Open Access
Open access
npj 2D Materials and Applications, volume 4, issue 1, publication number 21

Broadband optical properties of monolayer and bulk MoS2

Stebunov Yury V 2, 3
Nikitin Alexey Y 2, 5, 6
Arsenin Aleksey V. 2, 3
Volkov Valentyn S. 2, 3
Publication typeJournal Article
Publication date2020-07-10
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor9.7
ISSN23977132
General Chemistry
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Mechanics of Materials
Abstract

Layered semiconductors such as transition metal dichalcogenides (TMDs) offer endless possibilities for designing modern photonic and optoelectronic components. However, their optical engineering is still a challenging task owing to multiple obstacles, including the absence of a rapid, contactless, and the reliable method to obtain their dielectric function as well as to evaluate in situ the changes in optical constants and exciton binding energies. Here, we present an advanced approach based on ellipsometry measurements for retrieval of dielectric functions and the excitonic properties of both monolayer and bulk TMDs. Using this method, we conduct a detailed study of monolayer MoS2 and its bulk crystal in the broad spectral range (290–3300 nm). In the near- and mid-infrared ranges, both configurations appear to have no optical absorption and possess an extremely high dielectric permittivity making them favorable for lossless subwavelength photonics. In addition, the proposed approach opens a possibility to observe a previously unreported peak in the dielectric function of monolayer MoS2 induced by the use of perylene-3,4,9,10-tetracarboxylic acid tetrapotassium salt (PTAS) seeding promoters for MoS2 synthesis and thus enables its applications in chemical and biological sensing. Therefore, this technique as a whole offers a state-of-the-art metrological tool for next-generation TMD-based devices.

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Ermolaev G. A. et al. Broadband optical properties of monolayer and bulk MoS2 // npj 2D Materials and Applications. 2020. Vol. 4. No. 1. 21
GOST all authors (up to 50) Copy
Ermolaev G. A., Stebunov Y. V., Vyshnevyy A. A., Tatarkin D. E., Yakubovsky D. I., Novikov S., Baranov D. G., Shegai T. O., Nikitin A. Y., Arsenin A. V., Volkov V. S. Broadband optical properties of monolayer and bulk MoS2 // npj 2D Materials and Applications. 2020. Vol. 4. No. 1. 21
RIS |
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RIS Copy
TY - JOUR
DO - 10.1038/s41699-020-0155-x
UR - https://doi.org/10.1038%2Fs41699-020-0155-x
TI - Broadband optical properties of monolayer and bulk MoS2
T2 - npj 2D Materials and Applications
AU - Ermolaev, Georgy A.
AU - Vyshnevyy, Andrey A.
AU - Tatarkin, Dmitry E
AU - Yakubovsky, Dmitry I.
AU - Novikov, Sergey
AU - Baranov, Denis G.
AU - Shegai, Timur O.
AU - Nikitin, Alexey Y
AU - Arsenin, Aleksey V.
AU - Volkov, Valentyn S.
AU - Stebunov, Yury V
PY - 2020
DA - 2020/07/10 00:00:00
PB - Springer Nature
IS - 1
VL - 4
SN - 2397-7132
ER -
BibTex
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BibTex Copy
@article{2020_Ermolaev
author = {Georgy A. Ermolaev and Andrey A. Vyshnevyy and Dmitry E Tatarkin and Dmitry I. Yakubovsky and Sergey Novikov and Denis G. Baranov and Timur O. Shegai and Alexey Y Nikitin and Aleksey V. Arsenin and Valentyn S. Volkov and Yury V Stebunov},
title = {Broadband optical properties of monolayer and bulk MoS2},
journal = {npj 2D Materials and Applications},
year = {2020},
volume = {4},
publisher = {Springer Nature},
month = {jul},
url = {https://doi.org/10.1038%2Fs41699-020-0155-x},
number = {1},
doi = {10.1038/s41699-020-0155-x}
}
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