Physical Chemistry Chemical Physics, volume 4, issue 22, pages 5442-5447
EPR investigation of atoms in chemical traps
Publication type: Journal Article
Publication date: 2002-11-01
Journal:
Physical Chemistry Chemical Physics
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor: 3.3
ISSN: 14639076, 14639084
DOI:
10.1039/b206261e
Physical and Theoretical Chemistry
General Physics and Astronomy
Abstract
Magnetic properties of atoms and molecular clusters encapsulated in fullerenes and other chemical traps are studied using various EPR and ENDOR techniques. From these results exceptional topological and electronic properties of these new compounds can be derived. Making use of the high symmetry at the site of the encased paramagnetic atom, details of the deformation of the spin density distribution resulting from the confinement are deduced. Dissolving N@C60 and N@C70 in a liquid crystal, the order parameter of the solute can be studied by invoking the fine structure interaction of confined nitrogen in its 4S3/2 ground state. Information about the interaction potential locating the neutral atoms at the cage centre is obtained from an analysis of the temperature dependence of the hyperfine coupling constant. Values deduced are in good agreement with vibrational frequencies calculated in harmonic approximation.
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GOST
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Dinse K. EPR investigation of atoms in chemical traps // Physical Chemistry Chemical Physics. 2002. Vol. 4. No. 22. pp. 5442-5447.
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Dinse K. EPR investigation of atoms in chemical traps // Physical Chemistry Chemical Physics. 2002. Vol. 4. No. 22. pp. 5442-5447.
Cite this
RIS
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TY - JOUR
DO - 10.1039/b206261e
UR - https://doi.org/10.1039/b206261e
TI - EPR investigation of atoms in chemical traps
T2 - Physical Chemistry Chemical Physics
AU - Dinse, Klaus-Peter
PY - 2002
DA - 2002/11/01
PB - Royal Society of Chemistry (RSC)
SP - 5442-5447
IS - 22
VL - 4
SN - 1463-9076
SN - 1463-9084
ER -
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BibTex
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@article{2002_Dinse,
author = {Klaus-Peter Dinse},
title = {EPR investigation of atoms in chemical traps},
journal = {Physical Chemistry Chemical Physics},
year = {2002},
volume = {4},
publisher = {Royal Society of Chemistry (RSC)},
month = {nov},
url = {https://doi.org/10.1039/b206261e},
number = {22},
pages = {5442--5447},
doi = {10.1039/b206261e}
}
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MLA
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Dinse, Klaus-Peter. “EPR investigation of atoms in chemical traps.” Physical Chemistry Chemical Physics, vol. 4, no. 22, Nov. 2002, pp. 5442-5447. https://doi.org/10.1039/b206261e.