Journal of Chemical Physics, volume 115, issue 2, pages 1028-1040
``On''/``off'' fluorescence intermittency of single semiconductor quantum dots
Publication type: Journal Article
Publication date: 2001-07-08
Journal:
Journal of Chemical Physics
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 4.4
ISSN: 00219606, 10897690
Physical and Theoretical Chemistry
General Physics and Astronomy
Abstract
Single molecule confocal microscopy is used to investigate the detailed kinetics of fluorescence intermittency in colloidal II–VI (CdSe) semiconductor quantum dots. Two distinct modes of behavior are observed corresponding to (i) sustained “on” episodes (τon) of rapid laser absorption/fluorescence cycling, followed by (ii) sustained “off” episodes (τoff) where essentially no light is emitted despite continuous laser excitation. Both on-time and off-time probability densities follow an inverse power law, P(τon/off)∝1/τon/offm, over more than seven decades in probability density and five decades in time. Such inverse power law behavior is an unambiguous signature of highly distributed kinetics with rates varying over 105-fold, in contrast with models for switching between “on” and “off” configurations of the system via single rate constant processes. The unprecedented dynamic range of the current data permits several kinetic models of fluorescence intermittency to be evaluated at the single molecule level and indicate the importance of fluctuations in the quantum dot environment.
Top-30
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Citations by publishers
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American Chemical Society (ACS)
157 publications, 32.85%
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Elsevier
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Optical Society of America
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Taylor & Francis
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Proceedings of the National Academy of Sciences (PNAS)
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2 publications, 0.42%
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IEEE
2 publications, 0.42%
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The Electrochemical Society of Japan
1 publication, 0.21%
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1 publication, 0.21%
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1 publication, 0.21%
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1 publication, 0.21%
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1 publication, 0.21%
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1 publication, 0.21%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Kuno M. et al. ``On''/``off'' fluorescence intermittency of single semiconductor quantum dots // Journal of Chemical Physics. 2001. Vol. 115. No. 2. pp. 1028-1040.
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Kuno M., Fromm D. P., Hamann H., Gallagher A., Nesbitt D. J. ``On''/``off'' fluorescence intermittency of single semiconductor quantum dots // Journal of Chemical Physics. 2001. Vol. 115. No. 2. pp. 1028-1040.
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TY - JOUR
DO - 10.1063/1.1377883
UR - https://doi.org/10.1063/1.1377883
TI - ``On''/``off'' fluorescence intermittency of single semiconductor quantum dots
T2 - Journal of Chemical Physics
AU - Kuno, M
AU - Fromm, D. P.
AU - Hamann, H.F.
AU - Gallagher, A.
AU - Nesbitt, D J
PY - 2001
DA - 2001/07/08 00:00:00
PB - American Institute of Physics (AIP)
SP - 1028-1040
IS - 2
VL - 115
SN - 0021-9606
SN - 1089-7690
ER -
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@article{2001_Kuno,
author = {M Kuno and D. P. Fromm and H.F. Hamann and A. Gallagher and D J Nesbitt},
title = {``On''/``off'' fluorescence intermittency of single semiconductor quantum dots},
journal = {Journal of Chemical Physics},
year = {2001},
volume = {115},
publisher = {American Institute of Physics (AIP)},
month = {jul},
url = {https://doi.org/10.1063/1.1377883},
number = {2},
pages = {1028--1040},
doi = {10.1063/1.1377883}
}
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Kuno, M., et al. “``On''/``off'' fluorescence intermittency of single semiconductor quantum dots.” Journal of Chemical Physics, vol. 115, no. 2, Jul. 2001, pp. 1028-1040. https://doi.org/10.1063/1.1377883.
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