Detailed electronic structure of a high-spin cobalt(ii) complex determined from NMR and THz-EPR spectroscopy.
Тип публикации: Journal Article
Дата публикации: 2019-04-01
scimago Q2
wos Q2
БС2
SJR: 0.698
CiteScore: 5.3
Impact factor: 2.9
ISSN: 14639076, 14639084
PubMed ID:
30950488
Physical and Theoretical Chemistry
General Physics and Astronomy
Краткое описание
Here we report a combined use of THz-EPR and NMR spectroscopy for obtaining a detailed electronic structure of a long-known high-spin complex, cobalt(ii) bis[tris(pyrazolyl)borate]. The lowest inter-Kramers transition was directly measured by THz-EPR spectroscopy, while the energies of higher Kramers doublets were estimated by a recently proposed NMR-based approach. Together, they produced magnetic parameters for a full model that explicitly includes spin-orbit coupling. This approach is applicable to all transition metal ions for which the spin-orbit coupling cannot be treated perturbatively.
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Pavlov A. A. et al. Detailed electronic structure of a high-spin cobalt(ii) complex determined from NMR and THz-EPR spectroscopy. // Physical Chemistry Chemical Physics. 2019. Vol. 21. No. 16. pp. 8201-8204.
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Pavlov A. A., Nehrkorn J., Pankratova Y. A., Ozerov M., Mikhalyova E. A., Polezhaev A., Polezhaev A. V., Nelyubina Y. V., Novikov V. V. Detailed electronic structure of a high-spin cobalt(ii) complex determined from NMR and THz-EPR spectroscopy. // Physical Chemistry Chemical Physics. 2019. Vol. 21. No. 16. pp. 8201-8204.
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TY - JOUR
DO - 10.1039/C9CP01474H
UR - https://xlink.rsc.org/?DOI=C9CP01474H
TI - Detailed electronic structure of a high-spin cobalt(ii) complex determined from NMR and THz-EPR spectroscopy.
T2 - Physical Chemistry Chemical Physics
AU - Pavlov, Alexander A
AU - Nehrkorn, Joscha
AU - Pankratova, Yanina A
AU - Ozerov, M.
AU - Mikhalyova, Elena A
AU - Polezhaev, Alexander
AU - Polezhaev, Alexander V
AU - Nelyubina, Yulia V.
AU - Novikov, Valentin V
PY - 2019
DA - 2019/04/01
PB - Royal Society of Chemistry (RSC)
SP - 8201-8204
IS - 16
VL - 21
PMID - 30950488
SN - 1463-9076
SN - 1463-9084
ER -
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@article{2019_Pavlov,
author = {Alexander A Pavlov and Joscha Nehrkorn and Yanina A Pankratova and M. Ozerov and Elena A Mikhalyova and Alexander Polezhaev and Alexander V Polezhaev and Yulia V. Nelyubina and Valentin V Novikov},
title = {Detailed electronic structure of a high-spin cobalt(ii) complex determined from NMR and THz-EPR spectroscopy.},
journal = {Physical Chemistry Chemical Physics},
year = {2019},
volume = {21},
publisher = {Royal Society of Chemistry (RSC)},
month = {apr},
url = {https://xlink.rsc.org/?DOI=C9CP01474H},
number = {16},
pages = {8201--8204},
doi = {10.1039/C9CP01474H}
}
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MLA
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Pavlov, Alexander A., et al. “Detailed electronic structure of a high-spin cobalt(ii) complex determined from NMR and THz-EPR spectroscopy..” Physical Chemistry Chemical Physics, vol. 21, no. 16, Apr. 2019, pp. 8201-8204. https://xlink.rsc.org/?DOI=C9CP01474H.