Nature, volume 275, issue 5676, pages 115-116
Photoelectrochemical reduction of aqueous carbon dioxide on p-type gallium phosphide in liquid junction solar cells
Publication type: Journal Article
Publication date: 1978-09-01
DOI:
10.1038/275115a0
Multidisciplinary
Abstract
THE non-biological reduction of carbon dioxide to organic compounds is of interest, as an alternative to natural photosynthesis, for the production of organic raw materials or fuel. In one approach, the required energy was supplied by irradiation with UV light, in the presence of ferrous salts, and resulted in the production of formic acid and of formaldehyde1. In another approach, the energy was supplied from an external power source by electrochemical reduction of aqueous carbon dioxide. The reduction of carbon dioxide and production of formic acid during the electrolysis of sodium bicarbonate in aqueous solutions has also been reported2, and a study of the reduction of carbon dioxide on a mercury cathode reviews earlier work3. Polarographic measurements on mercury electrodes showed that carbon dioxide, rather than the bicarbonate ion, is the electroactive species, with a half-wave reduction potential of −2.1 V (relative to SCE), and that formic acid is the only product4. We report here the photoassisted electrolytic reduction of aqueous carbon dioxide, achieved using p-type gallium phosphide as a photocathode, with part or all of the energy being supplied by light. The products were formic acid, formaldehyde and methanol.
Top-30
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6 publications, 0.73%
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Citations by publishers
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Elsevier
293 publications, 35.56%
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Wiley
140 publications, 16.99%
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American Chemical Society (ACS)
118 publications, 14.32%
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Springer Nature
47 publications, 5.7%
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17 publications, 2.06%
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IOP Publishing
12 publications, 1.46%
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The Chemical Society of Japan
8 publications, 0.97%
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Trans Tech Publications
6 publications, 0.73%
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Taylor & Francis
5 publications, 0.61%
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American Institute of Physics (AIP)
3 publications, 0.36%
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Proceedings of the National Academy of Sciences (PNAS)
3 publications, 0.36%
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The Electrochemical Society
2 publications, 0.24%
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Frontiers Media S.A.
2 publications, 0.24%
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Walter de Gruyter
2 publications, 0.24%
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Hindawi Limited
2 publications, 0.24%
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EDP Sciences
1 publication, 0.12%
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World Scientific
1 publication, 0.12%
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Thomas Telford
1 publication, 0.12%
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Shanghai Institute of Organic Chemistry
1 publication, 0.12%
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Shanghai Institute of Ceramics
1 publication, 0.12%
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Tianjin Daxue/Tianjin University
1 publication, 0.12%
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Korean Society of Industrial Engineering Chemistry
1 publication, 0.12%
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IGI Global
1 publication, 0.12%
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Oxford University Press
1 publication, 0.12%
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Scientific Research Publishing
1 publication, 0.12%
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American Association for the Advancement of Science (AAAS)
1 publication, 0.12%
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1 publication, 0.12%
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Annual Reviews
1 publication, 0.12%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Halmann M. Photoelectrochemical reduction of aqueous carbon dioxide on p-type gallium phosphide in liquid junction solar cells // Nature. 1978. Vol. 275. No. 5676. pp. 115-116.
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Halmann M. Photoelectrochemical reduction of aqueous carbon dioxide on p-type gallium phosphide in liquid junction solar cells // Nature. 1978. Vol. 275. No. 5676. pp. 115-116.
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TY - JOUR
DO - 10.1038/275115a0
UR - https://doi.org/10.1038/275115a0
TI - Photoelectrochemical reduction of aqueous carbon dioxide on p-type gallium phosphide in liquid junction solar cells
T2 - Nature
AU - Halmann, M.
PY - 1978
DA - 1978/09/01 00:00:00
PB - Springer Nature
SP - 115-116
IS - 5676
VL - 275
SN - 0028-0836
SN - 1476-4687
ER -
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@article{1978_Halmann,
author = {M. Halmann},
title = {Photoelectrochemical reduction of aqueous carbon dioxide on p-type gallium phosphide in liquid junction solar cells},
journal = {Nature},
year = {1978},
volume = {275},
publisher = {Springer Nature},
month = {sep},
url = {https://doi.org/10.1038/275115a0},
number = {5676},
pages = {115--116},
doi = {10.1038/275115a0}
}
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MLA
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Halmann, M.. “Photoelectrochemical reduction of aqueous carbon dioxide on p-type gallium phosphide in liquid junction solar cells.” Nature, vol. 275, no. 5676, Sep. 1978, pp. 115-116. https://doi.org/10.1038/275115a0.