Open Access

Nature Communications, volume 4, issue 1, publication number 2981

Heterovalent cation substitutional doping for quantum dot homojunction solar cells

Alexandros Stavrinadis ¹

Arup K. Rath ¹

F Pelayo García De Arquer ¹

Silke L Diedenhofen ¹

Cesar Magen ²

LUIS MARTÍNEZ ¹

David So ¹

Gerasimos Konstantatos ¹

Hide authors affiliations Show authors affiliations: 2 affiliations

ICFO-Institut de Ciències Fotòniques, Castelldefels, Spain |

Instituto de Nanociencia de Aragon (INA) - ARAID and Departamento de Fisica de la Materia Condensada, Laboratorio de Microscopías Avanzadas (LMA), Universidad de Zaragoza, Zaragoza, Spain |

Publication type: Journal Article

Publication date: 2013-12-18

Springer Nature

Journal: Nature Communications

Quartile SCImago

Quartile WOS

Impact factor: 16.6

ISSN: 20411723, 20411723

DOI: 10.1038/ncomms3981

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General Chemistry

General Biochemistry, Genetics and Molecular Biology

General Physics and Astronomy

Abstract

Colloidal quantum dots have emerged as a material platform for low-cost high-performance optoelectronics. At the heart of optoelectronic devices lies the formation of a junction, which requires the intimate contact of n-type and p-type semiconductors. Doping in bulk semiconductors has been largely deployed for many decades, yet electronically active doping in quantum dots has remained a challenge and the demonstration of robust functional optoelectronic devices had thus far been elusive. Here we report an optoelectronic device, a quantum dot homojunction solar cell, based on heterovalent cation substitution. We used PbS quantum dots as a reference material, which is a p-type semiconductor, and we employed Bi-doping to transform it into an n-type semiconductor. We then combined the two layers into a homojunction device operating as a solar cell robustly under ambient air conditions with power conversion efficiency of 2.7%. To use colloidal quantum dots in applications such as p-n junction solar cells, doping of the quantum dots is needed. Here, Stavrinadis et al. achieve lead sulphide quantum dot p-n homojunctions by heterovalent cation substitution of lead using bismuth.

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	1 2 3 4 5 6 7
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 7, 6.03% Journal of Physical Chemistry Letters 7 publications, 6.03%
Chemistry of Materials	Chemistry of Materials, 6, 5.17% Chemistry of Materials 6 publications, 5.17%
Journal of the American Chemical Society	Journal of the American Chemical Society, 5, 4.31% Journal of the American Chemical Society 5 publications, 4.31%
Advanced Materials	Advanced Materials, 4, 3.45% Advanced Materials 4 publications, 3.45%
ACS applied materials & interfaces	ACS applied materials & interfaces, 4, 3.45% ACS applied materials & interfaces 4 publications, 3.45%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 4, 3.45% Journal of Materials Chemistry A 4 publications, 3.45%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 3, 2.59% Journal of Physical Chemistry C 3 publications, 2.59%
ACS Applied Electronic Materials	ACS Applied Electronic Materials, 3, 2.59% ACS Applied Electronic Materials 3 publications, 2.59%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 3, 2.59% Journal of Materials Chemistry C 3 publications, 2.59%
Energy and Environmental Science	Energy and Environmental Science, 3, 2.59% Energy and Environmental Science 3 publications, 2.59%
Chemical Engineering Journal	Chemical Engineering Journal, 2, 1.72% Chemical Engineering Journal 2 publications, 1.72%
Surfaces and Interfaces	Surfaces and Interfaces, 2, 1.72% Surfaces and Interfaces 2 publications, 1.72%
Small	Small, 2, 1.72% Small 2 publications, 1.72%
Advanced Functional Materials	Advanced Functional Materials, 2, 1.72% Advanced Functional Materials 2 publications, 1.72%
Solar RRL	Solar RRL, 2, 1.72% Solar RRL 2 publications, 1.72%
Advanced Optical Materials	Advanced Optical Materials, 2, 1.72% Advanced Optical Materials 2 publications, 1.72%
ACS Energy Letters	ACS Energy Letters, 2, 1.72% ACS Energy Letters 2 publications, 1.72%
Nano Letters	Nano Letters, 2, 1.72% Nano Letters 2 publications, 1.72%
ACS Applied Nano Materials	ACS Applied Nano Materials, 2, 1.72% ACS Applied Nano Materials 2 publications, 1.72%
Applied Physics Letters	Applied Physics Letters, 1, 0.86% Applied Physics Letters 1 publication, 0.86%
Journal of Applied Physics	Journal of Applied Physics, 1, 0.86% Journal of Applied Physics 1 publication, 0.86%
Energies	Energies, 1, 0.86% Energies 1 publication, 0.86%
Nature Communications	Nature Communications, 1, 0.86% Nature Communications 1 publication, 0.86%
Nature Photonics	Nature Photonics, 1, 0.86% Nature Photonics 1 publication, 0.86%
Scientific Reports	Scientific Reports, 1, 0.86% Scientific Reports 1 publication, 0.86%
Journal of Cluster Science	Journal of Cluster Science, 1, 0.86% Journal of Cluster Science 1 publication, 0.86%
Applied Physics A: Materials Science and Processing	Applied Physics A: Materials Science and Processing, 1, 0.86% Applied Physics A: Materials Science and Processing 1 publication, 0.86%
Frontiers of Optoelectronics	Frontiers of Optoelectronics, 1, 0.86% Frontiers of Optoelectronics 1 publication, 0.86%
Nature Nanotechnology	Nature Nanotechnology, 1, 0.86% Nature Nanotechnology 1 publication, 0.86%
	1 2 3 4 5 6 7

