Open Access
Open access
Scientific Reports, volume 8, issue 1, publication number 6107

Photoluminescence quenching of dye molecules near a resonant silicon nanoparticle

Zyuzin M V 1, 2
Baranov Denis G. 2, 3, 4
Escudero A. 1, 5
Tsypkin Anton 2
Kraus Florain 6
Parak Wolfgang 1, 7
1
 
Fachbereich Physik, Philipps-Universität Marburg, Marburg, Germany
5
 
Instituto de Ciencia de Materiales de Sevilla, CSIC – Universidad de Sevilla, Seville, Spain
6
 
Fachbereich Chemie, Philipps-Universität Marburg, Marburg, Germany
7
 
Fachbereich Physik und Chemie und CHyN, Universität Hamburg, Hamburg, Germany
Publication typeJournal Article
Publication date2018-04-17
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor4.6
ISSN20452322
Multidisciplinary
Abstract

Luminescent molecules attached to resonant colloidal particles are an important tool to study light-matter interaction. A traditional approach to enhance the photoluminescence intensity of the luminescent molecules in such conjugates is to incorporate spacer-coated plasmonic nanoantennas, where the spacer prevents intense non-radiative decay of the luminescent molecules. Here, we explore the capabilities of an alternative platform for photoluminescence enhancement, which is based on low-loss Mie-resonant colloidal silicon particles. We demonstrate that resonant silicon particles of spherical shape are more efficient for photoluminescence enhancement than their plasmonic counterparts in spacer-free configuration. Our theoretical calculations show that significant enhancement originates from larger quantum yields supported by silicon particles and their resonant features. Our results prove the potential of high-index dielectric particles for spacer-free enhancement of photoluminescence, which potentially could be a future platform for bioimaging and nanolasers.

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GOST Copy
Zyuzin M. V. et al. Photoluminescence quenching of dye molecules near a resonant silicon nanoparticle // Scientific Reports. 2018. Vol. 8. No. 1. 6107
GOST all authors (up to 50) Copy
Zyuzin M. V., Baranov D. G., Escudero A., Chakraborty I., Tsypkin A., Ushakova E. V., Kraus F., Parak W., Makarov S. V. Photoluminescence quenching of dye molecules near a resonant silicon nanoparticle // Scientific Reports. 2018. Vol. 8. No. 1. 6107
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RIS Copy
TY - JOUR
DO - 10.1038/s41598-018-24492-y
UR - https://doi.org/10.1038%2Fs41598-018-24492-y
TI - Photoluminescence quenching of dye molecules near a resonant silicon nanoparticle
T2 - Scientific Reports
AU - Zyuzin, M V
AU - Baranov, Denis G.
AU - Escudero, A.
AU - Chakraborty, Indranath
AU - Tsypkin, Anton
AU - Kraus, Florain
AU - Parak, Wolfgang
AU - Makarov, Sergey V
AU - Ushakova, Elena V.
PY - 2018
DA - 2018/04/17 00:00:00
PB - Springer Nature
IS - 1
VL - 8
PMID - 29666416
SN - 2045-2322
ER -
BibTex
Cite this
BibTex Copy
@article{2018_Zyuzin,
author = {M V Zyuzin and Denis G. Baranov and A. Escudero and Indranath Chakraborty and Anton Tsypkin and Florain Kraus and Wolfgang Parak and Sergey V Makarov and Elena V. Ushakova},
title = {Photoluminescence quenching of dye molecules near a resonant silicon nanoparticle},
journal = {Scientific Reports},
year = {2018},
volume = {8},
publisher = {Springer Nature},
month = {apr},
url = {https://doi.org/10.1038%2Fs41598-018-24492-y},
number = {1},
doi = {10.1038/s41598-018-24492-y}
}
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