Nature Energy, volume 6, issue 10, pages 987-994

Pressure-tailored lithium deposition and dissolution in lithium metal batteries

Chengcheng Fang ^{1, 2}

Bingyu Lu ¹

Gorakh M. Pawar ³

Minghao Zhang ¹

Diyi Cheng ¹

Shuru Chen ⁴

Miguel Ceja ¹

Jean-Marie Doux ¹

Henry Musrock ²

Mei Cai ⁴

Bor Yann Liaw ³

Ying Meng ¹

Hide authors affiliations Show authors affiliations: 4 affiliations

Department of NanoEngineering, University of California San Diego, La Jolla, USA |

Department of Chemical Engineering and Materials Science, Michigan State University, East Lansing, USA |

Energy and Environmental Science and Technology Directorate, Idaho National Laboratory, Idaho Falls, USA |

⁴

General Motors Research and Development Center, Warren, USA |

Publication type: Journal Article

Publication date: 2021-10-19

Springer Nature

Journal: Nature Energy

Quartile SCImago

Quartile WOS

Impact factor: 56.7

ISSN: 20587546

DOI: 10.1038/s41560-021-00917-3

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Electronic, Optical and Magnetic Materials

Energy Engineering and Power Technology

Fuel Technology

Renewable Energy, Sustainability and the Environment

Abstract

Unregulated lithium (Li) growth is the major cause of low Coulombic efficiency, short cycle life and safety hazards for rechargeable Li metal batteries. Strategies that aim to achieve large granular Li deposits have been extensively explored, and yet it remains a challenge to achieve the ideal Li deposits, which consist of large Li particles that are seamlessly packed on the electrode and can be reversibly deposited and stripped. Here we report a dense Li deposition (99.49% electrode density) with an ideal columnar structure that is achieved by controlling the uniaxial stack pressure during battery operation. Using multiscale characterization and simulation, we elucidate the critical role of stack pressure on Li nucleation, growth and dissolution processes and propose a Li-reservoir-testing protocol to maintain the ideal Li morphology during extended cycling. The precise manipulation of Li deposition and dissolution is a critical step to enable fast charging and a low-temperature operation for Li metal batteries. Li electrodeposition is a fundamental process in Li metal batteries and its reversibility is crucial for battery operation. The authors investigate the effects of stack pressure on Li deposition and associated processes and discuss strategies for achieving dense Li deposits and practical Li metal batteries.

By date By citations

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Citations by journals

	5 10 15 20 25
Advanced Energy Materials	Advanced Energy Materials, 21, 8.5% Advanced Energy Materials 21 publications, 8.5%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 14, 5.67% Journal of the Electrochemical Society 14 publications, 5.67%
Advanced Functional Materials	Advanced Functional Materials, 12, 4.86% Advanced Functional Materials 12 publications, 4.86%
Advanced Materials	Advanced Materials, 11, 4.45% Advanced Materials 11 publications, 4.45%
ACS Energy Letters	ACS Energy Letters, 11, 4.45% ACS Energy Letters 11 publications, 4.45%
ACS applied materials & interfaces	ACS applied materials & interfaces, 10, 4.05% ACS applied materials & interfaces 10 publications, 4.05%
Energy Storage Materials	Energy Storage Materials, 10, 4.05% Energy Storage Materials 10 publications, 4.05%
Small	Small, 7, 2.83% Small 7 publications, 2.83%
Angewandte Chemie	Angewandte Chemie, 7, 2.83% Angewandte Chemie 7 publications, 2.83%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 7, 2.83% Angewandte Chemie - International Edition 7 publications, 2.83%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 7, 2.83% Journal of Materials Chemistry A 7 publications, 2.83%
ACS Nano	ACS Nano, 6, 2.43% ACS Nano 6 publications, 2.43%
Energy and Environmental Science	Energy and Environmental Science, 6, 2.43% Energy and Environmental Science 6 publications, 2.43%
Nature Energy	Nature Energy, 6, 2.43% Nature Energy 6 publications, 2.43%
Nature Communications	Nature Communications, 6, 2.43% Nature Communications 6 publications, 2.43%
Journal of Energy Storage	Journal of Energy Storage, 5, 2.02% Journal of Energy Storage 5 publications, 2.02%
Advanced Science	Advanced Science, 4, 1.62% Advanced Science 4 publications, 1.62%
Journal of Power Sources	Journal of Power Sources, 4, 1.62% Journal of Power Sources 4 publications, 1.62%
ACS Applied Energy Materials	ACS Applied Energy Materials, 4, 1.62% ACS Applied Energy Materials 4 publications, 1.62%
Small Structures	Small Structures, 3, 1.21% Small Structures 3 publications, 1.21%
Cell Reports Physical Science	Cell Reports Physical Science, 3, 1.21% Cell Reports Physical Science 3 publications, 1.21%
eScience	eScience, 3, 1.21% eScience 3 publications, 1.21%
Nano Energy	Nano Energy, 3, 1.21% Nano Energy 3 publications, 1.21%
Joule	Joule, 3, 1.21% Joule 3 publications, 1.21%
Journal of the American Chemical Society	Journal of the American Chemical Society, 2, 0.81% Journal of the American Chemical Society 2 publications, 0.81%
Rare Metals	Rare Metals, 2, 0.81% Rare Metals 2 publications, 0.81%
Matter	Matter, 2, 0.81% Matter 2 publications, 0.81%
Materials Today Energy	Materials Today Energy, 2, 0.81% Materials Today Energy 2 publications, 0.81%
Electrochimica Acta	Electrochimica Acta, 2, 0.81% Electrochimica Acta 2 publications, 0.81%
Journal of Energy Chemistry	Journal of Energy Chemistry, 2, 0.81% Journal of Energy Chemistry 2 publications, 0.81%
	5 10 15 20 25

