Hybrid organic-inorganic supramolecular systems based on a pyridine end-decorated molybdenum(ii) halide cluster and zinc(ii) porphyrinate
Тип публикации: Journal Article
Дата публикации: 2019-01-03
scimago Q2
wos Q1
БС1
SJR: 0.653
CiteScore: 6
Impact factor: 3.3
ISSN: 14779226, 14779234
PubMed ID:
30648714
Inorganic Chemistry
Краткое описание
Herein, first examples of supramolecular hybrid organic–inorganic cluster-porphyrin [CPn (n = 2, 6)] systems constructed via metal–ligand coordination have been reported. The pyridine end-decorated Mo(II) halide cluster ((Bu4N)2[{Mo6I8}(OOC-C5H4N)6]), possessing remarkable photophysical properties, was chosen as the inorganic part and A2-type zinc porphyrin 5,15-bis[(p-tolyl)porphyrinato(2-)]zinc was selected as the organic part. The crystal structures of CP2 and CP6 hybrids have been characterised by single crystal X-ray diffraction. The CP2 complex is composed of two zinc porphyrins, coordinated to pyridyl moieties of the same cluster molecule, related by an inversion center. In the case of the CP6 complex, each cluster has three pairs of coordinated symmetrically equivalent zinc porphyrins. Also, the formation of supramolecular hybrid CPn (n = 2, 6) systems was unambiguously demonstrated in solution via NMR and UV-Vis spectroscopy titration and diffusion ordered NMR spectroscopy (DOSY).
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Volostnykh M. V. et al. Hybrid organic-inorganic supramolecular systems based on a pyridine end-decorated molybdenum(ii) halide cluster and zinc(ii) porphyrinate // Dalton Transactions. 2019. Vol. 48. No. 5. pp. 1835-1842.
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Volostnykh M. V., Mikhaylov M. A., Sinelshchikova A., Kirakosyan G., Martynov A. G., Grigoriev M. S., Piryazev D. A., Tsivadze A. Y., Sokolov M., Gorbunova Y. G. Hybrid organic-inorganic supramolecular systems based on a pyridine end-decorated molybdenum(ii) halide cluster and zinc(ii) porphyrinate // Dalton Transactions. 2019. Vol. 48. No. 5. pp. 1835-1842.
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TY - JOUR
DO - 10.1039/c8dt04452j
UR - https://xlink.rsc.org/?DOI=C8DT04452J
TI - Hybrid organic-inorganic supramolecular systems based on a pyridine end-decorated molybdenum(ii) halide cluster and zinc(ii) porphyrinate
T2 - Dalton Transactions
AU - Volostnykh, Marina V
AU - Mikhaylov, Maxim A
AU - Sinelshchikova, Anna
AU - Kirakosyan, Gayane
AU - Martynov, Alexander G.
AU - Grigoriev, Mikhail S.
AU - Piryazev, Dmitry A
AU - Tsivadze, Aslan Yu.
AU - Sokolov, Maxim
AU - Gorbunova, Yulia G.
PY - 2019
DA - 2019/01/03
PB - Royal Society of Chemistry (RSC)
SP - 1835-1842
IS - 5
VL - 48
PMID - 30648714
SN - 1477-9226
SN - 1477-9234
ER -
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@article{2019_Volostnykh,
author = {Marina V Volostnykh and Maxim A Mikhaylov and Anna Sinelshchikova and Gayane Kirakosyan and Alexander G. Martynov and Mikhail S. Grigoriev and Dmitry A Piryazev and Aslan Yu. Tsivadze and Maxim Sokolov and Yulia G. Gorbunova},
title = {Hybrid organic-inorganic supramolecular systems based on a pyridine end-decorated molybdenum(ii) halide cluster and zinc(ii) porphyrinate},
journal = {Dalton Transactions},
year = {2019},
volume = {48},
publisher = {Royal Society of Chemistry (RSC)},
month = {jan},
url = {https://xlink.rsc.org/?DOI=C8DT04452J},
number = {5},
pages = {1835--1842},
doi = {10.1039/c8dt04452j}
}
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MLA
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Volostnykh, Marina V., et al. “Hybrid organic-inorganic supramolecular systems based on a pyridine end-decorated molybdenum(ii) halide cluster and zinc(ii) porphyrinate.” Dalton Transactions, vol. 48, no. 5, Jan. 2019, pp. 1835-1842. https://xlink.rsc.org/?DOI=C8DT04452J.
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