Photochemical and Photobiological Sciences, volume 11, issue 7, pages 1220-1232

Controlled surface trap state photoluminescence from CdS QDs impregnated in poly(methyl methacrylate)

Santanu Karan ^{1, 2}

Manisree Majumder ¹

Biswanath Mallik ¹

Hide authors affiliations Show authors affiliations: 2 affiliations

Department of Spectroscopy, Indian Association for the Cultivation of Science, Jadavpur, India |

Polymer Materials Unit, Separation Functional Materials Group, National Institute for Materials Science (NIMS), Tsukuba, Japan |

Publication type: Journal Article

Publication date: 2012-07-01

Springer Nature

Journal: Photochemical and Photobiological Sciences

Quartile SCImago

Quartile WOS

Impact factor: 3.1

ISSN: 1474905X, 14749092

DOI: 10.1039/c2pp25023c

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Physical and Theoretical Chemistry

Abstract

A method of microwave (MW) assisted synthesis was employed to prepare cadmium sulfide (CdS) quantum dots (QDs) in dimethylformamide in the presence of poly(methyl methacrylate) (PMMA). The MW irradiation was carried out for a fixed time of 20–30 s and the size of QDs varied from 2.9–5.5 nm. Before each irradiation the solution was cooled down to ambient temperature and the irradiation process was repeated six times. An increase in the intensity and red shift of the characteristic UV-vis absorption peak originating from CdS QDs were observed with repeated MW irradiation, suggesting that the amount of generated CdS QDs increased within the PMMA network and aggregated with repeated MW irradiation. MW irradiation could influence selectively the nucleation and growing rates of PMMA-CdS QDs systems. The broadness and large Stokes shift of the emission from Cd2+-rich PMMA-CdS QDs was due to the surface trap state photoluminescence. The recombination of shallow trapped electrons and shallow trapped holes has been considered as the primary source of the surface trap state photoluminescence in Cd2+-rich PMMA-CdS QDs. The photoluminescence lifetime was observed to be decreased sharply when the amount of QDs was less, showing the emission decay was dependent on the surface property of PMMA-CdS QDs. The origin of the longer lifetime was due to the involvement of surface trap states and dependent on the amount of CdS QDs present within PMMA and its environment. The effect of the concentration of Cd2+, S2− and PMMA on the generation of CdS QDs within PMMA and the effect of repeated MW irradiation on the optical properties was studied and the results are discussed in this article.

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Citations by journals

	1 2 3
International Journal of Hydrogen Energy	International Journal of Hydrogen Energy, 3, 7.14% International Journal of Hydrogen Energy 3 publications, 7.14%
ACS applied materials & interfaces	ACS applied materials & interfaces, 3, 7.14% ACS applied materials & interfaces 3 publications, 7.14%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 3, 7.14% Journal of Materials Chemistry C 3 publications, 7.14%
Nanomaterials	Nanomaterials, 2, 4.76% Nanomaterials 2 publications, 4.76%
Journal of Luminescence	Journal of Luminescence, 2, 4.76% Journal of Luminescence 2 publications, 4.76%
Journal of the American Chemical Society	Journal of the American Chemical Society, 2, 4.76% Journal of the American Chemical Society 2 publications, 4.76%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 2, 4.76% Journal of Physical Chemistry C 2 publications, 4.76%
ACS Omega	ACS Omega, 2, 4.76% ACS Omega 2 publications, 4.76%
Journal of Applied Physics	Journal of Applied Physics, 1, 2.38% Journal of Applied Physics 1 publication, 2.38%
Journal of Materials Science: Materials in Electronics	Journal of Materials Science: Materials in Electronics, 1, 2.38% Journal of Materials Science: Materials in Electronics 1 publication, 2.38%
Chemosphere	Chemosphere, 1, 2.38% Chemosphere 1 publication, 2.38%
Semiconductor Science and Technology	Semiconductor Science and Technology, 1, 2.38% Semiconductor Science and Technology 1 publication, 2.38%
Nano-Structures and Nano-Objects	Nano-Structures and Nano-Objects, 1, 2.38% Nano-Structures and Nano-Objects 1 publication, 2.38%
Materials Science in Semiconductor Processing	Materials Science in Semiconductor Processing, 1, 2.38% Materials Science in Semiconductor Processing 1 publication, 2.38%
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 1, 2.38% Journal of Colloid and Interface Science 1 publication, 2.38%
Thin Solid Films	Thin Solid Films, 1, 2.38% Thin Solid Films 1 publication, 2.38%
Materials Chemistry and Physics	Materials Chemistry and Physics, 1, 2.38% Materials Chemistry and Physics 1 publication, 2.38%
Polymer Composites	Polymer Composites, 1, 2.38% Polymer Composites 1 publication, 2.38%
Chemistry - A European Journal	Chemistry - A European Journal, 1, 2.38% Chemistry - A European Journal 1 publication, 2.38%
Chemical Reviews	Chemical Reviews, 1, 2.38% Chemical Reviews 1 publication, 2.38%
Nano Letters	Nano Letters, 1, 2.38% Nano Letters 1 publication, 2.38%
RSC Advances	RSC Advances, 1, 2.38% RSC Advances 1 publication, 2.38%
Nanoscale	Nanoscale, 1, 2.38% Nanoscale 1 publication, 2.38%
New Journal of Chemistry	New Journal of Chemistry, 1, 2.38% New Journal of Chemistry 1 publication, 2.38%
Nanotechnologies in Russia	Nanotechnologies in Russia, 1, 2.38% Nanotechnologies in Russia 1 publication, 2.38%
Materials Technology	Materials Technology, 1, 2.38% Materials Technology 1 publication, 2.38%
Materials Today: Proceedings	Materials Today: Proceedings, 1, 2.38% Materials Today: Proceedings 1 publication, 2.38%
Russian Chemical Reviews	Russian Chemical Reviews, 1, 2.38% Russian Chemical Reviews 1 publication, 2.38%
Nano Express	Nano Express, 1, 2.38% Nano Express 1 publication, 2.38%
	1 2 3

