The role of ferroelectric-ferromagnetic layers on the properties of superlattice-based multiferroics
A series of superlattices and trilayers composed of ferromagnetic and ferroelectric or paraelectric layers were grown on (100) SrTiO3 by the pulsed-laser deposition technique. Their structural and magnetoelectric properties were examined. The superlattices made of ferromagnetic Pr0.85Ca0.15MnO3 (PCMO) and a ferroelectric, namely, Ba0.6Sr0.4TiO3 (BST) or BaTiO3, showed enhanced magnetoresistance (MR) at high applied magnetic field, whereas such enhancement was absent in Pr0.85Ca0.15MnO3∕SrTiO3 superlattices, which clearly demonstrates the preponderant role of the ferroelectric layers in this enhanced MR. Furthermore, the absence of enhanced MR in trilayers of PCMO∕BST indicates that the magnetoelectric coupling which is responsible for MR in these systems is stronger in multilayers than in their trilayer counterparts.
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