Nature, volume 597, issue 7875, pages 214-219
Tunable self-assembled Casimir microcavities and polaritons
Publication type: Journal Article
Publication date: 2021-09-08
Multidisciplinary
Abstract
Spontaneous formation of ordered structures—self-assembly—is ubiquitous in nature and observed on different length scales, ranging from atomic and molecular systems to micrometre-scale objects and living matter1. Self-ordering in molecular and biological systems typically involves short-range hydrophobic and van der Waals interactions2,3. Here we introduce an approach to micrometre-scale self-assembly based on the joint action of attractive Casimir and repulsive electrostatic forces arising between charged metallic nanoflakes in an aqueous solution. This system forms a self-assembled optical Fabry–Pérot microcavity with a fundamental mode in the visible range (long-range separation distance about 100–200 nanometres) and a tunable equilibrium configuration. Furthermore, by placing an excitonic material in the microcavity region, we are able to realize hybrid light–matter states (polaritons4–6), whose properties, such as coupling strength and eigenstate composition, can be controlled in real time by the concentration of ligand molecules in the solution and light pressure. These Casimir microcavities could find future use as sensitive and tunable platforms for a variety of applications, including opto-mechanics7, nanomachinery8 and cavity-induced polaritonic chemistry9. Gold nanoflake pairs form by self-assembly in an aqueous ligand solution and offer stable and tunable microcavities by virtue of equilibrium between attractive Casimir forces and repulsive electrostatic forces.
Citations by journals
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Nature Communications
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Nature Communications
4 publications, 8.51%
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ACS Nano
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ACS Nano
3 publications, 6.38%
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Nature Physics
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Nature Physics
2 publications, 4.26%
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Nature
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Nature
2 publications, 4.26%
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Chemical Reviews
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Chemical Reviews
2 publications, 4.26%
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Nano Letters
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Nano Letters
2 publications, 4.26%
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Journal of Physical Chemistry Letters
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Journal of Physical Chemistry Letters
2 publications, 4.26%
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Physical Review A
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Physical Review A
2 publications, 4.26%
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Journal of Chemical Physics
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Journal of Chemical Physics
1 publication, 2.13%
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European Physical Journal: Special Topics
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European Physical Journal: Special Topics
1 publication, 2.13%
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Physics
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Physics
1 publication, 2.13%
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Separation and Purification Technology
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Separation and Purification Technology
1 publication, 2.13%
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Optik
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Optik
1 publication, 2.13%
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Physics Letters, Section A: General, Atomic and Solid State Physics
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Physics Letters, Section A: General, Atomic and Solid State Physics
1 publication, 2.13%
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Journal of Quantitative Spectroscopy and Radiative Transfer
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Journal of Quantitative Spectroscopy and Radiative Transfer
1 publication, 2.13%
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Physics Reports
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Physics Reports
1 publication, 2.13%
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Journal of Optics (United Kingdom)
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Journal of Optics (United Kingdom)
1 publication, 2.13%
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Nature Reviews Materials
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Nature Reviews Materials
1 publication, 2.13%
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Advanced Science
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Advanced Science
1 publication, 2.13%
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Advanced Energy Materials
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Advanced Energy Materials
1 publication, 2.13%
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Small Structures
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Small Structures
1 publication, 2.13%
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Physical Review Letters
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Physical Review Letters
1 publication, 2.13%
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Advanced Materials
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Advanced Materials
1 publication, 2.13%
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Journal of the American Chemical Society
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Journal of the American Chemical Society
1 publication, 2.13%
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Optics Express
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Optics Express
1 publication, 2.13%
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Physical Review E
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Physical Review E
1 publication, 2.13%
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Physical Chemistry Chemical Physics
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Physical Chemistry Chemical Physics
1 publication, 2.13%
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Springer Theses
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Springer Theses
1 publication, 2.13%
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ChemistrySelect
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ChemistrySelect
1 publication, 2.13%
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Advanced Physics Research
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Advanced Physics Research
1 publication, 2.13%
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Citations by publishers
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12
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American Chemical Society (ACS)
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American Chemical Society (ACS)
12 publications, 25.53%
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Springer Nature
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Springer Nature
12 publications, 25.53%
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Wiley
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Wiley
8 publications, 17.02%
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American Physical Society (APS)
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American Physical Society (APS)
6 publications, 12.77%
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Elsevier
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Elsevier
5 publications, 10.64%
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American Institute of Physics (AIP)
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American Institute of Physics (AIP)
1 publication, 2.13%
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Optical Society of America
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Optical Society of America
1 publication, 2.13%
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Royal Society of Chemistry (RSC)
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Royal Society of Chemistry (RSC)
1 publication, 2.13%
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IOP Publishing
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IOP Publishing
1 publication, 2.13%
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- We do not take into account publications that without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Munkhbat B. et al. Tunable self-assembled Casimir microcavities and polaritons // Nature. 2021. Vol. 597. No. 7875. pp. 214-219.
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Munkhbat B., Canales A., Küçüköz B., Baranov D. G., Shegai T. O. Tunable self-assembled Casimir microcavities and polaritons // Nature. 2021. Vol. 597. No. 7875. pp. 214-219.
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TY - JOUR
DO - 10.1038/s41586-021-03826-3
UR - https://doi.org/10.1038%2Fs41586-021-03826-3
TI - Tunable self-assembled Casimir microcavities and polaritons
T2 - Nature
AU - Munkhbat, Battulga
AU - Canales, Adriana
AU - Küçüköz, Betül
AU - Baranov, Denis G.
AU - Shegai, Timur O.
PY - 2021
DA - 2021/09/08 00:00:00
PB - Springer Nature
SP - 214-219
IS - 7875
VL - 597
SN - 0028-0836
SN - 1476-4687
ER -
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@article{2021_Munkhbat,
author = {Battulga Munkhbat and Adriana Canales and Betül Küçüköz and Denis G. Baranov and Timur O. Shegai},
title = {Tunable self-assembled Casimir microcavities and polaritons},
journal = {Nature},
year = {2021},
volume = {597},
publisher = {Springer Nature},
month = {sep},
url = {https://doi.org/10.1038%2Fs41586-021-03826-3},
number = {7875},
pages = {214--219},
doi = {10.1038/s41586-021-03826-3}
}
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MLA
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Munkhbat, Battulga, et al. “Tunable self-assembled Casimir microcavities and polaritons.” Nature, vol. 597, no. 7875, Sep. 2021, pp. 214-219. https://doi.org/10.1038%2Fs41586-021-03826-3.