Citations by publishers

	2 4 6 8 10 12
Elsevier	Elsevier, 12, 28.57% Elsevier 12 publications, 28.57%
American Chemical Society (ACS)	American Chemical Society (ACS), 11, 26.19% American Chemical Society (ACS) 11 publications, 26.19%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 6, 14.29% Royal Society of Chemistry (RSC) 6 publications, 14.29%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 4.76% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 4.76%
IOP Publishing	IOP Publishing, 2, 4.76% IOP Publishing 2 publications, 4.76%
Wiley	Wiley, 2, 4.76% Wiley 2 publications, 4.76%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 1, 2.38% American Institute of Physics (AIP) 1 publication, 2.38%
Springer Nature	Springer Nature, 1, 2.38% Springer Nature 1 publication, 2.38%
Pleiades Publishing	Pleiades Publishing, 1, 2.38% Pleiades Publishing 1 publication, 2.38%
Taylor & Francis	Taylor & Francis, 1, 2.38% Taylor & Francis 1 publication, 2.38%
Research Square Platform LLC	Research Square Platform LLC, 1, 2.38% Research Square Platform LLC 1 publication, 2.38%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 2.38% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 2.38%
	2 4 6 8 10 12

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Karan S. et al. Controlled surface trap state photoluminescence from CdS QDs impregnated in poly(methyl methacrylate) // Photochemical and Photobiological Sciences. 2012. Vol. 11. No. 7. pp. 1220-1232.

GOST all authors (up to 50) Copy

Karan S., Majumder M., Mallik B. Controlled surface trap state photoluminescence from CdS QDs impregnated in poly(methyl methacrylate) // Photochemical and Photobiological Sciences. 2012. Vol. 11. No. 7. pp. 1220-1232.

RIS |

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TY - JOUR

DO - 10.1039/c2pp25023c

UR - https://doi.org/10.1039/c2pp25023c

TI - Controlled surface trap state photoluminescence from CdS QDs impregnated in poly(methyl methacrylate)

T2 - Photochemical and Photobiological Sciences

AU - Karan, Santanu

AU - Majumder, Manisree

AU - Mallik, Biswanath

PY - 2012

DA - 2012/07/01 00:00:00

PB - Springer Nature

SP - 1220-1232

IS - 7

VL - 11

SN - 1474-905X

SN - 1474-9092

ER -

BibTex |

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BibTex Copy

@article{2012_Karan,

author = {Santanu Karan and Manisree Majumder and Biswanath Mallik},

title = {Controlled surface trap state photoluminescence from CdS QDs impregnated in poly(methyl methacrylate)},

journal = {Photochemical and Photobiological Sciences},

year = {2012},

volume = {11},

publisher = {Springer Nature},

month = {jul},

url = {https://doi.org/10.1039/c2pp25023c},

number = {7},

pages = {1220--1232},

doi = {10.1039/c2pp25023c}

}

MLA

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Karan, Santanu, et al. “Controlled surface trap state photoluminescence from CdS QDs impregnated in poly(methyl methacrylate).” Photochemical and Photobiological Sciences, vol. 11, no. 7, Jul. 2012, pp. 1220-1232. https://doi.org/10.1039/c2pp25023c.

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Springer Nature

Journal

Photochemical and Photobiological Sciences

Quartile SCImago

Quartile WOS

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3.1

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1474905X (Print)
14749092 (Electronic)