Chemical Communications, volume 51, issue 54, pages 10907-10909
Acrylate formation from CO2 and ethylene: catalysis with palladium and mechanistic insight
S Chantal E Stieber
1
,
Núria Huguet
1
,
Takeharu Kageyama
1
,
Ivana Jevtovikj
1
,
Piyal Ariyananda
1
,
Alvaro Gordillo
1, 2
,
Stephan A. Schunk
2
,
Frank Rominger
3
,
Peter Hofmann
1, 3
,
Michael Limbach
1, 4
1
CaRLa (Catalysis Research Laboratory), Im Neuenheimer Feld 584, 69120 Heidelberg, Germany
|
2
hte Aktiengesellschaft, Kurpfalzring 104, 69123 Heidelberg, Germany
|
4
BASF SE, Carl-Bosch-Strasse 38, 67056 Ludwigshafen, Germany
|
Publication type: Journal Article
Publication date: 2015-06-03
Journal:
Chemical Communications
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor: 4.9
ISSN: 13597345, 1364548X
Materials Chemistry
Metals and Alloys
Surfaces, Coatings and Films
General Chemistry
Ceramics and Composites
Electronic, Optical and Magnetic Materials
Catalysis
Abstract
We report the first catalyst based on palladium for the reaction of CO2, alkene and a base to form sodium acrylate and derivatives. A mechanism similar to a previously reported Ni(0)-catalyst is proposed based on stoichiometric in situ NMR experiments, isolated intermediates and a parent palladalactone. Our palladium catalyst was applied to the coupling of CO2 with conjugated alkenes.
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GOST
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Stieber S. C. E. et al. Acrylate formation from CO2 and ethylene: catalysis with palladium and mechanistic insight // Chemical Communications. 2015. Vol. 51. No. 54. pp. 10907-10909.
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Stieber S. C. E., Huguet N., Kageyama T., Jevtovikj I., Ariyananda P., Gordillo A., Schunk S. A., Rominger F., Hofmann P., Limbach M. Acrylate formation from CO2 and ethylene: catalysis with palladium and mechanistic insight // Chemical Communications. 2015. Vol. 51. No. 54. pp. 10907-10909.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1039/c5cc01932j
UR - https://doi.org/10.1039/c5cc01932j
TI - Acrylate formation from CO2 and ethylene: catalysis with palladium and mechanistic insight
T2 - Chemical Communications
AU - Stieber, S Chantal E
AU - Huguet, Núria
AU - Kageyama, Takeharu
AU - Jevtovikj, Ivana
AU - Ariyananda, Piyal
AU - Gordillo, Alvaro
AU - Rominger, Frank
AU - Hofmann, Peter
AU - Limbach, Michael
AU - Schunk, Stephan A.
PY - 2015
DA - 2015/06/03
PB - Royal Society of Chemistry (RSC)
SP - 10907-10909
IS - 54
VL - 51
SN - 1359-7345
SN - 1364-548X
ER -
Cite this
BibTex
Copy
@article{2015_Stieber,
author = {S Chantal E Stieber and Núria Huguet and Takeharu Kageyama and Ivana Jevtovikj and Piyal Ariyananda and Alvaro Gordillo and Frank Rominger and Peter Hofmann and Michael Limbach and Stephan A. Schunk},
title = {Acrylate formation from CO2 and ethylene: catalysis with palladium and mechanistic insight},
journal = {Chemical Communications},
year = {2015},
volume = {51},
publisher = {Royal Society of Chemistry (RSC)},
month = {jun},
url = {https://doi.org/10.1039/c5cc01932j},
number = {54},
pages = {10907--10909},
doi = {10.1039/c5cc01932j}
}
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MLA
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Stieber, S. Chantal E., et al. “Acrylate formation from CO2 and ethylene: catalysis with palladium and mechanistic insight.” Chemical Communications, vol. 51, no. 54, Jun. 2015, pp. 10907-10909. https://doi.org/10.1039/c5cc01932j.