Chemical Society Reviews, volume 46, issue 3, pages 797-815
Single lithium-ion conducting solid polymer electrolytes: advances and perspectives.
Heng Zhang
1
,
Chunmei Li
1
,
Michal Piszcz
1
,
Estibaliz Coya
1
,
Jun Lu
1
,
Lide M. Rodríguez-Martínez
1
,
Lide M. Rodriguez-Martinez
1
,
Michel Armand
1
,
Zhibin Zhou
2
1
CIC EnergiGUNE, Albert Einstein 48, 01510 Miñano, Álava, Spain
|
Publication type: Journal Article
Publication date: 2017-01-18
Journal:
Chemical Society Reviews
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 46.2
ISSN: 03060012, 14604744
General Chemistry
Abstract
Electrochemical energy storage is one of the main societal challenges to humankind in this century. The performances of classical Li-ion batteries (LIBs) with non-aqueous liquid electrolytes have made great advances in the past two decades, but the intrinsic instability of liquid electrolytes results in safety issues, and the energy density of the state-of-the-art LIBs cannot satisfy the practical requirement. Therefore, rechargeable lithium metal batteries (LMBs) have been intensively investigated considering the high theoretical capacity of lithium metal and its low negative potential. However, the progress in the field of non-aqueous liquid electrolytes for LMBs has been sluggish, with several seemingly insurmountable barriers, including dendritic Li growth and rapid capacity fading. Solid polymer electrolytes (SPEs) offer a perfect solution to these safety concerns and to the enhancement of energy density. Traditional SPEs are dual-ion conductors, in which both cations and anions are mobile and will cause a concentration polarization thus leading to poor performances of both LIBs and LMBs. Single lithium-ion (Li-ion) conducting solid polymer electrolytes (SLIC-SPEs), which have anions covalently bonded to the polymer, inorganic backbone, or immobilized by anion acceptors, are generally accepted to have advantages over conventional dual-ion conducting SPEs for application in LMBs. A high Li-ion transference number (LTN), the absence of the detrimental effect of anion polarization, and the low rate of Li dendrite growth are examples of benefits of SLIC-SPEs. To date, many types of SLIC-SPEs have been reported, including those based on organic polymers, organic-inorganic hybrid polymers and anion acceptors. In this review, a brief overview of synthetic strategies on how to realize SLIC-SPEs is given. The fundamental physical and electrochemical properties of SLIC-SPEs prepared by different methods are discussed in detail. In particular, special attention is paid to the SLIC-SPEs with high ionic conductivity and high LTN. Finally, perspectives on the main challenges and focus on the future research are also presented.
Top-30
Citations by journals
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ACS Macro Letters
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10 publications, 1.11%
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10 publications, 1.11%
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RSC Advances
8 publications, 0.89%
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Citations by publishers
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Elsevier
223 publications, 24.86%
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Wiley
202 publications, 22.52%
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American Chemical Society (ACS)
201 publications, 22.41%
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Royal Society of Chemistry (RSC)
107 publications, 11.93%
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Springer Nature
48 publications, 5.35%
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Multidisciplinary Digital Publishing Institute (MDPI)
24 publications, 2.68%
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The Electrochemical Society
24 publications, 2.68%
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American Institute of Physics (AIP)
9 publications, 1%
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Pleiades Publishing
8 publications, 0.89%
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IOP Publishing
6 publications, 0.67%
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Frontiers Media S.A.
6 publications, 0.67%
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American Association for the Advancement of Science (AAAS)
3 publications, 0.33%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
2 publications, 0.22%
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American Physical Society (APS)
2 publications, 0.22%
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The Chemical Society of Japan
2 publications, 0.22%
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University of Science and Technology Beijing
2 publications, 0.22%
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Taylor & Francis
2 publications, 0.22%
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Oxford University Press
2 publications, 0.22%
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OAE Publishing Inc.
2 publications, 0.22%
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ASME
1 publication, 0.11%
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American Vacuum Society
1 publication, 0.11%
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Bentham Science
1 publication, 0.11%
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Cambridge University Press
1 publication, 0.11%
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Nonferrous Metals Society of China
1 publication, 0.11%
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Korean Society of Industrial Engineering Chemistry
1 publication, 0.11%
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Chinese Physical Society
1 publication, 0.11%
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Hans Publishers
1 publication, 0.11%
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SAGE
1 publication, 0.11%
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Ivanovo State University of Chemistry and Technology
1 publication, 0.11%
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50
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Zhang H. et al. Single lithium-ion conducting solid polymer electrolytes: advances and perspectives. // Chemical Society Reviews. 2017. Vol. 46. No. 3. pp. 797-815.
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Zhang H., Li C., Piszcz M., Coya E., Lu J., Rodríguez-Martínez L. M., Rodriguez-Martinez L. M., Armand M., Zhou Z. Single lithium-ion conducting solid polymer electrolytes: advances and perspectives. // Chemical Society Reviews. 2017. Vol. 46. No. 3. pp. 797-815.
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TY - JOUR
DO - 10.1039/C6CS00491A
UR - https://doi.org/10.1039/C6CS00491A
TI - Single lithium-ion conducting solid polymer electrolytes: advances and perspectives.
T2 - Chemical Society Reviews
AU - Zhang, Heng
AU - Coya, Estibaliz
AU - Rodríguez-Martínez, Lide M.
AU - Li, Chunmei
AU - Piszcz, Michal
AU - Lu, Jun
AU - Armand, Michel
AU - Zhou, Zhibin
AU - Rodriguez-Martinez, Lide M.
PY - 2017
DA - 2017/01/18 00:00:00
PB - Royal Society of Chemistry (RSC)
SP - 797-815
IS - 3
VL - 46
SN - 0306-0012
SN - 1460-4744
ER -
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@article{2017_Zhang,
author = {Heng Zhang and Estibaliz Coya and Lide M. Rodríguez-Martínez and Chunmei Li and Michal Piszcz and Jun Lu and Michel Armand and Zhibin Zhou and Lide M. Rodriguez-Martinez},
title = {Single lithium-ion conducting solid polymer electrolytes: advances and perspectives.},
journal = {Chemical Society Reviews},
year = {2017},
volume = {46},
publisher = {Royal Society of Chemistry (RSC)},
month = {jan},
url = {https://doi.org/10.1039/C6CS00491A},
number = {3},
pages = {797--815},
doi = {10.1039/C6CS00491A}
}
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Zhang, Heng, et al. “Single lithium-ion conducting solid polymer electrolytes: advances and perspectives..” Chemical Society Reviews, vol. 46, no. 3, Jan. 2017, pp. 797-815. https://doi.org/10.1039/C6CS00491A.
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