Citations by publishers

	5 10 15 20 25 30 35 40
American Chemical Society (ACS)	American Chemical Society (ACS), 38, 32.76% American Chemical Society (ACS) 38 publications, 32.76%
Elsevier	Elsevier, 22, 18.97% Elsevier 22 publications, 18.97%
Wiley	Wiley, 20, 17.24% Wiley 20 publications, 17.24%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 15, 12.93% Royal Society of Chemistry (RSC) 15 publications, 12.93%
Springer Nature	Springer Nature, 9, 7.76% Springer Nature 9 publications, 7.76%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 3, 2.59% American Institute of Physics (AIP) 3 publications, 2.59%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 1.72% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 1.72%
IOP Publishing	IOP Publishing, 2, 1.72% IOP Publishing 2 publications, 1.72%
Optical Society of America	Optical Society of America, 1, 0.86% Optical Society of America 1 publication, 0.86%
Hindawi Limited	Hindawi Limited, 1, 0.86% Hindawi Limited 1 publication, 0.86%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.86% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.86%
	5 10 15 20 25 30 35 40

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Stavrinadis A. et al. Heterovalent cation substitutional doping for quantum dot homojunction solar cells // Nature Communications. 2013. Vol. 4. No. 1. 2981

GOST all authors (up to 50) Copy

Stavrinadis A., Rath A. K., De Arquer F. P. G., Diedenhofen S. L., Magen C., MARTÍNEZ L., So D., Konstantatos G. Heterovalent cation substitutional doping for quantum dot homojunction solar cells // Nature Communications. 2013. Vol. 4. No. 1. 2981

RIS |

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RIS Copy

TY - JOUR

DO - 10.1038/ncomms3981

UR - https://doi.org/10.1038/ncomms3981

TI - Heterovalent cation substitutional doping for quantum dot homojunction solar cells

T2 - Nature Communications

AU - Stavrinadis, Alexandros

AU - Rath, Arup K.

AU - De Arquer, F Pelayo García

AU - Diedenhofen, Silke L

AU - Magen, Cesar

AU - MARTÍNEZ, LUIS

AU - So, David

AU - Konstantatos, Gerasimos

PY - 2013

DA - 2013/12/18 00:00:00

PB - Springer Nature

IS - 1

VL - 4

SN - 2041-1723

ER -

BibTex

Cite this

BibTex Copy

@article{2013_Stavrinadis,

author = {Alexandros Stavrinadis and Arup K. Rath and F Pelayo García De Arquer and Silke L Diedenhofen and Cesar Magen and LUIS MARTÍNEZ and David So and Gerasimos Konstantatos},

title = {Heterovalent cation substitutional doping for quantum dot homojunction solar cells},

journal = {Nature Communications},

year = {2013},

volume = {4},

publisher = {Springer Nature},

month = {dec},

url = {https://doi.org/10.1038/ncomms3981},

number = {1},

doi = {10.1038/ncomms3981}

}

Found error?

Publisher

Springer Nature

Journal

Nature Communications

Quartile SCImago

Quartile WOS

Impact factor

16.6

ISSN

20411723 (Print)
20411723 (Electronic)