Citations by publishers

	10 20 30 40 50 60 70 80 90
Wiley	Wiley, 85, 34.41% Wiley 85 publications, 34.41%
Elsevier	Elsevier, 59, 23.89% Elsevier 59 publications, 23.89%
American Chemical Society (ACS)	American Chemical Society (ACS), 38, 15.38% American Chemical Society (ACS) 38 publications, 15.38%
Springer Nature	Springer Nature, 23, 9.31% Springer Nature 23 publications, 9.31%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 15, 6.07% Royal Society of Chemistry (RSC) 15 publications, 6.07%
The Electrochemical Society	The Electrochemical Society, 14, 5.67% The Electrochemical Society 14 publications, 5.67%
Frontiers Media S.A.	Frontiers Media S.A., 2, 0.81% Frontiers Media S.A. 2 publications, 0.81%
The Electrochemical Society of Japan	The Electrochemical Society of Japan, 2, 0.81% The Electrochemical Society of Japan 2 publications, 0.81%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.4% American Association for the Advancement of Science (AAAS) 1 publication, 0.4%
IEEE	IEEE, 1, 0.4% IEEE 1 publication, 0.4%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 1, 0.4% Nonferrous Metals Society of China 1 publication, 0.4%
ASME	ASME, 1, 0.4% ASME 1 publication, 0.4%
Oxford University Press	Oxford University Press, 1, 0.4% Oxford University Press 1 publication, 0.4%
OAE Publishing Inc.	OAE Publishing Inc., 1, 0.4% OAE Publishing Inc. 1 publication, 0.4%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 1, 0.4% Proceedings of the National Academy of Sciences (PNAS) 1 publication, 0.4%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.4% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.4%
	10 20 30 40 50 60 70 80 90

We do not take into account publications without a DOI.
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Fang C. et al. Pressure-tailored lithium deposition and dissolution in lithium metal batteries // Nature Energy. 2021. Vol. 6. No. 10. pp. 987-994.

GOST all authors (up to 50) Copy

Fang C., Lu B., Pawar G. M., Zhang M., Cheng D., Chen S., Ceja M., Doux J., Musrock H., Cai M., Liaw B. Y., Meng Y. Pressure-tailored lithium deposition and dissolution in lithium metal batteries // Nature Energy. 2021. Vol. 6. No. 10. pp. 987-994.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1038/s41560-021-00917-3

UR - https://doi.org/10.1038/s41560-021-00917-3

TI - Pressure-tailored lithium deposition and dissolution in lithium metal batteries

T2 - Nature Energy

AU - Fang, Chengcheng

AU - Lu, Bingyu

AU - Pawar, Gorakh M.

AU - Zhang, Minghao

AU - Cheng, Diyi

AU - Chen, Shuru

AU - Ceja, Miguel

AU - Doux, Jean-Marie

AU - Musrock, Henry

AU - Cai, Mei

AU - Liaw, Bor Yann

AU - Meng, Ying

PY - 2021

DA - 2021/10/19 00:00:00

PB - Springer Nature

SP - 987-994

IS - 10

VL - 6

SN - 2058-7546

ER -

BibTex |

Cite this

BibTex Copy

@article{2021_Fang,

author = {Chengcheng Fang and Bingyu Lu and Gorakh M. Pawar and Minghao Zhang and Diyi Cheng and Shuru Chen and Miguel Ceja and Jean-Marie Doux and Henry Musrock and Mei Cai and Bor Yann Liaw and Ying Meng},

title = {Pressure-tailored lithium deposition and dissolution in lithium metal batteries},

journal = {Nature Energy},

year = {2021},

volume = {6},

publisher = {Springer Nature},

month = {oct},

url = {https://doi.org/10.1038/s41560-021-00917-3},

number = {10},

pages = {987--994},

doi = {10.1038/s41560-021-00917-3}

}

MLA

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MLA Copy

Fang, Chengcheng, et al. “Pressure-tailored lithium deposition and dissolution in lithium metal batteries.” Nature Energy, vol. 6, no. 10, Oct. 2021, pp. 987-994. https://doi.org/10.1038/s41560-021-00917-3.

Found error?

Publisher

Springer Nature

Journal

Nature Energy

Quartile SCImago

Quartile WOS

Impact factor

56.7

ISSN

20587546 (Electronic)