Nature, volume 420, issue 6917, pages 800-803

Electroluminescence from single monolayers of nanocrystals in molecular organic devices

Seth Coe ¹

Wing-Keung Woo ²

Moungi Bawendi ²

Vladimir Bulović ¹

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Laboratory of Organic Optoelectronics, Department of Electrical Engineering and Computer Science,

Center for Materials Science and Engineering, Department of Chemistry, Massachusetts Institute of Technology, Cambridge, USA |

Publication type: Journal Article

Publication date: 2002-12-18

Springer Nature

Journal: Nature

Quartile SCImago

Quartile WOS

Impact factor: 64.8

ISSN: 00280836, 14764687

DOI: 10.1038/nature01217

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Multidisciplinary

Abstract

The integration of organic and inorganic materials at the nanometre scale into hybrid optoelectronic structures enables active devices1,2,3 that combine the diversity of organic materials with the high-performance electronic and optical properties of inorganic nanocrystals4. The optimization of such hybrid devices ultimately depends upon the precise positioning of the functionally distinct materials. Previous studies5,6 have already emphasized that this is a challenge, owing to the lack of well-developed nanometre-scale fabrication techniques. Here we demonstrate a hybrid light-emitting diode (LED) that combines the ease of processability of organic materials with the narrow-band, efficient luminescence of colloidal quantum dots7 (QDs). To isolate the luminescence processes from charge conduction, we fabricate a quantum-dot LED (QD-LED) that contains only a single monolayer of QDs, sandwiched between two organic thin films. This is achieved by a method that uses material phase segregation between the QD aliphatic capping groups and the aromatic organic materials. In our devices, where QDs function exclusively as lumophores, we observe a 25-fold improvement in luminescence efficiency (1.6 cd A-1 at 2,000 cd m-2) over the best previous QD-LED results5. The reproducibility and precision of our phase-segregation approach suggests that this technique could be widely applicable to the fabrication of other hybrid organic/inorganic devices.

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Citations by journals

	20 40 60 80 100 120
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 114, 5.01% Journal of Physical Chemistry C 114 publications, 5.01%
Applied Physics Letters	Applied Physics Letters, 79, 3.47% Applied Physics Letters 79 publications, 3.47%
Nano Letters	Nano Letters, 70, 3.08% Nano Letters 70 publications, 3.08%
Advanced Materials	Advanced Materials, 57, 2.51% Advanced Materials 57 publications, 2.51%
ACS Nano	ACS Nano, 53, 2.33% ACS Nano 53 publications, 2.33%
Nanotechnology	Nanotechnology, 53, 2.33% Nanotechnology 53 publications, 2.33%
Chemistry of Materials	Chemistry of Materials, 52, 2.29% Chemistry of Materials 52 publications, 2.29%
Nanoscale	Nanoscale, 49, 2.15% Nanoscale 49 publications, 2.15%
Journal of the American Chemical Society	Journal of the American Chemical Society, 41, 1.8% Journal of the American Chemical Society 41 publications, 1.8%
ACS applied materials & interfaces	ACS applied materials & interfaces, 40, 1.76% ACS applied materials & interfaces 40 publications, 1.76%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 38, 1.67% Journal of Materials Chemistry C 38 publications, 1.67%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 35, 1.54% Journal of Materials Chemistry A 35 publications, 1.54%
Advanced Functional Materials	Advanced Functional Materials, 33, 1.45% Advanced Functional Materials 33 publications, 1.45%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 30, 1.32% Journal of Physical Chemistry Letters 30 publications, 1.32%
SID Symposium Digest of Technical Papers	SID Symposium Digest of Technical Papers, 29, 1.27% SID Symposium Digest of Technical Papers 29 publications, 1.27%
RSC Advances	RSC Advances, 29, 1.27% RSC Advances 29 publications, 1.27%
Journal of Applied Physics	Journal of Applied Physics, 28, 1.23% Journal of Applied Physics 28 publications, 1.23%
Langmuir	Langmuir, 28, 1.23% Langmuir 28 publications, 1.23%
Journal of Luminescence	Journal of Luminescence, 25, 1.1% Journal of Luminescence 25 publications, 1.1%
Physical Review B	Physical Review B, 24, 1.05% Physical Review B 24 publications, 1.05%
Chemical Communications	Chemical Communications, 22, 0.97% Chemical Communications 22 publications, 0.97%
Journal of Physical Chemistry B	Journal of Physical Chemistry B, 20, 0.88% Journal of Physical Chemistry B 20 publications, 0.88%
Organic Electronics	Organic Electronics, 19, 0.84% Organic Electronics 19 publications, 0.84%
Small	Small, 19, 0.84% Small 19 publications, 0.84%
Nature Communications	Nature Communications, 19, 0.84% Nature Communications 19 publications, 0.84%
Applied Surface Science	Applied Surface Science, 18, 0.79% Applied Surface Science 18 publications, 0.79%
Journal of Materials Science: Materials in Electronics	Journal of Materials Science: Materials in Electronics, 18, 0.79% Journal of Materials Science: Materials in Electronics 18 publications, 0.79%
MRS Proceedings	MRS Proceedings, 18, 0.79% MRS Proceedings 18 publications, 0.79%
Journal of Chemical Physics	Journal of Chemical Physics, 17, 0.75% Journal of Chemical Physics 17 publications, 0.75%
	20 40 60 80 100 120

