Open Access
Functionalized heterocycle-appended porphyrins: Catalysis matters
Inna A Abdulaeva
1, 2, 3, 4
,
Kirill P. Birin
1, 2, 3, 4
,
Daria A. Polivanovskaia
1, 2, 3, 4
,
Yulia G. Gorbunova
1, 2, 3, 4, 5, 6
,
Aslan Tsivadze
1, 2, 3, 4, 5, 6
3
Moscow
4
Russia
|
5
Publication type: Journal Article
Publication date: 2020-11-23
scimago Q1
wos Q2
SJR: 0.777
CiteScore: 7.6
Impact factor: 4.6
ISSN: 20462069
PubMed ID:
35516736
General Chemistry
General Chemical Engineering
Abstract
The scope and limitations of the condensation of labile 2,3-diaminoporphyrin derivatives with aromatic aldehydes to provide functionalized imidazole- and pyrazine-appended porphyrins were investigated in detail. The presence of an acidic catalyst in the reaction was found to be a tool that allows the reaction path to be switched. The influence of the electronic origin of the substituents in the carbonyl components of the condensation on the yields and selectivity of the reaction was revealed. Metal-promoted cross-coupling transformations were found to be convenient for the further targeted construction of functional derivatives based on the prepared bromo-substituted pyrazinoporphyrins. Overall, these strategies provide a versatile technique for the elaboration of a variety of functionalized heterocycle-appended porphyrins for further application in the development of hybrid materials.
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15
Total citations:
15
Citations from 2024:
7
(46%)
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MLA
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GOST
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Abdulaeva I. A. et al. Functionalized heterocycle-appended porphyrins: Catalysis matters // RSC Advances. 2020. Vol. 10. No. 69. pp. 42388-42399.
GOST all authors (up to 50)
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Abdulaeva I. A., Birin K. P., Polivanovskaia D. A., Gorbunova Y. G., Tsivadze A. Functionalized heterocycle-appended porphyrins: Catalysis matters // RSC Advances. 2020. Vol. 10. No. 69. pp. 42388-42399.
Cite this
RIS
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TY - JOUR
DO - 10.1039/d0ra08603g
UR - https://xlink.rsc.org/?DOI=D0RA08603G
TI - Functionalized heterocycle-appended porphyrins: Catalysis matters
T2 - RSC Advances
AU - Abdulaeva, Inna A
AU - Birin, Kirill P.
AU - Polivanovskaia, Daria A.
AU - Gorbunova, Yulia G.
AU - Tsivadze, Aslan
PY - 2020
DA - 2020/11/23
PB - Royal Society of Chemistry (RSC)
SP - 42388-42399
IS - 69
VL - 10
PMID - 35516736
SN - 2046-2069
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2020_Abdulaeva,
author = {Inna A Abdulaeva and Kirill P. Birin and Daria A. Polivanovskaia and Yulia G. Gorbunova and Aslan Tsivadze},
title = {Functionalized heterocycle-appended porphyrins: Catalysis matters},
journal = {RSC Advances},
year = {2020},
volume = {10},
publisher = {Royal Society of Chemistry (RSC)},
month = {nov},
url = {https://xlink.rsc.org/?DOI=D0RA08603G},
number = {69},
pages = {42388--42399},
doi = {10.1039/d0ra08603g}
}
Cite this
MLA
Copy
Abdulaeva, Inna A., et al. “Functionalized heterocycle-appended porphyrins: Catalysis matters.” RSC Advances, vol. 10, no. 69, Nov. 2020, pp. 42388-42399. https://xlink.rsc.org/?DOI=D0RA08603G.