Raman spectroscopy of intermolecular charge transfer complex between a conjugated polymer and an organic acceptor molecule
Тип публикации: Journal Article
Дата публикации: 2007-09-14
SCImago Q1
WOS Q1
БС2
SJR: 0.877
CiteScore: 5.3
Impact factor: 3.7
ISSN: 00219606, 10897690
PubMed ID:
17867778
Physical and Theoretical Chemistry
General Physics and Astronomy
Краткое описание
Intermolecular donor-acceptor charge transfer complex (CTC) formed in the electronic ground state between poly[2-methoxy-5-(2-ethylhexyloxy)-1,4-phenylenevinylene] (MEH-PPV) and 2,4,7-trinitrofluorenone (TNF) has been investigated by Raman and optical absorption spectroscopies. Blending of MEH-PPV and TNF results in appearance of the CTC absorption band in the optical gap of the both components and in changes in the characteristic MEH-PPV Raman bands including shifts, change in bandwidth, and intensity. The experimental data are similar in films and solutions indicating the CTC formation in both. We associate the low-frequency shift of the strongest MEH-PPV Raman band at approximately 1580 cm(-1) reaching 5 cm(-1) with partial electron transfer from MEH-PPV to TNF amounting approximately 0.2e(-). We suggest that polymer conjugated segments can form the CTC of variable composition MEH-PPV:TNF=1:X, where X
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Bruevich V. V. et al. Raman spectroscopy of intermolecular charge transfer complex between a conjugated polymer and an organic acceptor molecule // Journal of Chemical Physics. 2007. Vol. 127. No. 10. p. 104905.
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Bruevich V. V., Makhmutov T. S., Elizarov S., Nechvolodova E., Paraschuk D. Yu. Raman spectroscopy of intermolecular charge transfer complex between a conjugated polymer and an organic acceptor molecule // Journal of Chemical Physics. 2007. Vol. 127. No. 10. p. 104905.
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TY - JOUR
DO - 10.1063/1.2767266
UR - https://doi.org/10.1063/1.2767266
TI - Raman spectroscopy of intermolecular charge transfer complex between a conjugated polymer and an organic acceptor molecule
T2 - Journal of Chemical Physics
AU - Bruevich, V. V.
AU - Makhmutov, T Sh
AU - Elizarov, S.G.
AU - Nechvolodova, E.M.
AU - Paraschuk, D Yu
PY - 2007
DA - 2007/09/14
PB - AIP Publishing
SP - 104905
IS - 10
VL - 127
PMID - 17867778
SN - 0021-9606
SN - 1089-7690
ER -
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BibTex (до 50 авторов)
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@article{2007_Bruevich,
author = {V. V. Bruevich and T Sh Makhmutov and S.G. Elizarov and E.M. Nechvolodova and D Yu Paraschuk},
title = {Raman spectroscopy of intermolecular charge transfer complex between a conjugated polymer and an organic acceptor molecule},
journal = {Journal of Chemical Physics},
year = {2007},
volume = {127},
publisher = {AIP Publishing},
month = {sep},
url = {https://doi.org/10.1063/1.2767266},
number = {10},
pages = {104905},
doi = {10.1063/1.2767266}
}
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MLA
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Bruevich, V. V., et al. “Raman spectroscopy of intermolecular charge transfer complex between a conjugated polymer and an organic acceptor molecule.” Journal of Chemical Physics, vol. 127, no. 10, Sep. 2007, p. 104905. https://doi.org/10.1063/1.2767266.
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