Citations by publishers

	100 200 300 400 500 600
American Chemical Society (ACS)	American Chemical Society (ACS), 517, 22.73% American Chemical Society (ACS) 517 publications, 22.73%
Elsevier	Elsevier, 357, 15.69% Elsevier 357 publications, 15.69%
Wiley	Wiley, 288, 12.66% Wiley 288 publications, 12.66%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 245, 10.77% Royal Society of Chemistry (RSC) 245 publications, 10.77%
Springer Nature	Springer Nature, 225, 9.89% Springer Nature 225 publications, 9.89%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 133, 5.85% American Institute of Physics (AIP) 133 publications, 5.85%
IOP Publishing	IOP Publishing, 102, 4.48% IOP Publishing 102 publications, 4.48%
American Physical Society (APS)	American Physical Society (APS), 34, 1.49% American Physical Society (APS) 34 publications, 1.49%
Taylor & Francis	Taylor & Francis, 23, 1.01% Taylor & Francis 23 publications, 1.01%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 22, 0.97% Multidisciplinary Digital Publishing Institute (MDPI) 22 publications, 0.97%
IEEE	IEEE, 21, 0.92% IEEE 21 publications, 0.92%
Materials Research Society	Materials Research Society, 19, 0.84% Materials Research Society 19 publications, 0.84%
Optical Society of America	Optical Society of America, 18, 0.79% Optical Society of America 18 publications, 0.79%
Pleiades Publishing	Pleiades Publishing, 16, 0.7% Pleiades Publishing 16 publications, 0.7%
SPIE	SPIE, 11, 0.48% SPIE 11 publications, 0.48%
Cambridge University Press	Cambridge University Press, 11, 0.48% Cambridge University Press 11 publications, 0.48%
The Electrochemical Society	The Electrochemical Society, 10, 0.44% The Electrochemical Society 10 publications, 0.44%
Trans Tech Publications	Trans Tech Publications, 10, 0.44% Trans Tech Publications 10 publications, 0.44%
The Chemical Society of Japan	The Chemical Society of Japan, 9, 0.4% The Chemical Society of Japan 9 publications, 0.4%
Japan Society of Applied Physics	Japan Society of Applied Physics, 9, 0.4% Japan Society of Applied Physics 9 publications, 0.4%
Hindawi Limited	Hindawi Limited, 9, 0.4% Hindawi Limited 9 publications, 0.4%
Walter de Gruyter	Walter de Gruyter, 6, 0.26% Walter de Gruyter 6 publications, 0.26%
American Vacuum Society	American Vacuum Society, 5, 0.22% American Vacuum Society 5 publications, 0.22%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 5, 0.22% American Association for the Advancement of Science (AAAS) 5 publications, 0.22%
World Scientific	World Scientific, 4, 0.18% World Scientific 4 publications, 0.18%
Korean Institute of Metals and Materials	Korean Institute of Metals and Materials, 4, 0.18% Korean Institute of Metals and Materials 4 publications, 0.18%
Beilstein-Institut	Beilstein-Institut, 3, 0.13% Beilstein-Institut 3 publications, 0.13%
Institution of Engineering and Technology (IET)	Institution of Engineering and Technology (IET), 3, 0.13% Institution of Engineering and Technology (IET) 3 publications, 0.13%
SAGE	SAGE, 3, 0.13% SAGE 3 publications, 0.13%
	100 200 300 400 500 600

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Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

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Coe S. et al. Electroluminescence from single monolayers of nanocrystals in molecular organic devices // Nature. 2002. Vol. 420. No. 6917. pp. 800-803.

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Coe S., Woo W., Bawendi M., Bulović V. Electroluminescence from single monolayers of nanocrystals in molecular organic devices // Nature. 2002. Vol. 420. No. 6917. pp. 800-803.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1038/nature01217

UR - https://doi.org/10.1038/nature01217

TI - Electroluminescence from single monolayers of nanocrystals in molecular organic devices

T2 - Nature

AU - Coe, Seth

AU - Woo, Wing-Keung

AU - Bawendi, Moungi

AU - Bulović, Vladimir

PY - 2002

DA - 2002/12/18 00:00:00

PB - Springer Nature

SP - 800-803

IS - 6917

VL - 420

SN - 0028-0836

SN - 1476-4687

ER -

BibTex |

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BibTex Copy

@article{2002_Coe,

author = {Seth Coe and Wing-Keung Woo and Moungi Bawendi and Vladimir Bulović},

title = {Electroluminescence from single monolayers of nanocrystals in molecular organic devices},

journal = {Nature},

year = {2002},

volume = {420},

publisher = {Springer Nature},

month = {dec},

url = {https://doi.org/10.1038/nature01217},

number = {6917},

pages = {800--803},

doi = {10.1038/nature01217}

}

MLA

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MLA Copy

Coe, Seth, et al. “Electroluminescence from single monolayers of nanocrystals in molecular organic devices.” Nature, vol. 420, no. 6917, Dec. 2002, pp. 800-803. https://doi.org/10.1038/nature01217.

Found error?

Publisher

Springer Nature

Journal

Nature

Quartile SCImago

Quartile WOS

Impact factor

64.8

ISSN

00280836 (Print)
14764687 (Electronic)