Nature Materials, volume 4, issue 2, pages 138-142

Solution-processed PbS quantum dot infrared photodetectors and photovoltaics

Steven A Mcdonald ¹

Gerasimos Konstantatos ¹

Shiguo Zhang ¹

Paul W. Cyr ^{1, 2}

Ethan J. D. Klem ¹

Larissa Levina ¹

Edward H Sargent ¹

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Department of Electrical and Computer Engineering, University of Toronto, Toronto, Canada |

Department of Chemistry, University of Toronto, Toronto, Canada |

Publication type: Journal Article

Publication date: 2005-01-09

Springer Nature

Journal: Nature Materials

Quartile SCImago

Quartile WOS

Impact factor: 41.2

ISSN: 14761122, 14764660

DOI: 10.1038/nmat1299

Copy DOI

General Chemistry

Condensed Matter Physics

General Materials Science

Mechanical Engineering

Mechanics of Materials

Abstract

In contrast to traditional semiconductors, conjugated polymers provide ease of processing, low cost, physical flexibility and large area coverage1. These active optoelectronic materials produce and harvest light efficiently in the visible spectrum. The same functions are required in the infrared for telecommunications (1,300–1,600 nm), thermal imaging (1,500 nm and beyond), biological imaging (transparent tissue windows at 800 nm and 1,100 nm), thermal photovoltaics (>1,900 nm), and solar cells (800–2,000 nm). Photoconductive polymer devices have yet to demonstrate sensitivity beyond ∼800 nm (refs 2,3). Sensitizing conjugated polymers with infrared-active nanocrystal quantum dots provides a spectrally tunable means of accessing the infrared while maintaining the advantageous properties of polymers. Here we use such a nanocomposite approach in which PbS nanocrystals tuned by the quantum size effect sensitize the conjugated polymer poly[2-methoxy-5-(2′-ethylhexyloxy-p-phenylenevinylene)] (MEH-PPV) into the infrared. We achieve, in a solution-processed device and with sensitivity far beyond 800 nm, harvesting of infrared-photogenerated carriers and the demonstration of an infrared photovoltaic effect. We also make use of the wavelength tunability afforded by the nanocrystals to show photocurrent spectra tailored to three different regions of the infrared spectrum.

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Citations by journals

	10 20 30 40 50 60 70 80
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 78, 4.44% Journal of Physical Chemistry C 78 publications, 4.44%
Advanced Materials	Advanced Materials, 66, 3.76% Advanced Materials 66 publications, 3.76%
ACS Nano	ACS Nano, 60, 3.42% ACS Nano 60 publications, 3.42%
ACS applied materials & interfaces	ACS applied materials & interfaces, 50, 2.85% ACS applied materials & interfaces 50 publications, 2.85%
Nano Letters	Nano Letters, 48, 2.73% Nano Letters 48 publications, 2.73%
Applied Physics Letters	Applied Physics Letters, 46, 2.62% Applied Physics Letters 46 publications, 2.62%
Nanoscale	Nanoscale, 46, 2.62% Nanoscale 46 publications, 2.62%
Chemistry of Materials	Chemistry of Materials, 40, 2.28% Chemistry of Materials 40 publications, 2.28%
Nanotechnology	Nanotechnology, 37, 2.11% Nanotechnology 37 publications, 2.11%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 35, 1.99% Journal of Materials Chemistry A 35 publications, 1.99%
Advanced Functional Materials	Advanced Functional Materials, 32, 1.82% Advanced Functional Materials 32 publications, 1.82%
Journal of the American Chemical Society	Journal of the American Chemical Society, 29, 1.65% Journal of the American Chemical Society 29 publications, 1.65%
RSC Advances	RSC Advances, 29, 1.65% RSC Advances 29 publications, 1.65%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 27, 1.54% Journal of Materials Chemistry C 27 publications, 1.54%
Small	Small, 23, 1.31% Small 23 publications, 1.31%
Journal of Applied Physics	Journal of Applied Physics, 19, 1.08% Journal of Applied Physics 19 publications, 1.08%
Solar Energy Materials and Solar Cells	Solar Energy Materials and Solar Cells, 19, 1.08% Solar Energy Materials and Solar Cells 19 publications, 1.08%
Advanced Optical Materials	Advanced Optical Materials, 17, 0.97% Advanced Optical Materials 17 publications, 0.97%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 15, 0.85% Journal of Alloys and Compounds 15 publications, 0.85%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 15, 0.85% Journal of Physical Chemistry Letters 15 publications, 0.85%
Chemical Communications	Chemical Communications, 14, 0.8% Chemical Communications 14 publications, 0.8%
Langmuir	Langmuir, 13, 0.74% Langmuir 13 publications, 0.74%
CrystEngComm	CrystEngComm, 13, 0.74% CrystEngComm 13 publications, 0.74%
Physical Review B	Physical Review B, 12, 0.68% Physical Review B 12 publications, 0.68%
Nanomaterials	Nanomaterials, 12, 0.68% Nanomaterials 12 publications, 0.68%
Scientific Reports	Scientific Reports, 12, 0.68% Scientific Reports 12 publications, 0.68%
Nano Research	Nano Research, 12, 0.68% Nano Research 12 publications, 0.68%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 12, 0.68% Physical Chemistry Chemical Physics 12 publications, 0.68%
ACS Photonics	ACS Photonics, 11, 0.63% ACS Photonics 11 publications, 0.63%
	10 20 30 40 50 60 70 80

