Nature Reviews Chemistry, volume 4, issue 10, pages 508-527

Chemistry under high pressure

Maosheng Miao ¹

Yuan-Hui Sun ¹

Eva D. Zurek ²

Haiqing Lin ^{3, 4}

Hide authors affiliations Show authors affiliations: 4 affiliations

Department of Chemistry and Biochemistry, California State University, Northridge, Northridge, USA |

Department of Chemistry, State University of New York at Buffalo, Buffalo, USA |

Beijing Computational Science Research Center, Beijing, China |

⁴

Department of physics, Beijing Normal University, Beijing, China |

Publication type: Journal Article

Publication date: 2020-09-14

Springer Nature

Journal: Nature Reviews Chemistry

Quartile SCImago

Quartile WOS

Impact factor: 36.3

ISSN: 23973358

DOI: 10.1038/s41570-020-0213-0

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General Chemistry

General Chemical Engineering

Abstract

Thanks to the development of experimental high-pressure techniques and methods for crystal-structure prediction based on quantum mechanics, in the past decade, numerous new compounds, mostly binary, with atypical compositions have been predicted, and some have been synthesized. Differing from conventional solid-state materials, many of these new compounds are comprised of various homonuclear chemical species, such as dimers, trimers, pentagonal and heptagonal rings, polymeric chains, atomic layers and 3D networks. Strikingly, it has been shown that pressure can alter the chemistry of an element by activating its (semi)core electrons, unoccupied orbitals and even the non-atom-centred quantum orbitals located on the interstitial sites, leading to many new surprising phenomena. This Review provides a summary of atypical compounds that result from the effects of high pressure on either the chemical bonds or the local orbitals. We describe various unusual chemical species and motifs, show how the chemical properties of the elements are altered under pressure and illustrate how compound formation is favoured even in situations in which chemical bonds are not formed. An extraordinary new picture of chemistry emerges as we piece together these unexpected high-pressure phenomena. In marked contrast to the previously held beliefs regarding the behaviour of solids under pressure, we are learning that the quantum-mechanical features of electrons, such as those that lead to the formation of directional bonds, inhomogeneous distributions of electrons and atoms, as well as variations in symmetry, might be magnified under pressure. We discuss the influence of these phenomena on future studies that will probe chemistry at higher pressures and explore more complex chemical compositions than those that have been studied to date. High pressure leads to striking new chemistry. Many new compounds with atypical compositions and a plethora of novel chemical species can be stabilized by the formation of homonuclear bonds and the activation of core electrons, non-valence and non-atomic orbitals.

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	2 4 6 8 10 12
Physical Review B	Physical Review B, 12, 8.57% Physical Review B 12 publications, 8.57%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 9, 6.43% Physical Chemistry Chemical Physics 9 publications, 6.43%
Journal of Physics Condensed Matter	Journal of Physics Condensed Matter, 8, 5.71% Journal of Physics Condensed Matter 8 publications, 5.71%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 8, 5.71% Journal of Physical Chemistry C 8 publications, 5.71%
Journal of Chemical Physics	Journal of Chemical Physics, 6, 4.29% Journal of Chemical Physics 6 publications, 4.29%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 6, 4.29% Journal of Physical Chemistry Letters 6 publications, 4.29%
Angewandte Chemie	Angewandte Chemie, 5, 3.57% Angewandte Chemie 5 publications, 3.57%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 5, 3.57% Angewandte Chemie - International Edition 5 publications, 3.57%
Inorganic Chemistry	Inorganic Chemistry, 5, 3.57% Inorganic Chemistry 5 publications, 3.57%
Journal of the American Chemical Society	Journal of the American Chemical Society, 4, 2.86% Journal of the American Chemical Society 4 publications, 2.86%
Journal of Applied Physics	Journal of Applied Physics, 3, 2.14% Journal of Applied Physics 3 publications, 2.14%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 3, 2.14% Journal of Alloys and Compounds 3 publications, 2.14%
Chinese Physics B	Chinese Physics B, 3, 2.14% Chinese Physics B 3 publications, 2.14%
APL Materials	APL Materials, 2, 1.43% APL Materials 2 publications, 1.43%
Physical Review Materials	Physical Review Materials, 2, 1.43% Physical Review Materials 2 publications, 1.43%
Physical Review Letters	Physical Review Letters, 2, 1.43% Physical Review Letters 2 publications, 1.43%
Nature Communications	Nature Communications, 2, 1.43% Nature Communications 2 publications, 1.43%
Wiley Interdisciplinary Reviews: Computational Molecular Science	Wiley Interdisciplinary Reviews: Computational Molecular Science, 2, 1.43% Wiley Interdisciplinary Reviews: Computational Molecular Science 2 publications, 1.43%
JACS Au	JACS Au, 2, 1.43% JACS Au 2 publications, 1.43%
Chemical Science	Chemical Science, 2, 1.43% Chemical Science 2 publications, 1.43%
Chemistry of Materials	Chemistry of Materials, 2, 1.43% Chemistry of Materials 2 publications, 1.43%
Physical Review Research	Physical Review Research, 2, 1.43% Physical Review Research 2 publications, 1.43%
Review of Scientific Instruments	Review of Scientific Instruments, 1, 0.71% Review of Scientific Instruments 1 publication, 0.71%
Matter and Radiation at Extremes	Matter and Radiation at Extremes, 1, 0.71% Matter and Radiation at Extremes 1 publication, 0.71%
Journal of Manufacturing and Materials Processing	Journal of Manufacturing and Materials Processing, 1, 0.71% Journal of Manufacturing and Materials Processing 1 publication, 0.71%
Molecules	Molecules, 1, 0.71% Molecules 1 publication, 0.71%
Applied Sciences (Switzerland)	Applied Sciences (Switzerland), 1, 0.71% Applied Sciences (Switzerland) 1 publication, 0.71%
Frontiers in Chemistry	Frontiers in Chemistry, 1, 0.71% Frontiers in Chemistry 1 publication, 0.71%
Communications Chemistry	Communications Chemistry, 1, 0.71% Communications Chemistry 1 publication, 0.71%
	2 4 6 8 10 12

