Physical Chemistry Chemical Physics, volume 16, issue 28, pages 14669-14674
A new ultrafast superionic Li-conductor: ion dynamics in Li11Si2PS12and comparison with other tetragonal LGPS-type electrolytes
Alexander Kühn
1
,
Alexander Kuhn
1
,
Oliver Gerbig
1
,
Changbao Zhu
1
,
Frank Falkenberg
1
,
Joachim Maier
1
,
B. V. Lotsch
1, 2, 3
3
Nanosystems Initiative Munich (NIM) and Center for Nanoscience (CeNS), Schellingstr. 4, 80799 München, Germany
|
Publication type: Journal Article
Publication date: 2014-05-30
Journal:
Physical Chemistry Chemical Physics
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor: 3.3
ISSN: 14639076, 14639084
Physical and Theoretical Chemistry
General Physics and Astronomy
Abstract
We report on a new ultrafast solid electrolyte of the composition Li11Si2PS12, which exhibits a higher room-temperature Li ion diffusivity than the present record holder Li10GeP2S12. We discuss the high-pressure synthesis and ion dynamics of tetragonal Li11Si2PS12, and comparison is made with our investigations of related members of the LMePS family, i.e. electrolytes of the general formula Li11-xMe2-xP1+xS12 with Me = Ge, Sn : Li10GeP2S12, Li7GePS8, Li10SnP2S12. The structure and dynamics were studied with multiple complementary techniques and the macroscopic diffusion could be traced back to fast Li ion hopping in the crystalline lattice. A clear correlation between the diffusivity and the unit cell volume of the LGPS-type electrolytes was observed.
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Citations by publishers
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80
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78 publications, 30.23%
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10
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- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
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Kühn A. et al. A new ultrafast superionic Li-conductor: ion dynamics in Li11Si2PS12and comparison with other tetragonal LGPS-type electrolytes // Physical Chemistry Chemical Physics. 2014. Vol. 16. No. 28. pp. 14669-14674.
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Kühn A., Kuhn A., Gerbig O., Zhu C., Falkenberg F., Maier J., Lotsch B. V. A new ultrafast superionic Li-conductor: ion dynamics in Li11Si2PS12and comparison with other tetragonal LGPS-type electrolytes // Physical Chemistry Chemical Physics. 2014. Vol. 16. No. 28. pp. 14669-14674.
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TY - JOUR
DO - 10.1039/C4CP02046D
UR - https://doi.org/10.1039/C4CP02046D
TI - A new ultrafast superionic Li-conductor: ion dynamics in Li11Si2PS12and comparison with other tetragonal LGPS-type electrolytes
T2 - Physical Chemistry Chemical Physics
AU - Kühn, Alexander
AU - Gerbig, Oliver
AU - Falkenberg, Frank
AU - Zhu, Changbao
AU - Maier, Joachim
AU - Lotsch, B. V.
AU - Kuhn, Alexander
PY - 2014
DA - 2014/05/30 00:00:00
PB - Royal Society of Chemistry (RSC)
SP - 14669-14674
IS - 28
VL - 16
SN - 1463-9076
SN - 1463-9084
ER -
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@article{2014_Kühn,
author = {Alexander Kühn and Oliver Gerbig and Frank Falkenberg and Changbao Zhu and Joachim Maier and B. V. Lotsch and Alexander Kuhn},
title = {A new ultrafast superionic Li-conductor: ion dynamics in Li11Si2PS12and comparison with other tetragonal LGPS-type electrolytes},
journal = {Physical Chemistry Chemical Physics},
year = {2014},
volume = {16},
publisher = {Royal Society of Chemistry (RSC)},
month = {may},
url = {https://doi.org/10.1039/C4CP02046D},
number = {28},
pages = {14669--14674},
doi = {10.1039/C4CP02046D}
}
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Kühn, Alexander, et al. “A new ultrafast superionic Li-conductor: ion dynamics in Li11Si2PS12and comparison with other tetragonal LGPS-type electrolytes.” Physical Chemistry Chemical Physics, vol. 16, no. 28, May. 2014, pp. 14669-14674. https://doi.org/10.1039/C4CP02046D.
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