Citations by publishers

	50 100 150 200 250 300 350 400
American Chemical Society (ACS)	American Chemical Society (ACS), 399, 22.72% American Chemical Society (ACS) 399 publications, 22.72%
Elsevier	Elsevier, 291, 16.57% Elsevier 291 publications, 16.57%
Wiley	Wiley, 265, 15.09% Wiley 265 publications, 15.09%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 223, 12.7% Royal Society of Chemistry (RSC) 223 publications, 12.7%
Springer Nature	Springer Nature, 135, 7.69% Springer Nature 135 publications, 7.69%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 79, 4.5% American Institute of Physics (AIP) 79 publications, 4.5%
IOP Publishing	IOP Publishing, 66, 3.76% IOP Publishing 66 publications, 3.76%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 36, 2.05% Multidisciplinary Digital Publishing Institute (MDPI) 36 publications, 2.05%
IEEE	IEEE, 26, 1.48% IEEE 26 publications, 1.48%
Optical Society of America	Optical Society of America, 22, 1.25% Optical Society of America 22 publications, 1.25%
American Physical Society (APS)	American Physical Society (APS), 15, 0.85% American Physical Society (APS) 15 publications, 0.85%
Taylor & Francis	Taylor & Francis, 12, 0.68% Taylor & Francis 12 publications, 0.68%
Trans Tech Publications	Trans Tech Publications, 12, 0.68% Trans Tech Publications 12 publications, 0.68%
Cambridge University Press	Cambridge University Press, 10, 0.57% Cambridge University Press 10 publications, 0.57%
Materials Research Society	Materials Research Society, 9, 0.51% Materials Research Society 9 publications, 0.51%
SPIE	SPIE, 7, 0.4% SPIE 7 publications, 0.4%
Hindawi Limited	Hindawi Limited, 7, 0.4% Hindawi Limited 7 publications, 0.4%
American Vacuum Society	American Vacuum Society, 5, 0.28% American Vacuum Society 5 publications, 0.28%
The Electrochemical Society	The Electrochemical Society, 5, 0.28% The Electrochemical Society 5 publications, 0.28%
Japan Society of Applied Physics	Japan Society of Applied Physics, 5, 0.28% Japan Society of Applied Physics 5 publications, 0.28%
Walter de Gruyter	Walter de Gruyter, 5, 0.28% Walter de Gruyter 5 publications, 0.28%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 5, 0.28% American Association for the Advancement of Science (AAAS) 5 publications, 0.28%
The Chemical Society of Japan	The Chemical Society of Japan, 4, 0.23% The Chemical Society of Japan 4 publications, 0.23%
World Scientific	World Scientific, 4, 0.23% World Scientific 4 publications, 0.23%
Pleiades Publishing	Pleiades Publishing, 4, 0.23% Pleiades Publishing 4 publications, 0.23%
University of Electronic Science and Technology of China	University of Electronic Science and Technology of China, 2, 0.11% University of Electronic Science and Technology of China 2 publications, 0.11%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 2, 0.11% Korean Society of Industrial Engineering Chemistry 2 publications, 0.11%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 2, 0.11% Proceedings of the National Academy of Sciences (PNAS) 2 publications, 0.11%
Chinese Physical Society	Chinese Physical Society, 2, 0.11% Chinese Physical Society 2 publications, 0.11%
	50 100 150 200 250 300 350 400

We do not take into account publications without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

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Mcdonald S. A. et al. Solution-processed PbS quantum dot infrared photodetectors and photovoltaics // Nature Materials. 2005. Vol. 4. No. 2. pp. 138-142.

GOST all authors (up to 50) Copy

Mcdonald S. A., Konstantatos G., Zhang S., Cyr P. W., Klem E. J. D., Levina L., Sargent E. H. Solution-processed PbS quantum dot infrared photodetectors and photovoltaics // Nature Materials. 2005. Vol. 4. No. 2. pp. 138-142.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1038/nmat1299

UR - https://doi.org/10.1038/nmat1299

TI - Solution-processed PbS quantum dot infrared photodetectors and photovoltaics

T2 - Nature Materials

AU - Mcdonald, Steven A

AU - Konstantatos, Gerasimos

AU - Zhang, Shiguo

AU - Cyr, Paul W.

AU - Klem, Ethan J. D.

AU - Levina, Larissa

AU - Sargent, Edward H

PY - 2005

DA - 2005/01/09 00:00:00

PB - Springer Nature

SP - 138-142

IS - 2

VL - 4

SN - 1476-1122

SN - 1476-4660

ER -

BibTex |

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BibTex Copy

@article{2005_Mcdonald,

author = {Steven A Mcdonald and Gerasimos Konstantatos and Shiguo Zhang and Paul W. Cyr and Ethan J. D. Klem and Larissa Levina and Edward H Sargent},

title = {Solution-processed PbS quantum dot infrared photodetectors and photovoltaics},

journal = {Nature Materials},

year = {2005},

volume = {4},

publisher = {Springer Nature},

month = {jan},

url = {https://doi.org/10.1038/nmat1299},

number = {2},

pages = {138--142},

doi = {10.1038/nmat1299}

}

MLA

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MLA Copy

Mcdonald, Steven A., et al. “Solution-processed PbS quantum dot infrared photodetectors and photovoltaics.” Nature Materials, vol. 4, no. 2, Jan. 2005, pp. 138-142. https://doi.org/10.1038/nmat1299.

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Publisher

Springer Nature

Journal

Nature Materials

Quartile SCImago

Quartile WOS

Impact factor

41.2

ISSN

14761122 (Print)
14764660 (Electronic)