Chemical Communications

, том 51 , издание 54 , страницы 10907-10909

Acrylate formation from CO₂ and ethylene: catalysis with palladium and mechanistic insight

Тип публикации: Journal Article

Дата публикации: 2015-06-03

Royal Society of Chemistry (RSC)

Chemical Communications

scimago Q1

wos Q2

white level БС1

SJR: 1.037

CiteScore: 7.4

Impact factor: 4.2

ISSN: 13597345, 1364548X

DOI: 10.1039/c5cc01932j

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PubMed ID: 26060842

Materials Chemistry

Metals and Alloys

Surfaces, Coatings and Films

General Chemistry

Ceramics and Composites

Electronic, Optical and Magnetic Materials

Catalysis

Краткое описание

We report the first catalyst based on palladium for the reaction of CO2, alkene and a base to form sodium acrylate and derivatives. A mechanism similar to a previously reported Ni(0)-catalyst is proposed based on stoichiometric in situ NMR experiments, isolated intermediates and a parent palladalactone. Our palladium catalyst was applied to the coupling of CO2 with conjugated alkenes.

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Stieber S. C. E. et al. Acrylate formation from CO2 and ethylene: catalysis with palladium and mechanistic insight // Chemical Communications. 2015. Vol. 51. No. 54. pp. 10907-10909.

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Stieber S. C. E., Huguet N., Kageyama T., Jevtovikj I., Ariyananda P., Gordillo A., Schunk S. A., Rominger F., Hofmann P., Limbach M. Acrylate formation from CO2 and ethylene: catalysis with palladium and mechanistic insight // Chemical Communications. 2015. Vol. 51. No. 54. pp. 10907-10909.

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TY - JOUR

DO - 10.1039/c5cc01932j

UR - https://doi.org/10.1039/c5cc01932j

TI - Acrylate formation from CO2 and ethylene: catalysis with palladium and mechanistic insight

T2 - Chemical Communications

AU - Stieber, S Chantal E

AU - Huguet, Núria

AU - Kageyama, Takeharu

AU - Jevtovikj, Ivana

AU - Ariyananda, Piyal

AU - Gordillo, Alvaro

AU - Schunk, Stephan A.

AU - Rominger, Frank

AU - Hofmann, Peter

AU - Limbach, Michael

PY - 2015

DA - 2015/06/03

PB - Royal Society of Chemistry (RSC)

SP - 10907-10909

IS - 54

VL - 51

PMID - 26060842

SN - 1359-7345

SN - 1364-548X

ER -

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@article{2015_Stieber,

author = {S Chantal E Stieber and Núria Huguet and Takeharu Kageyama and Ivana Jevtovikj and Piyal Ariyananda and Alvaro Gordillo and Stephan A. Schunk and Frank Rominger and Peter Hofmann and Michael Limbach},

title = {Acrylate formation from CO2 and ethylene: catalysis with palladium and mechanistic insight},

journal = {Chemical Communications},

year = {2015},

volume = {51},

publisher = {Royal Society of Chemistry (RSC)},

month = {jun},

url = {https://doi.org/10.1039/c5cc01932j},

number = {54},

pages = {10907--10909},

doi = {10.1039/c5cc01932j}

}

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Stieber, S. Chantal E., et al. “Acrylate formation from CO2 and ethylene: catalysis with palladium and mechanistic insight.” Chemical Communications, vol. 51, no. 54, Jun. 2015, pp. 10907-10909. https://doi.org/10.1039/c5cc01932j.