Synthesis and crystal structure of the Sr2 Al1.07 Mn0.93 O5 brownmillerite
Joke Hadermann
1
,
Artem M. Abakumov
1, 2
,
Hans D'Hondt
1
,
Anna S Kalyuzhnaya
2
,
Marina G Rozova
2
,
Maria M. Markina
3
,
Mikhail G Mikheev
3
,
Natalia Tristan
4
,
Р. Клингелер
4
,
B. Büchner
4
,
4
Institute for Solid State Research, Dresden, Germany
|
Publication type: Journal Article
Publication date: 2007-01-01
scimago Q1
wos Q1
SJR: 2.462
CiteScore: 16.7
Impact factor: 9.5
ISSN: 20507488, 20507496, 09599428, 13645501
DOI:
10.1039/b614168d
Materials Chemistry
General Chemistry
Abstract
A new brownmillerite-type compound Sr2Al1.07Mn0.93O5 was synthesized. The crystal structure was determined using electron diffraction and high resolution transmission electron microscopy and refined from X-ray powder diffraction data (space group Imma, a = 5.4358(1) A, b = 15.6230(4) A, c = 5.6075(1) A, RI = 0.036, RP = 0.023). The structure is characterized by a disordered distribution of the tetrahedral chains in L and R configuration and a partial occupation of the octahedral position by the Mn3+ and Al3+ cations. The relationships between the crystal structures of Sr2Al1.07Mn0.93O5 and its A2B′MnO5 analogues (A = Ca, Sr, B′ = Al, Ga) and the structural reasons for the different types of tetrahedral chain ordering in brownmillerites are discussed. The temperature dependences of the magnetic susceptibility and specific heat reveal that the compound is antiferromagnetically ordered below TN = 105 K.
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Hadermann J. et al. Synthesis and crystal structure of the Sr2Al1.07Mn0.93O5 brownmillerite // Journal of Materials Chemistry A. 2007. Vol. 17. No. 7. pp. 692-698.
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Hadermann J., Abakumov A. M., D'Hondt H., Kalyuzhnaya A. S., Rozova M. G., Markina M. M., Mikheev M. G., Tristan N., Клингелер Р., Büchner B., Antipov E. V. Synthesis and crystal structure of the Sr2Al1.07Mn0.93O5 brownmillerite // Journal of Materials Chemistry A. 2007. Vol. 17. No. 7. pp. 692-698.
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RIS
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TY - JOUR
DO - 10.1039/b614168d
UR - https://xlink.rsc.org/?DOI=B614168D
TI - Synthesis and crystal structure of the Sr2Al1.07Mn0.93O5 brownmillerite
T2 - Journal of Materials Chemistry A
AU - Hadermann, Joke
AU - Abakumov, Artem M.
AU - D'Hondt, Hans
AU - Kalyuzhnaya, Anna S
AU - Rozova, Marina G
AU - Markina, Maria M.
AU - Mikheev, Mikhail G
AU - Tristan, Natalia
AU - Клингелер, Р.
AU - Büchner, B.
AU - Antipov, Evgeny V.
PY - 2007
DA - 2007/01/01
PB - Royal Society of Chemistry (RSC)
SP - 692-698
IS - 7
VL - 17
SN - 2050-7488
SN - 2050-7496
SN - 0959-9428
SN - 1364-5501
ER -
Cite this
BibTex (up to 50 authors)
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@article{2007_Hadermann,
author = {Joke Hadermann and Artem M. Abakumov and Hans D'Hondt and Anna S Kalyuzhnaya and Marina G Rozova and Maria M. Markina and Mikhail G Mikheev and Natalia Tristan and Р. Клингелер and B. Büchner and Evgeny V. Antipov},
title = {Synthesis and crystal structure of the Sr2Al1.07Mn0.93O5 brownmillerite},
journal = {Journal of Materials Chemistry A},
year = {2007},
volume = {17},
publisher = {Royal Society of Chemistry (RSC)},
month = {jan},
url = {https://xlink.rsc.org/?DOI=B614168D},
number = {7},
pages = {692--698},
doi = {10.1039/b614168d}
}
Cite this
MLA
Copy
Hadermann, Joke, et al. “Synthesis and crystal structure of the Sr2Al1.07Mn0.93O5 brownmillerite.” Journal of Materials Chemistry A, vol. 17, no. 7, Jan. 2007, pp. 692-698. https://xlink.rsc.org/?DOI=B614168D.