Nature Energy, volume 4, issue 10, pages 882-890

All-temperature batteries enabled by fluorinated electrolytes with non-polar solvents

Xiulin Fan ^{1, 2}

Xiao Ji ¹

Long Chen ¹

Ji Chen ¹

Tao Deng ¹

Fudong Han ¹

Jie Yue ¹

Nan Piao ¹

Rui_Xing WANG ³

Xiuquan Zhou ³

X Z Xiao ²

Lixin Chen ²

Chunsheng Wang ^{1, 3}

Hide authors affiliations Show authors affiliations: 3 affiliations

Department of Chemical and Biomolecular Engineering, University of Maryland, College Park, USA |

State Key Laboratory of Silicon Materials and School of Materials Science and Engineering, Zhejiang University, Hangzhou, China |

Department of Chemistry and Biochemistry, University of Maryland, College Park, USA |

Publication type: Journal Article

Publication date: 2019-10-11

Springer Nature

Journal: Nature Energy

Quartile SCImago

Quartile WOS

Impact factor: 56.7

ISSN: 20587546

DOI: 10.1038/s41560-019-0474-3

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Electronic, Optical and Magnetic Materials

Energy Engineering and Power Technology

Fuel Technology

Renewable Energy, Sustainability and the Environment

Abstract

Carbonate electrolytes are commonly used in commercial non-aqueous Li-ion batteries. However, the high affinity between the solvents and the ions and high flammability of the carbonate electrolytes limits the battery operation temperature window to −20 to + 50 °C and the voltage window to 0.0 to 4.3 V. Here, we tame the affinity between solvents and Li ions by dissolving fluorinated electrolytes into highly fluorinated non-polar solvents. In addition to their non-flammable characteristic, our electrolytes enable high electrochemical stability in a wide voltage window of 0.0 to 5.6 V, and high ionic conductivities in a wide temperature range from −125 to + 70 °C. We show that between −95 and + 70 °C, the electrolytes enable LiNi0.8Co0.15Al0.05O2 cathodes to achieve high Coulombic efficiencies of >99.9%, and the aggressive Li anodes and the high-voltage (5.4 V) LiCoMnO4 to achieve Coulombic efficiencies of >99.4% and 99%, respectively. Even at −85 °C, the LiNi0.8Co0.15Al0.05O2 || Li battery can still deliver ~50% of its room-temperature capacity.Batteries generally do not perform well at extreme temperatures, and electrolytes are mainly to blame. Here, the authors dissolve fluorinated electrolytes in highly fluorinated non-polar solvents, enabling batteries that can operate at a wide temperature range (−125 to +70 °C).

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Citations by journals

	5 10 15 20 25 30 35 40 45
Energy Storage Materials	Energy Storage Materials, 41, 6.42% Energy Storage Materials 41 publications, 6.42%
Angewandte Chemie	Angewandte Chemie, 41, 6.42% Angewandte Chemie 41 publications, 6.42%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 40, 6.26% Angewandte Chemie - International Edition 40 publications, 6.26%
Advanced Energy Materials	Advanced Energy Materials, 33, 5.16% Advanced Energy Materials 33 publications, 5.16%
Advanced Functional Materials	Advanced Functional Materials, 29, 4.54% Advanced Functional Materials 29 publications, 4.54%
Advanced Materials	Advanced Materials, 28, 4.38% Advanced Materials 28 publications, 4.38%
Journal of Power Sources	Journal of Power Sources, 23, 3.6% Journal of Power Sources 23 publications, 3.6%
ACS Energy Letters	ACS Energy Letters, 22, 3.44% ACS Energy Letters 22 publications, 3.44%
Nature Communications	Nature Communications, 19, 2.97% Nature Communications 19 publications, 2.97%
Energy and Environmental Science	Energy and Environmental Science, 17, 2.66% Energy and Environmental Science 17 publications, 2.66%
Chemical Engineering Journal	Chemical Engineering Journal, 16, 2.5% Chemical Engineering Journal 16 publications, 2.5%
Small	Small, 15, 2.35% Small 15 publications, 2.35%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 15, 2.35% Journal of Materials Chemistry A 15 publications, 2.35%
ACS applied materials & interfaces	ACS applied materials & interfaces, 14, 2.19% ACS applied materials & interfaces 14 publications, 2.19%
Advanced Science	Advanced Science, 14, 2.19% Advanced Science 14 publications, 2.19%
Journal of the American Chemical Society	Journal of the American Chemical Society, 9, 1.41% Journal of the American Chemical Society 9 publications, 1.41%
Nature Energy	Nature Energy, 9, 1.41% Nature Energy 9 publications, 1.41%
Batteries & Supercaps	Batteries & Supercaps, 9, 1.41% Batteries & Supercaps 9 publications, 1.41%
Nano Research	Nano Research, 8, 1.25% Nano Research 8 publications, 1.25%
ACS Applied Energy Materials	ACS Applied Energy Materials, 8, 1.25% ACS Applied Energy Materials 8 publications, 1.25%
ACS Nano	ACS Nano, 8, 1.25% ACS Nano 8 publications, 1.25%
Nano Energy	Nano Energy, 7, 1.1% Nano Energy 7 publications, 1.1%
Cell Reports Physical Science	Cell Reports Physical Science, 7, 1.1% Cell Reports Physical Science 7 publications, 1.1%
Energy & Environmental Materials	Energy & Environmental Materials, 7, 1.1% Energy & Environmental Materials 7 publications, 1.1%
Nano Letters	Nano Letters, 6, 0.94% Nano Letters 6 publications, 0.94%
Journal of Energy Chemistry	Journal of Energy Chemistry, 6, 0.94% Journal of Energy Chemistry 6 publications, 0.94%
Chemical Communications	Chemical Communications, 6, 0.94% Chemical Communications 6 publications, 0.94%
Proceedings of the National Academy of Sciences of the United States of America	Proceedings of the National Academy of Sciences of the United States of America, 6, 0.94% Proceedings of the National Academy of Sciences of the United States of America 6 publications, 0.94%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 5, 0.78% Journal of the Electrochemical Society 5 publications, 0.78%
Joule	Joule, 4, 0.63% Joule 4 publications, 0.63%
	5 10 15 20 25 30 35 40 45

