Nature Energy, volume 5, issue 7, pages 534-542

Low-temperature and high-rate-charging lithium metal batteries enabled by an electrochemically active monolayer-regulated interface

Yue Gao ¹

Tomas Rojas ^{2, 3}

Ke Wang ⁴

Shuai Liu ¹

Daiwei Wang ¹

Tianhang Chen ¹

Haiying Wang ⁴

Anh T. Ngo ^{2, 5}

Donghai Wang ¹

Hide authors affiliations Show authors affiliations: 5 affiliations

Department of Mechanical Engineering, The Pennsylvania State University, University Park, USA |

Materials Science Division, Argonne National laboratory, Lemont, USA |

Nanoscale and Quantum Phenomena Institute and the Department of Physics and Astronomy, Ohio University, Athens, USA |

⁴

Materials Research Institute, the Pennsylvania State University, University Park, USA |

⁵

Department of Chemical Engineering, University of Illinois at Chicago, Chicago, USA |

Publication type: Journal Article

Publication date: 2020-06-22

Springer Nature

Journal: Nature Energy

Quartile SCImago

Quartile WOS

Impact factor: 56.7

ISSN: 20587546

DOI: 10.1038/s41560-020-0640-7

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Electronic, Optical and Magnetic Materials

Energy Engineering and Power Technology

Fuel Technology

Renewable Energy, Sustainability and the Environment

Abstract

Stable operation of rechargeable lithium-based batteries at low temperatures is important for cold-climate applications, but is plagued by dendritic Li plating and unstable solid–electrolyte interphase (SEI). Here, we report on high-performance Li metal batteries under low-temperature and high-rate-charging conditions. The high performance is achieved by using a self-assembled monolayer of electrochemically active molecules on current collectors that regulates the nanostructure and composition of the SEI and deposition morphology of Li metal anodes. A multilayer SEI that contains a lithium fluoride-rich inner phase and amorphous outer layer effectively seals the Li surface, in contrast to the conventional SEI, which is non-passive at low temperatures. Consequently, galvanic Li corrosion and self-discharge are suppressed, stable Li deposition is achieved from −60 °C to 45 °C, and a Li | LiCoO2 cell with a capacity of 2.0 mAh cm−2 displays a 200-cycle life at −15 °C with a recharge time of 45 min. In addition to high energy, batteries need to possess high power and to be able to operate in all climates. Here, the authors present an electrochemically active monolayer-coated current collector that is used to produce high-performance Li metal batteries under low-temperature and high-rate-charging conditions.

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Citations by journals

	5 10 15 20 25
Advanced Energy Materials	Advanced Energy Materials, 24, 7.59% Advanced Energy Materials 24 publications, 7.59%
Energy Storage Materials	Energy Storage Materials, 22, 6.96% Energy Storage Materials 22 publications, 6.96%
Angewandte Chemie	Angewandte Chemie, 15, 4.75% Angewandte Chemie 15 publications, 4.75%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 15, 4.75% Angewandte Chemie - International Edition 15 publications, 4.75%
Advanced Materials	Advanced Materials, 15, 4.75% Advanced Materials 15 publications, 4.75%
Advanced Functional Materials	Advanced Functional Materials, 13, 4.11% Advanced Functional Materials 13 publications, 4.11%
ACS applied materials & interfaces	ACS applied materials & interfaces, 13, 4.11% ACS applied materials & interfaces 13 publications, 4.11%
Small	Small, 10, 3.16% Small 10 publications, 3.16%
Chemical Engineering Journal	Chemical Engineering Journal, 8, 2.53% Chemical Engineering Journal 8 publications, 2.53%
ACS Nano	ACS Nano, 7, 2.22% ACS Nano 7 publications, 2.22%
Nature Communications	Nature Communications, 6, 1.9% Nature Communications 6 publications, 1.9%
Nano Energy	Nano Energy, 6, 1.9% Nano Energy 6 publications, 1.9%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 6, 1.9% Journal of Materials Chemistry A 6 publications, 1.9%
Journal of Energy Chemistry	Journal of Energy Chemistry, 6, 1.9% Journal of Energy Chemistry 6 publications, 1.9%
ACS Energy Letters	ACS Energy Letters, 5, 1.58% ACS Energy Letters 5 publications, 1.58%
Nature Energy	Nature Energy, 5, 1.58% Nature Energy 5 publications, 1.58%
ACS Applied Energy Materials	ACS Applied Energy Materials, 5, 1.58% ACS Applied Energy Materials 5 publications, 1.58%
Journal of Power Sources	Journal of Power Sources, 4, 1.27% Journal of Power Sources 4 publications, 1.27%
Advanced Science	Advanced Science, 4, 1.27% Advanced Science 4 publications, 1.27%
Nano-Micro Letters	Nano-Micro Letters, 4, 1.27% Nano-Micro Letters 4 publications, 1.27%
Electrochimica Acta	Electrochimica Acta, 4, 1.27% Electrochimica Acta 4 publications, 1.27%
Science advances	Science advances, 4, 1.27% Science advances 4 publications, 1.27%
Energy and Environmental Science	Energy and Environmental Science, 4, 1.27% Energy and Environmental Science 4 publications, 1.27%
Cell Reports Physical Science	Cell Reports Physical Science, 3, 0.95% Cell Reports Physical Science 3 publications, 0.95%
InfoMat	InfoMat, 3, 0.95% InfoMat 3 publications, 0.95%
Small Science	Small Science, 3, 0.95% Small Science 3 publications, 0.95%
Batteries & Supercaps	Batteries & Supercaps, 3, 0.95% Batteries & Supercaps 3 publications, 0.95%
Journal of the American Chemical Society	Journal of the American Chemical Society, 3, 0.95% Journal of the American Chemical Society 3 publications, 0.95%
Materials Chemistry Frontiers	Materials Chemistry Frontiers, 3, 0.95% Materials Chemistry Frontiers 3 publications, 0.95%
	5 10 15 20 25