Citations by publishers

	5 10 15 20 25 30 35
American Chemical Society (ACS)	American Chemical Society (ACS), 34, 24.29% American Chemical Society (ACS) 34 publications, 24.29%
Wiley	Wiley, 19, 13.57% Wiley 19 publications, 13.57%
American Physical Society (APS)	American Physical Society (APS), 18, 12.86% American Physical Society (APS) 18 publications, 12.86%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 13, 9.29% American Institute of Physics (AIP) 13 publications, 9.29%
Elsevier	Elsevier, 13, 9.29% Elsevier 13 publications, 9.29%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 13, 9.29% Royal Society of Chemistry (RSC) 13 publications, 9.29%
IOP Publishing	IOP Publishing, 12, 8.57% IOP Publishing 12 publications, 8.57%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 5, 3.57% Multidisciplinary Digital Publishing Institute (MDPI) 5 publications, 3.57%
Springer Nature	Springer Nature, 5, 3.57% Springer Nature 5 publications, 3.57%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 2, 1.43% American Association for the Advancement of Science (AAAS) 2 publications, 1.43%
Frontiers Media S.A.	Frontiers Media S.A., 1, 0.71% Frontiers Media S.A. 1 publication, 0.71%
King Saud University	King Saud University, 1, 0.71% King Saud University 1 publication, 0.71%
Walter de Gruyter	Walter de Gruyter, 1, 0.71% Walter de Gruyter 1 publication, 0.71%
Taylor & Francis	Taylor & Francis, 1, 0.71% Taylor & Francis 1 publication, 0.71%
Chinese Physical Society	Chinese Physical Society, 1, 0.71% Chinese Physical Society 1 publication, 0.71%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.71% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.71%
	5 10 15 20 25 30 35

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Miao M. et al. Chemistry under high pressure // Nature Reviews Chemistry. 2020. Vol. 4. No. 10. pp. 508-527.

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Miao M., Sun Y., Zurek E. D., Lin H. Chemistry under high pressure // Nature Reviews Chemistry. 2020. Vol. 4. No. 10. pp. 508-527.

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TY - JOUR

DO - 10.1038/s41570-020-0213-0

UR - https://doi.org/10.1038/s41570-020-0213-0

TI - Chemistry under high pressure

T2 - Nature Reviews Chemistry

AU - Miao, Maosheng

AU - Sun, Yuan-Hui

AU - Zurek, Eva D.

AU - Lin, Haiqing

PY - 2020

DA - 2020/09/14 00:00:00

PB - Springer Nature

SP - 508-527

IS - 10

VL - 4

SN - 2397-3358

ER -

BibTex |

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@article{2020_Miao,

author = {Maosheng Miao and Yuan-Hui Sun and Eva D. Zurek and Haiqing Lin},

title = {Chemistry under high pressure},

journal = {Nature Reviews Chemistry},

year = {2020},

volume = {4},

publisher = {Springer Nature},

month = {sep},

url = {https://doi.org/10.1038/s41570-020-0213-0},

number = {10},

pages = {508--527},

doi = {10.1038/s41570-020-0213-0}

}

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Miao, Maosheng, et al. “Chemistry under high pressure.” Nature Reviews Chemistry, vol. 4, no. 10, Sep. 2020, pp. 508-527. https://doi.org/10.1038/s41570-020-0213-0.

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Nature Reviews Chemistry

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23973358 (Electronic)