Citations by publishers

	50 100 150 200 250
Wiley	Wiley, 246, 38.5% Wiley 246 publications, 38.5%
Elsevier	Elsevier, 152, 23.79% Elsevier 152 publications, 23.79%
American Chemical Society (ACS)	American Chemical Society (ACS), 94, 14.71% American Chemical Society (ACS) 94 publications, 14.71%
Springer Nature	Springer Nature, 59, 9.23% Springer Nature 59 publications, 9.23%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 54, 8.45% Royal Society of Chemistry (RSC) 54 publications, 8.45%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 6, 0.94% Proceedings of the National Academy of Sciences (PNAS) 6 publications, 0.94%
The Electrochemical Society	The Electrochemical Society, 5, 0.78% The Electrochemical Society 5 publications, 0.78%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 3, 0.47% Multidisciplinary Digital Publishing Institute (MDPI) 3 publications, 0.47%
OAE Publishing Inc.	OAE Publishing Inc., 3, 0.47% OAE Publishing Inc. 3 publications, 0.47%
Frontiers Media S.A.	Frontiers Media S.A., 2, 0.31% Frontiers Media S.A. 2 publications, 0.31%
IOP Publishing	IOP Publishing, 2, 0.31% IOP Publishing 2 publications, 0.31%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 2, 0.31% American Association for the Advancement of Science (AAAS) 2 publications, 0.31%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 1, 0.16% American Institute of Physics (AIP) 1 publication, 0.16%
Cambridge University Press	Cambridge University Press, 1, 0.16% Cambridge University Press 1 publication, 0.16%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 1, 0.16% Nonferrous Metals Society of China 1 publication, 0.16%
Higher Education Press	Higher Education Press, 1, 0.16% Higher Education Press 1 publication, 0.16%
KeAi Communications Co.	KeAi Communications Co., 1, 0.16% KeAi Communications Co. 1 publication, 0.16%
IEEE	IEEE, 1, 0.16% IEEE 1 publication, 0.16%
Chinese Physical Society	Chinese Physical Society, 1, 0.16% Chinese Physical Society 1 publication, 0.16%
Saratov State University	Saratov State University, 1, 0.16% Saratov State University 1 publication, 0.16%
Research Square Platform LLC	Research Square Platform LLC, 1, 0.16% Research Square Platform LLC 1 publication, 0.16%
Social Science Electronic Publishing	Social Science Electronic Publishing, 1, 0.16% Social Science Electronic Publishing 1 publication, 0.16%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.16% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.16%
	50 100 150 200 250

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Fan X. et al. All-temperature batteries enabled by fluorinated electrolytes with non-polar solvents // Nature Energy. 2019. Vol. 4. No. 10. pp. 882-890.

GOST all authors (up to 50) Copy

Fan X., Ji X., Chen L., Chen J., Deng T., Han F., Yue J., Piao N., WANG R., Zhou X., Xiao X. Z., Chen L., Wang C. All-temperature batteries enabled by fluorinated electrolytes with non-polar solvents // Nature Energy. 2019. Vol. 4. No. 10. pp. 882-890.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1038/s41560-019-0474-3

UR - https://doi.org/10.1038/s41560-019-0474-3

TI - All-temperature batteries enabled by fluorinated electrolytes with non-polar solvents

T2 - Nature Energy

AU - Fan, Xiulin

AU - Ji, Xiao

AU - Chen, Long

AU - Chen, Ji

AU - Deng, Tao

AU - Han, Fudong

AU - Yue, Jie

AU - Piao, Nan

AU - WANG, Rui_Xing

AU - Zhou, Xiuquan

AU - Xiao, X Z

AU - Chen, Lixin

AU - Wang, Chunsheng

PY - 2019

DA - 2019/10/11 00:00:00

PB - Springer Nature

SP - 882-890

IS - 10

VL - 4

SN - 2058-7546

ER -

BibTex |

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@article{2019_Fan,

author = {Xiulin Fan and Xiao Ji and Long Chen and Ji Chen and Tao Deng and Fudong Han and Jie Yue and Nan Piao and Rui_Xing WANG and Xiuquan Zhou and X Z Xiao and Lixin Chen and Chunsheng Wang},

title = {All-temperature batteries enabled by fluorinated electrolytes with non-polar solvents},

journal = {Nature Energy},

year = {2019},

volume = {4},

publisher = {Springer Nature},

month = {oct},

url = {https://doi.org/10.1038/s41560-019-0474-3},

number = {10},

pages = {882--890},

doi = {10.1038/s41560-019-0474-3}

}

MLA

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MLA Copy

Fan, Xiulin, et al. “All-temperature batteries enabled by fluorinated electrolytes with non-polar solvents.” Nature Energy, vol. 4, no. 10, Oct. 2019, pp. 882-890. https://doi.org/10.1038/s41560-019-0474-3.

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Publisher

Springer Nature

Journal

Nature Energy

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Quartile WOS

Impact factor

56.7

ISSN

20587546 (Electronic)