Citations by publishers

	20 40 60 80 100 120 140
Wiley	Wiley, 121, 38.29% Wiley 121 publications, 38.29%
Elsevier	Elsevier, 77, 24.37% Elsevier 77 publications, 24.37%
American Chemical Society (ACS)	American Chemical Society (ACS), 46, 14.56% American Chemical Society (ACS) 46 publications, 14.56%
Springer Nature	Springer Nature, 24, 7.59% Springer Nature 24 publications, 7.59%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 23, 7.28% Royal Society of Chemistry (RSC) 23 publications, 7.28%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 5, 1.58% American Association for the Advancement of Science (AAAS) 5 publications, 1.58%
Frontiers Media S.A.	Frontiers Media S.A., 3, 0.95% Frontiers Media S.A. 3 publications, 0.95%
IEEE	IEEE, 3, 0.95% IEEE 3 publications, 0.95%
The Electrochemical Society	The Electrochemical Society, 2, 0.63% The Electrochemical Society 2 publications, 0.63%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 0.63% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 0.63%
OAE Publishing Inc.	OAE Publishing Inc., 2, 0.63% OAE Publishing Inc. 2 publications, 0.63%
Hans Publishers	Hans Publishers, 1, 0.32% Hans Publishers 1 publication, 0.32%
Saratov State University	Saratov State University, 1, 0.32% Saratov State University 1 publication, 0.32%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 1, 0.32% Proceedings of the National Academy of Sciences (PNAS) 1 publication, 0.32%
IOP Publishing	IOP Publishing, 1, 0.32% IOP Publishing 1 publication, 0.32%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.32% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.32%
	20 40 60 80 100 120 140

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Gao Y. et al. Low-temperature and high-rate-charging lithium metal batteries enabled by an electrochemically active monolayer-regulated interface // Nature Energy. 2020. Vol. 5. No. 7. pp. 534-542.

GOST all authors (up to 50) Copy

Gao Y., Rojas T., Wang K., Liu S., Wang D., Chen T., Wang H., Ngo A. T., Wang D. Low-temperature and high-rate-charging lithium metal batteries enabled by an electrochemically active monolayer-regulated interface // Nature Energy. 2020. Vol. 5. No. 7. pp. 534-542.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1038/s41560-020-0640-7

UR - https://www.nature.com/articles/s41560-020-0640-7

TI - Low-temperature and high-rate-charging lithium metal batteries enabled by an electrochemically active monolayer-regulated interface

T2 - Nature Energy

AU - Gao, Yue

AU - Rojas, Tomas

AU - Wang, Ke

AU - Liu, Shuai

AU - Wang, Daiwei

AU - Chen, Tianhang

AU - Wang, Haiying

AU - Ngo, Anh T.

AU - Wang, Donghai

PY - 2020

DA - 2020/06/22 00:00:00

PB - Springer Nature

SP - 534-542

IS - 7

VL - 5

SN - 2058-7546

ER -

BibTex |

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BibTex Copy

@article{2020_Gao,

author = {Yue Gao and Tomas Rojas and Ke Wang and Shuai Liu and Daiwei Wang and Tianhang Chen and Haiying Wang and Anh T. Ngo and Donghai Wang},

title = {Low-temperature and high-rate-charging lithium metal batteries enabled by an electrochemically active monolayer-regulated interface},

journal = {Nature Energy},

year = {2020},

volume = {5},

publisher = {Springer Nature},

month = {jun},

url = {https://www.nature.com/articles/s41560-020-0640-7},

number = {7},

pages = {534--542},

doi = {10.1038/s41560-020-0640-7}

}

MLA

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Gao, Yue, et al. “Low-temperature and high-rate-charging lithium metal batteries enabled by an electrochemically active monolayer-regulated interface.” Nature Energy, vol. 5, no. 7, Jun. 2020, pp. 534-542. https://www.nature.com/articles/s41560-020-0640-7.

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Publisher

Springer Nature

Journal

Nature Energy

Quartile SCImago

Quartile WOS

Impact factor

56.7

ISSN

20587546 (Electronic)