AU - Ikorskii, V. N.
AU - Eremenko, I. L.
PY - 2004
DA - 2004/07/01
PB - Springer Nature
SP - 1477-1487
IS - 7
VL - 53
SN - 1066-5285
SN - 1573-9171
ER -
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BibTex (up to 50 authors)
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@article{2004_Fomina,
author = {I.G. Fomina and A. A. Sidorov and G.G. Aleksandrov and T B Mikhailova and E V Pakhmutova and V. M. Novotortsev and V. N. Ikorskii and I. L. Eremenko},
title = {Influence of intermolecular hydrogen bonding on magnetic properties of mononuclear cobalt and nickel pivalates with amidine ligands},
journal = {Russian Chemical Bulletin},
year = {2004},
volume = {53},
publisher = {Springer Nature},
month = {jul},
url = {https://doi.org/10.1023/B:RUCB.0000046244.43123.98},
number = {7},
pages = {1477--1487},
doi = {10.1023/B:RUCB.0000046244.43123.98}
}
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MLA
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Fomina, I.G., et al. “Influence of intermolecular hydrogen bonding on magnetic properties of mononuclear cobalt and nickel pivalates with amidine ligands.” Russian Chemical Bulletin, vol. 53, no. 7, Jul. 2004, pp. 1477-1487. https://doi.org/10.1023/B:RUCB.0000046244.43123.98.