Visible light photoredox-catalysed remote C–H functionalisation enabled by 1,5-hydrogen atom transfer (1,5-HAT)
2
College of Chemistry & Molecular Engineering
4
Qingdao
|
5
P. R. China
|
7
Laboratory of Synthesis and Natural Products, Institute of Chemical Sciences and Engineering
10
1015 Lausanne
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11
SWITZERLAND
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Publication type: Journal Article
Publication date: 2021-05-20
scimago Q1
wos Q1
SJR: 11.467
CiteScore: 73.2
Impact factor: 39.0
ISSN: 03060012, 14604744
PubMed ID:
34013927
General Chemistry
Abstract
The generation of heteroatom-centred radicals (X˙), followed by intramolecular 1,5-hydrogen atom transfer (1,5-HAT) and the functionalisation of the translocated carbon-centred radicals, is the basic mechanism of the classic Hofmann–Löffler–Freytag (HLF) reaction and the Barton reaction. The chemoselectivity of the 1,5-HAT process is different from that of the transition metal-catalysed counterpart, providing, therefore, a complementary tool for remote C(sp3)–H bond functionalisation. There is a recent resurgence in this research field due to the emergence of visible light photocatalysis. This tutorial review summarises the recent progress in the remote functionalisation of C–H bonds featuring a key 1,5-HAT step with particular focus on photoredox-catalyzed remote C–H functionalisation.
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Guo W. et al. Visible light photoredox-catalysed remote C–H functionalisation enabled by 1,5-hydrogen atom transfer (1,5-HAT) // Chemical Society Reviews. 2021. Vol. 50. No. 13. pp. 7359-7377.
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Guo W., Wang Q., Zhu J. Visible light photoredox-catalysed remote C–H functionalisation enabled by 1,5-hydrogen atom transfer (1,5-HAT) // Chemical Society Reviews. 2021. Vol. 50. No. 13. pp. 7359-7377.
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TY - JOUR
DO - 10.1039/d0cs00774a
UR - https://xlink.rsc.org/?DOI=D0CS00774A
TI - Visible light photoredox-catalysed remote C–H functionalisation enabled by 1,5-hydrogen atom transfer (1,5-HAT)
T2 - Chemical Society Reviews
AU - Guo, Weisi
AU - Wang, Qian
AU - Zhu, Jieping
PY - 2021
DA - 2021/05/20
PB - Royal Society of Chemistry (RSC)
SP - 7359-7377
IS - 13
VL - 50
PMID - 34013927
SN - 0306-0012
SN - 1460-4744
ER -
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@article{2021_Guo,
author = {Weisi Guo and Qian Wang and Jieping Zhu},
title = {Visible light photoredox-catalysed remote C–H functionalisation enabled by 1,5-hydrogen atom transfer (1,5-HAT)},
journal = {Chemical Society Reviews},
year = {2021},
volume = {50},
publisher = {Royal Society of Chemistry (RSC)},
month = {may},
url = {https://xlink.rsc.org/?DOI=D0CS00774A},
number = {13},
pages = {7359--7377},
doi = {10.1039/d0cs00774a}
}
Cite this
MLA
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Guo, Weisi, et al. “Visible light photoredox-catalysed remote C–H functionalisation enabled by 1,5-hydrogen atom transfer (1,5-HAT).” Chemical Society Reviews, vol. 50, no. 13, May. 2021, pp. 7359-7377. https://xlink.rsc.org/?DOI=D0CS00774A.