Nature Materials, volume 10, issue 10, pages 765-771
Colloidal-quantum-dot photovoltaics using atomic-ligand passivation.
Jiang Tang
1
,
Kyle W Kemp
1
,
Sjoerd Hoogland
1
,
Kwang S Jeong
2
,
Huan Liu
1, 3
,
Larissa Levina
1
,
Melissa Furukawa
1
,
Xihua Wang
1
,
Ratan Debnath
1
,
Dongkyu Cha
4
,
Kang Wei Chou
5
,
Armin Fischer
1
,
Aram Amassian
5
,
John B. Asbury
2
,
Edward H Sargent
1
1
Department of electrical and computer engineering, University of Toronto, Toronto, Ontario, M5S 3G4, Canada
|
2
Publication type: Journal Article
Publication date: 2011-09-18
Journal:
Nature Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 41.2
ISSN: 14761122, 14764660
DOI:
10.1038/nmat3118
General Chemistry
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Mechanics of Materials
Abstract
Colloidal-quantum-dot (CQD) optoelectronics offer a compelling combination of solution processing and spectral tunability through quantum size effects. So far, CQD solar cells have relied on the use of organic ligands to passivate the surface of the semiconductor nanoparticles. Although inorganic metal chalcogenide ligands have led to record electronic transport parameters in CQD films, no photovoltaic device has been reported based on such compounds. Here we establish an atomic ligand strategy that makes use of monovalent halide anions to enhance electronic transport and successfully passivate surface defects in PbS CQD films. Both time-resolved infrared spectroscopy and transient device characterization indicate that the scheme leads to a shallower trap state distribution than the best organic ligands. Solar cells fabricated following this strategy show up to 6% solar AM1.5G power-conversion efficiency. The CQD films are deposited at room temperature and under ambient atmosphere, rendering the process amenable to low-cost, roll-by-roll fabrication.
Top-30
Citations by journals
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26 publications, 1.9%
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17 publications, 1.25%
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17 publications, 1.25%
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16 publications, 1.17%
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14 publications, 1.03%
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ACS Photonics
14 publications, 1.03%
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13 publications, 0.95%
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ACS Energy Letters
13 publications, 0.95%
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12 publications, 0.88%
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11 publications, 0.81%
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Langmuir
11 publications, 0.81%
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Citations by publishers
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American Chemical Society (ACS)
436 publications, 31.94%
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Wiley
217 publications, 15.9%
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Elsevier
215 publications, 15.75%
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Royal Society of Chemistry (RSC)
192 publications, 14.07%
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Springer Nature
112 publications, 8.21%
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American Institute of Physics (AIP)
41 publications, 3%
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Multidisciplinary Digital Publishing Institute (MDPI)
26 publications, 1.9%
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IOP Publishing
24 publications, 1.76%
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IEEE
10 publications, 0.73%
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Hindawi Limited
7 publications, 0.51%
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Taylor & Francis
6 publications, 0.44%
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Optical Society of America
5 publications, 0.37%
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American Physical Society (APS)
4 publications, 0.29%
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American Association for the Advancement of Science (AAAS)
4 publications, 0.29%
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Materials Research Society
3 publications, 0.22%
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Japan Society of Applied Physics
3 publications, 0.22%
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World Scientific
2 publications, 0.15%
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Frontiers Media S.A.
2 publications, 0.15%
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Cambridge University Press
2 publications, 0.15%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
2 publications, 0.15%
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Pleiades Publishing
2 publications, 0.15%
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Walter de Gruyter
2 publications, 0.15%
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Opto-Electronic Advances
2 publications, 0.15%
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Trans Tech Publications
2 publications, 0.15%
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Beilstein-Institut
1 publication, 0.07%
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American Scientific Publishers
1 publication, 0.07%
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American Vacuum Society
1 publication, 0.07%
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The Chemical Society of Japan
1 publication, 0.07%
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EDP Sciences
1 publication, 0.07%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Tang J. et al. Colloidal-quantum-dot photovoltaics using atomic-ligand passivation. // Nature Materials. 2011. Vol. 10. No. 10. pp. 765-771.
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Tang J., Kemp K. W., Hoogland S., Jeong K. S., Liu H., Levina L., Furukawa M., Wang X., Debnath R., Cha D., Chou K. W., Fischer A., Amassian A., Asbury J. B., Sargent E. H. Colloidal-quantum-dot photovoltaics using atomic-ligand passivation. // Nature Materials. 2011. Vol. 10. No. 10. pp. 765-771.
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TY - JOUR
DO - 10.1038/nmat3118
UR - https://doi.org/10.1038/nmat3118
TI - Colloidal-quantum-dot photovoltaics using atomic-ligand passivation.
T2 - Nature Materials
AU - Tang, Jiang
AU - Kemp, Kyle W
AU - Hoogland, Sjoerd
AU - Jeong, Kwang S
AU - Liu, Huan
AU - Levina, Larissa
AU - Furukawa, Melissa
AU - Wang, Xihua
AU - Debnath, Ratan
AU - Cha, Dongkyu
AU - Chou, Kang Wei
AU - Fischer, Armin
AU - Amassian, Aram
AU - Asbury, John B.
AU - Sargent, Edward H
PY - 2011
DA - 2011/09/18 00:00:00
PB - Springer Nature
SP - 765-771
IS - 10
VL - 10
SN - 1476-1122
SN - 1476-4660
ER -
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@article{2011_Tang,
author = {Jiang Tang and Kyle W Kemp and Sjoerd Hoogland and Kwang S Jeong and Huan Liu and Larissa Levina and Melissa Furukawa and Xihua Wang and Ratan Debnath and Dongkyu Cha and Kang Wei Chou and Armin Fischer and Aram Amassian and John B. Asbury and Edward H Sargent},
title = {Colloidal-quantum-dot photovoltaics using atomic-ligand passivation.},
journal = {Nature Materials},
year = {2011},
volume = {10},
publisher = {Springer Nature},
month = {sep},
url = {https://doi.org/10.1038/nmat3118},
number = {10},
pages = {765--771},
doi = {10.1038/nmat3118}
}
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Tang, Jiang, et al. “Colloidal-quantum-dot photovoltaics using atomic-ligand passivation..” Nature Materials, vol. 10, no. 10, Sep. 2011, pp. 765-771. https://doi.org/10.1038/nmat3118.