Open Access
Gold dissolution: towards understanding of noble metal corrosion
Тип публикации: Journal Article
Дата публикации: 2013-07-08
scimago Q1
wos Q2
БС1
SJR: 0.777
CiteScore: 7.6
Impact factor: 4.6
ISSN: 20462069
General Chemistry
General Chemical Engineering
Краткое описание
The electrochemical dissolution of gold is an intricate topic and even though it has been studied for more than 50 years, its understanding remains rather limited. In the current work, we obtain unique information on gold dissolution by using a setup composed of a micro-electrochemical scanning flow cell (SFC) and inductively coupled plasma mass spectrometry (ICP-MS). Thus, comprehensive online gold dissolution profiles during the initial stage of oxidation as a function of the potential, time and pH are presented. A microscopic model explaining the experimental findings is proposed. According to this model, two dissolution mechanisms take place in two different potential regions: at low anodic potentials the dissolution is driven by the place-exchange between metal and adsorbed hydroxyl/oxygen ions, while at higher potentials the oxygen evolution reaction taking place on the surface of gold oxide initiates concomitant gold loss.
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Метрики
172
Всего цитирований:
172
Цитирований c 2025:
21
(12.21%)
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ГОСТ |
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BibTex |
MLA
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ГОСТ
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Cherevko S. et al. Gold dissolution: towards understanding of noble metal corrosion // RSC Advances. 2013. Vol. 3. No. 37. p. 16516.
ГОСТ со всеми авторами (до 50)
Скопировать
Cherevko S., Topalov A. A., Zeradjanin A., Katsounaros I., Mayrhofer K. J. Gold dissolution: towards understanding of noble metal corrosion // RSC Advances. 2013. Vol. 3. No. 37. p. 16516.
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RIS
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TY - JOUR
DO - 10.1039/c3ra42684j
UR - https://doi.org/10.1039/c3ra42684j
TI - Gold dissolution: towards understanding of noble metal corrosion
T2 - RSC Advances
AU - Cherevko, Serhiy
AU - Topalov, Angel A.
AU - Zeradjanin, Aleksandar
AU - Katsounaros, Ioannis
AU - Mayrhofer, Karl J.
PY - 2013
DA - 2013/07/08
PB - Royal Society of Chemistry (RSC)
SP - 16516
IS - 37
VL - 3
SN - 2046-2069
ER -
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BibTex (до 50 авторов)
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@article{2013_Cherevko,
author = {Serhiy Cherevko and Angel A. Topalov and Aleksandar Zeradjanin and Ioannis Katsounaros and Karl J. Mayrhofer},
title = {Gold dissolution: towards understanding of noble metal corrosion},
journal = {RSC Advances},
year = {2013},
volume = {3},
publisher = {Royal Society of Chemistry (RSC)},
month = {jul},
url = {https://doi.org/10.1039/c3ra42684j},
number = {37},
pages = {16516},
doi = {10.1039/c3ra42684j}
}
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MLA
Скопировать
Cherevko, Serhiy, et al. “Gold dissolution: towards understanding of noble metal corrosion.” RSC Advances, vol. 3, no. 37, Jul. 2013, p. 16516. https://doi.org/10.1039/c3ra42684j.