том 40 издание 43 страницы 11474-11479

NMR investigation of intramolecular dynamics of heteroleptic triple-decker (porphyrinato)(phthalocyaninato) lanthanides

Тип публикацииJournal Article
Дата публикации2011-09-20
scimago Q2
wos Q1
БС1
SJR0.653
CiteScore6.0
Impact factor3.3
ISSN14779226, 14779234
Inorganic Chemistry
Краткое описание
Intramolecular dynamics of meso-aryl substituents of porphyrin deck in the triple-decker lanthanide (porphyrinato)(phthalocyaninates) of symmetrical type [Br(4)TPP]Ln[(15C5)(4)Pc]Ln[Br(4)TPP] (Ln = La, Nd, Eu; [Br(4)TPP] = tetrakis-5,10,15,20-(4-bromophenyl)-porphyrinato-ligand; [(15C5)(4)Pc] = tetrakis-(15-crown-5)-phthalocyaninato-ligand) are investigated. Attempts to achieve coalescence were not successful, although the trend of exchanging protons to coalescence point was observed in the case of Nd and Eu complexes. The analysis of NOESY cross-peaks between exchanging protons allowed to evaluate the rotation rate constants at different temperatures. The activation barrier of the meso-aryl substituent rotation was calculated with Arrhenius equation based on determined rate constants. The rate constants are lower and activation barriers are higher than ones found previously for related compounds.
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Inorganic Chemistry
3 публикации, 20%
Journal of Porphyrins and Phthalocyanines
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Birin K. P. et al. NMR investigation of intramolecular dynamics of heteroleptic triple-decker (porphyrinato)(phthalocyaninato) lanthanides // Dalton Transactions. 2011. Vol. 40. No. 43. pp. 11474-11479.
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Birin K. P., Gorbunova Y. G., Tsivadze A. NMR investigation of intramolecular dynamics of heteroleptic triple-decker (porphyrinato)(phthalocyaninato) lanthanides // Dalton Transactions. 2011. Vol. 40. No. 43. pp. 11474-11479.
RIS |
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TY - JOUR
DO - 10.1039/c1dt11231g
UR - https://xlink.rsc.org/?DOI=c1dt11231g
TI - NMR investigation of intramolecular dynamics of heteroleptic triple-decker (porphyrinato)(phthalocyaninato) lanthanides
T2 - Dalton Transactions
AU - Birin, Kirill P.
AU - Gorbunova, Yulia G.
AU - Tsivadze, Aslan
PY - 2011
DA - 2011/09/20
PB - Royal Society of Chemistry (RSC)
SP - 11474-11479
IS - 43
VL - 40
PMID - 21931915
SN - 1477-9226
SN - 1477-9234
ER -
BibTex |
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BibTex (до 50 авторов) Скопировать
@article{2011_Birin,
author = {Kirill P. Birin and Yulia G. Gorbunova and Aslan Tsivadze},
title = {NMR investigation of intramolecular dynamics of heteroleptic triple-decker (porphyrinato)(phthalocyaninato) lanthanides},
journal = {Dalton Transactions},
year = {2011},
volume = {40},
publisher = {Royal Society of Chemistry (RSC)},
month = {sep},
url = {https://xlink.rsc.org/?DOI=c1dt11231g},
number = {43},
pages = {11474--11479},
doi = {10.1039/c1dt11231g}
}
MLA
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Birin, Kirill P., et al. “NMR investigation of intramolecular dynamics of heteroleptic triple-decker (porphyrinato)(phthalocyaninato) lanthanides.” Dalton Transactions, vol. 40, no. 43, Sep. 2011, pp. 11474-11479. https://xlink.rsc.org/?DOI=c1dt11231g.